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排序方式: 共有7114条查询结果,搜索用时 46 毫秒
141.
Faisal Ahmed Carlos Rodríguez-Fernández Henry A. Fernandez Yi Zhang Abde Mayeen Shafi Md Gius Uddin Xiaoqi Cui Hoon Hahn Yoon Naveed Mehmood Andreas C. Liapis Lide Yao Humeyra Caglayan Zhipei Sun Harri Lipsanen 《Advanced functional materials》2023,33(33):2302051
Developing selective and coherent polymorphic crystals at the nanoscale offers a novel strategy for designing integrated architectures for photonic and optoelectronic applications such as metasurfaces, optical gratings, photodetectors, and image sensors. Here, a direct optical writing approach is demonstrated to deterministically create polymorphic 2D materials by locally inducing metallic 1T′-MoTe2 on the semiconducting 2H-MoTe2 host layer. In the polymorphic-engineered MoTe2, 2H- and 1T′- crystalline phases exhibit strong optical contrast from near-infrared to telecom-band ranges (1–1.5 µm), due to the change in the band structure and increase in surface roughness. Sevenfold enhancement of third harmonic generation intensity is realized with conversion efficiency (susceptibility) of ≈1.7 × 10−7 (1.1 × 10−19 m2 V−2) and ≈1.7 × 10−8 (0.3 × 10−19 m2 V−2) for 1T′ and 2H-MoTe2, respectively at telecom-band ultrafast pump laser. Lastly, based on polymorphic engineering on MoTe2, a Schottky photodiode with a high photoresponsivity of 90 AW−1 is demonstrated. This study proposes facile polymorphic engineered structures that will greatly benefit realizing integrated photonics and optoelectronic circuits. 相似文献
142.
Bahoumina Prince Hallil Hamida Lachaud Jean-Luc Rebière Dominique Dejous Corinne Abdelghani Aymen Frigui Kamel Bila Stephane Baillargeat Dominique Zhang Qing Coquet Phillipe Paragua Carlos Pichonat Emmanuelle Happy Henri 《Microsystem Technologies》2022,28(6):1365-1378
Microsystem Technologies - This study presents the results on the feasibility of a resonant planar chemical capacitive sensor in the microwave frequency range suitable for gas detection and... 相似文献
143.
In this paper, the authors study the problem of testing the hypothesis of a block compound symmetry covariance matrix with two-level multivariate observations, taken for m variables over u sites or time points. Through the use of a suitable block-diagonalization of the hypothesis matrix, it is possible to obtain a decomposition of the main hypothesis into two sub-hypotheses. Using this decomposition, it is then possible to obtain the likelihood ratio test statistic as well as its exact moments in a much simpler way. The exact distribution of the likelihood ratio test statistic is then analyzed. Because this distribution is quite elaborate, yielding a non-manageable distribution function, a manageable but very precise near-exact distribution is developed. Numerical studies conducted to evaluate the closeness between this near-exact distribution and the exact distribution show the very good performance of this approximation even for very small sample sizes and the approach followed allows us to extend its validity to situations where the population distributions are elliptically contoured. A real-data example is presented and a simulation study is also conducted. 相似文献
144.
Guilherme Ferreira Gomes Camila Aparecida Diniz Sebastião Simões da CunhaJr. Antonio Carlos AncelottiJr. 《Journal of Failure Analysis and Prevention》2017,17(4):740-749
The investigation of possible failures in composite materials is a matter of very great importance, and the Tsai-Wu criterion is an effective criterion for analyzing those flaws in anisotropic materials and defining whether the material at a given load will or will not suffer structural failure. In this study, an optimization procedure is proposed to minimize the maximum value of Tsai-Wu of laminated composite tubes subject to axial loading. Artificial neural networks and genetic algorithms are chosen as optimization tools. The results of this study show that the developed algorithm converges faster. Then, the maximum Tsai-Wu value is used as the objective function and the fiber orientations are the constraints in the optimization process. The results yielded by them are compared and discussed. Optimal results are compared with respect to the usual initial design. The design approach is recommended for structures where composites are the key load-carrying members such as orthopedic prosthesis. 相似文献
145.
