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81.
Yangyang Xu Peilin Deng Guangda Chen Jinxi Chen Ya Yan Kai Qi Hongfang Liu Bao Yu Xia 《Advanced functional materials》2020,30(6)
The rational construction of efficient bifunctional oxygen electrocatalysts is of immense significance yet challenging for rechargeable metal–air batteries. Herein, this work reports a metal–organic framework derived 2D nitrogen‐doped carbon nanotubes/graphene hybrid as the efficient bifunctional oxygen electrocatalyst for rechargeable zinc–air batteries. The as‐obtained hybrid exhibits excellent catalytic activity and durability for the oxygen electrochemical reactions due to the synergistic effect by the hierarchical structure and heteroatom doping. The assembled rechargeable zinc–air battery achieves a high power density of 253 mW cm?2 and specific capacity of 801 mAh gZn?1 with excellent cycle stability of over 3000 h at 5 mA cm?2. Moreover, the flexible solid‐state rechargeable zinc–air batteries assembled by this hybrid oxygen electrocatalyst exhibits a high discharge power density of 223 mW cm?2, which can power 45 light‐emitting diodes and charge a cellphone. This work provides valuable insights in designing efficient bifunctional oxygen electrocatalysts for long‐life metal–air batteries and related energy conversion technologies. 相似文献
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We report on room temperature continuous-wave optically pumped InAs/GaAs quantum dot whispering gallery mode microdisk lasers,heterogeneously integrated on silica/silicon chips.The microdisks are fabricated by photolithography and inductively coupled plasma etching.The lasing wavelength is approximately 1200 nm and the obtained lowest laser threshold is approximately 28μW.The experimental results show an approach of possible integrated Ⅲ-Ⅴ optical active materials on silica/silicon chip for low threshold WGM microdisk lasers. 相似文献
85.
Sisi Liu Chongjian Zhang Shuangyuan Li Yong Xia Kang Wang Kao Xiong Haodong Tang Linyuan Lian Xinxing Liu Ming-Yu Li Manlin Tan Liang Gao Guangda Niu Huan Liu Haisheng Song Daoli Zhang Jianbo Gao Xinzheng Lan Kai Wang Xiao Wei Sun Ye Yang Jiang Tang Jianbing Zhang 《Advanced functional materials》2021,31(9):2006864
Lead chalcogenide quantum dot (QD) infrared (IR) solar cells are promising devices for breaking through the theoretical efficiency limit of single-junction solar cells by harvesting the low-energy IR photons that cannot be utilized by common devices. However, the device performance of QD IR photovoltaic is limited by the restrictive relation between open-circuit voltages (VOC) and short circuit current densities (JSC), caused by the contradiction between surface passivation and electronic coupling of QD solids. Here, a strategy is developed to decouple this restriction via epitaxially coating a thin PbS shell over the PbSe QDs (PbSe/PbS QDs) combined with in situ halide passivation. The strong electronic coupling from the PbSe core gives rise to significant carrier delocalization, which guarantees effective carrier transport. Benefited from the protection of PbS shell and in situ halide passivation, excellent trap-state control of QDs is eventually achieved after the ligand exchange. By a fine control of the PbS shell thickness, outstanding IR JSC of 6.38 mA cm−2 and IR VOC of 0.347 V are simultaneously achieved under the 1100 nm-filtered solar illumination, providing a new route to unfreeze the trade-off between VOC and JSC limited by the photoactive layer with a given bandgap. 相似文献
86.
In this paper, we develop and validate a method to identify computationally efficient site- and patient-specific models of ultrasound thermal therapies from MR thermal images. The models of the specific absorption rate of the transduced energy and the temperature response of the therapy target are identified in the reduced basis of proper orthogonal decomposition of thermal images, acquired in response to a mild thermal test excitation. The method permits dynamic reidentification of the treatment models during the therapy by recursively utilizing newly acquired images. Such adaptation is particularly important during high-temperature therapies, which are known to substantially and rapidly change tissue properties and blood perfusion. The developed theory was validated for the case of focused ultrasound heating of a tissue phantom. The experimental and computational results indicate that the developed approach produces accurate low-dimensional treatment models despite temporal and spatial noises in MR images and slow image acquisition rate. 相似文献
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牛晓丹冯征 《电信工程技术与标准化》2016,(3)
【】:随着中国移动智能网近14年的建设及发展,传统的增值业务已无法满足用户日益更新的业务需求。但从智能网可提供的网络能力来看,有些能力在今后的业务发展中还将被保留或增强。本文基于现有智能网网络架构、业务发展情况,分析了目前业务发展受限的主要问题,提出了未来智能网将进行能力开放的发展思路及未来业务网架构的调整方向,并结合目前智能网设备的情况,现网SCP未来调整及演进方向。 相似文献
89.
Lead poisoning is a serious environmental concern, which is a health threat. Existing technologies always have some drawbacks, which restrict their application ranges, such as real time monitoring. To solve this problem, glutathione was functionalized on the Au-coated gate area of the pseudomorphic high electron mobility transistor (pHEMT) to detect trace amounts of Pb2+. The positive charge of lead ions will cause a positive potential on the Au gate of the pHEMT sensor, which will increase the current between the source and the drain. The response range for Pb2+ detection has been determined in the concentrations from 0.1 pmol/L to 10 pmol/L. To our knowledge, this is currently the best result for detecting lead ions. 相似文献
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