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1.
Summary
We report the synthesis of some new backbone fluorinated
polymers of the poly(phenylenevinylene) type. The new polymers
were characterised by NMR, SEC and X-ray powder diffraction. The
charge carrier mobilities were determined using pulse radiolysis
time resolved microwave conductivity (PR-TRMC) and the carrier
mobilities were compared to the similar non-fluorinated
analogues. The changes in charge carrier mobilities as a
function of molecular substitution pattern is discussed in terms
of other materials properties such as electronic structure and
absorption properties. The major result is that it was found
possible for this type of material to alter the electronic
energy levels by molecular substitution without imparting
significant changes in the magnitude of the charge carrier
mobilities and the optical properties. 相似文献
2.
Johannes G. A. Terlingen Gijsbert A. J. Takens Frederik J. Van Der Gaag Allan S. Hoffman Jan Feijen 《应用聚合物科学杂志》1994,52(1):39-53
Poly(acrylic acid) (PAAc) films were treated with either an argon or a tetrafluoromethane (CF4) plasma and subsequently analyzed with X-ray photoelectron spectroscopy (XPS). PAAc films were decarboxylated during both types of plasma treatments. In addition, during the CF4 plasma treatment, the PAAc films became fluorinated. The plasma phase during the argon plasma treatment of PAAc films was investigated with optical emission spectroscopy. It was shown that during this plasma treatment carbon dioxide, water, and possibly hydrogen were liberated from the PAAc surface. By covering the surface of PAAc films with different materials (lithium fluoride, UV fused silica, and glass) during the plasma treatment, it was possible to differentiate between photochemically induced and particle-induced changes of the surface. This method was used to show that decarboxylation during the argon plasma treatment was caused by vacuum UV radiation (wavelength < 150 nm) and the decarboxylation/fluorination during the CF4 plasma treatment was induced by reactive fluorine-containing species from the plasma phase. Furthermore, during both processes, etching of the PAAc surface occurred. Based on these mechanisms, kinetic models were derived that could be used to describe the measured kinetic data adequately. © 1994 John Wiley & Sons, Inc. 相似文献
3.
Frederik Verbist Nikos Deligiannis Marc Jacobs Joeri Barbarien Peter Schelkens Adrian Munteanu Jan Cornelis 《Multimedia Tools and Applications》2013,66(3):405-430
Distributed video coding (DVC) constitutes an original coding framework to meet the stringent requirements imposed by uplink-oriented and low-power mobile video applications. The quality of the side information available to the decoder and the efficiency of the employed channel codes are primary factors determining the success of a DVC system. This contribution introduces two novel techniques for probabilistic motion compensation in order to generate side information at the Wyner-Ziv decoder. The employed DVC scheme uses a base layer, serving as a hash to facilitate overlapped block motion estimation at the decoder side. On top of the base layer, a supplementary Wyner-Ziv layer is coded in the DCT domain. Both proposed probabilistic motion compensation techniques are driven by the actual correlation channel statistics and reuse information contained in the hash. Experimental results report significant rate savings caused by the novel side information generation methods compared to previous techniques. Moreover, the compression performance of the presented DVC architecture, featuring the proposed side-information generation techniques, delivers state-of-the-art compression performance. 相似文献
4.
Andreas Goralczyk Sofya Savicheva Ramin Montazeri Simona Fine Fadoua Mayoussi Pang Zhu Kay Steffen Frederik Kotz-Helmer Dorothea Helmer Bastian E. Rapp 《Advanced Engineering Materials》2023,25(8):2201314
Superhydrophobic coatings are widely applicable, e.g., as self-cleaning surfaces or water–oil separation membranes, yet their wider usage is impeded due to costs of fabrication, size, or substrate limitation. Spray-coating is a versatile coating procedures and might offer a good solution for the fabrication of these superhydrophobic coatings, due to the fact that coatings can be fabricated on various materials in a simple, fast, and inexpensive manner. Most procedures rely on hybrid coatings of hydrophobized nanoparticles and a polymeric matrix, which have several drawbacks including the easy loss of nanoparticles and difficult waste handling. Here, the fabrication of the superhydrophobic material, called Fluoropor, for the first time, by spray-coating on various substrates including metals, tissues, concrete, and glass is presented. It is fabricated by spray-coating a mixture of a highly fluorinated monomer blended with porogens followed by photopolymerization. The superhydrophobicity of the material relies on the porous structure on the micro-/nanoscale across the bulk material and does not require any nanoparticles. Excellent self-cleaning ability of these coatings, resistance against thermal and abrasive impact, and their application as oil–water separation membranes are shown. This versatile applicability is highly promising for real-world application as self-cleaning coatings or oil–water separating membranes. 相似文献
5.