Koen Nickmans Gerardus M. Bögels Carlos Sánchez‐Somolinos Jeffrey N. Murphy Philippe Leclère Ilja K. Voets Albertus P. H. J. Schenning 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(33)
While self‐assembled molecular building blocks could lead to many next‐generation functional organic nanomaterials, control over the thin‐film morphologies to yield monolithic sub‐5 nm patterns with 3D orientational control at macroscopic length scales remains a grand challenge. A series of photoresponsive hybrid oligo(dimethylsiloxane) liquid crystals that form periodic cylindrical nanostructures with periodicities between 3.8 and 5.1 nm is studied. The liquid crystals can be aligned in‐plane by exposure to actinic linearly polarized light and out‐of‐plane by exposure to actinic unpolarized light. The photoalignment is most efficient when performed just under the clearing point of the liquid crystal, at which the cylindrical nanostructures are reoriented within minutes. These results allow the generation of highly ordered sub‐5 nm patterns in thin films at macroscopic length scales, with control over the orientation in a noncontact fashion. 相似文献
146.
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148.
On the Structure of Amorphous Mesoporous Silica Nanoparticles by Aberration‐Corrected STEM
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Sebastian Calderon V Tânia Ribeiro José Paulo S. Farinha Carlos Baleizão Paulo J. Ferreira 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(40)
Mesoporous silica materials have demonstrated a vast spectrum of applications, stimulating an intensive field of study due to their potential use as nanocarriers. Nonetheless, when produced at the nanoscale, their structural characterization is hindered due to the re‐arrangement of the pores. To address this issue, this work combines molecular dynamics simulations with electron microscopy computer simulations and experimental results to provide an insight into the structure of amorphous mesoporous silica nanoparticles. The amorphous silica model is prepared using a simple melt‐quench molecular dynamics method, while the reconstruction of the mesoporous nanoparticles is carried out using a methodology to avoid false symmetry in the final model. Simulated scanning transmission electron microscopy images are compared with experimental images, revealing the existence of structural domains, created by the misalignment of the pores to compensate the surface tension of these spherical nanoparticles. 相似文献
149.
Carlos A. García-Velásquez Valentina Aristizábal-Marulanda Carlos A. Cardona 《Clean Technologies and Environmental Policy》2018,20(7):1599-1613
In this paper, a techno-economic and environmental assessment is performed to compare the stand-alone process and biorefinery ways to produce biodiesel, ethanol and butanol as potential cases for bioenergy production using fresh fruit bunches as raw material. Different levels of integration are considered (e.g., mass and energy integration, non-conventional technologies) along with the analysis of the process scale to determine the economic profitability and environmental impacts of the proposed cases. The results demonstrated that the biodiesel production based on the biorefinery concept has a positive effect on the profitability of the stand-alone process at different scales. The economic results were compared with data reported in the literature. Furthermore, the life cycle analysis of the proposed cases suggested that the deployment of the biorefinery concept at different levels of integration in the oil palm supply chain reduced the environmental impact of the biodiesel production, which was selected as the hotspot of the evaluated cases. 相似文献
150.
In this article, we present a new technique to actuate liquids in microchannels using ground-directed electric discharge generated
by a portable corona device. When an electric discharge is applied, the air in the microchannel is ionized causing a change
in the surface energy. The resulting change in the contact angle induces rapid liquid transport through the channel by capillary
action. In contrast to established plasma treatment this method employs a ground electrode that guides the electric field.
This approach enables rapid treatment of select microchannels and thus provides a means of real-time fluid actuation as opposed
to simply a pretreatment process. Instantaneous fluid velocities show power-law dependence with time and fit theoretical models
at a contact angle of 65°. Average fluid velocities are on the order of 5 cm/s, and thus channels on the order of 1-cm long
are filled in ~0.2 s. To demonstrate the potential of this technique for integrated lab-on-a-chip applications, the method
was employed in serpentine channel, for on-demand fluid routing, to initiate a mixing process, and through an on-chip integrated
microelectrode. 相似文献