Dennis Heinson York Yannikos Frederik Franke Christian Winter Markus Schneider 《Datenschutz und Datensicherheit - DuD》2010,34(2):75-79
Der Einsatz von Informationstechnologie (IT) in Organisationen bietet viele M?glichkeiten des Missbrauchs. Besch?ftigte k?nnen
sich die besonderen Eigenschaften der IT zunutze machen, um sich etwa in gesch?ftssch?digender Weise Vorteile zu verschaffen.
Gleichzeitig erm?glicht IT aber auch, verbotene Handlungen aufzuspüren und zu belegen (IT-Forensik). Der Beitrag beschreibt
die technische Praxis von IT-forensischen Analysen und geht auf damit verbundene rechtliche Fragestellungen ein. 相似文献
6.
We scan a large class of one-parameter families of elliptic curves for efficient arithmetic. The construction of the class is inspired by toric geometry, which provides a natural framework for the study of various forms of elliptic curves. The class both encompasses many prominent known forms and includes thousands of new forms. A powerful algorithm is described that automatically computes the most compact group operation formulas for any parameterized family of elliptic curves. The generality of this algorithm is further illustrated by computing uniform addition formulas and formulas for generalized Montgomery arithmetic. 相似文献
7.
Richard I. Hartley Frederik Schaffalitzky 《International Journal of Computer Vision》2009,83(3):274-293
In this paper a general procedure is given for reconstruction of a set of feature points in an arbitrary dimensional projective
space from their projections into lower dimensional spaces. This extends the methods applied in the well-studied problem of
reconstruction of scene points in ℘3 given their projections in a set of images. In this case, the bifocal, trifocal and quadrifocal tensors are used to carry
out this computation. It is shown that similar methods will apply in a much more general context, and hence may be applied
to projections from ℘
n
to ℘
m
, which have been used in the analysis of dynamic scenes, and in radial distortion correction. For sufficiently many generic
projections, reconstruction of the scene is shown to be unique up to projectivity, except in the case of projections onto
one-dimensional image spaces (lines), in which case there are two solutions.
Projections from ℘
n
to ℘2 have been considered by Wolf and Shashua (in International Journal of Computer Vision 48(1): 53–67, 2002), where they were applied to several different problems in dynamic scene analysis. They analyzed these projections using
tensors, but no general way of defining such tensors, and computing the projections was given. This paper settles the general
problem, showing that tensor definition and retrieval of the projections is always possible. 相似文献
8.
Frederik J. Hansen Zhiyuan Wu Paul David Anke Mittelstdt Anne Jacobsen Malgorzata J. Podolska Kenia Ubieta Maximilian Brunner Dina Kouhestani Izabela Swierzy Lotta Roßdeutsch Bettina Klsch Isabella Kutschick Susanne Merkel Axel Denz Klaus Weber Carol Geppert Robert Grützmann Alan Bnard Georg F. Weber 《International journal of molecular sciences》2022,23(9)
Immunotherapy has become increasingly important in the treatment of colorectal cancer (CRC). Currently, CD73, also known as ecto-5′-nucleotidase (NT5E), has gained considerable interest as a potential therapeutic target. CD73 is one of the key enzymes catalyzing the conversion of extracellular ATP into adenosine, which in turn exerts potent immune suppressive effects. However, the role of CD73 expression on various cell types within the CRC tumor microenvironment remains unresolved. The expression of CD73 on various cell types has been described recently, but the role of CD73 on B-cells in CRC remains unclear. Therefore, we analyzed CD73 on B-cells, especially on tumor-infiltrating B-cells, in paired tumor and adjacent normal tissue samples from 62 eligible CRC patients. The highest expression of CD73 on tumor-infiltrating B-cells was identified on class-switched memory B-cells, followed by naive B-cells, whereas no CD73 expression was observed on plasmablasts. Clinicopathological correlation analysis revealed that higher CD73+ B-cells infiltration in the CRC tumors was associated with better overall survival. Moreover, metastasized patients showed a significantly decreased number of tumor-infiltrating CD73+ B-cells. Finally, neoadjuvant therapy correlated with reduced CD73+ B-cell numbers and CD73 expression on B-cells in the CRC tumors. As promising new immune therapies are being developed, the role of CD73+ B-cells and their subsets in the development of colorectal cancer should be further explored to find new therapeutic options. 相似文献
9.
Koen Decroos Marc Seefeldt Carsten Ohms Roumen Petrov Frederik Verhaeghe Leo Kestens 《国际钢铁研究》2011,82(8):911-917
The relation between texture and microstructure and the macroscopic solidification direction has been investigated for an austenitic 316L stainless steel weld. The fusion zone has been characterised by EBSD. Texture development has been simulated by thermal Finite Element Analysis coupled with a simple model of preferential <100>‐oriented solidification following the solidification direction. The thermal part is validated by means of thermocouple measurements at several locations on the specimen. The predicted texture is in very good agreement with the measured one. 相似文献
10.