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991.
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The objective of this study was to assess the effectiveness of an engineered shallow water cover in reducing the oxidation of sulfidic mine tailings and thus preventing the development of acid rock drainage. Fresh tailings were submerged under a 0.3-m water cover in experimental field cells. From 1996 to 1998, we followed the chemistry of the interstitial water near the tailings-overlying water interface using in situ dialysis, and determined pH and dissolved oxygen (DO) profiles across the tailing water interface using micro-electrodes. Penetration of DO into the tailings was limited to <7 mm, even in the presence of DO produced by benthic periphyton. Anoxia in the tailings was further demonstrated by the appearance of dissolved sigmaH2S, Fe and Mn in pore water at depths -1.5 cm below the interface. However, there was clear evidence of surface oxidation of the mine tailings at the mm scale (i.e., DO depletion, coupled with localized increases in [H+] and [SO4(2-)]). Mobilization of Cd and Zn from this surface layer was indicated by the presence of sub-surface peaks in the concentrations of these two metals in the tailings interstitial water and by a change in their solid phase partitioning from refractory to more labile fractions. In contrast, mobilization of Cu from tailings was less evident. Unlike previous reports, which suggested that submerged tailings were effectively inert, our results show alteration of the superficial layer over time. 相似文献
994.
Metal uptake by young trees from dredged brackish sediment: limitations and possibilities for phytoextraction and phytostabilisation 总被引:8,自引:0,他引:8
Mertens J Vervaeke P De Schrijver A Luyssaert S 《The Science of the total environment》2004,326(1-3):209-215
Five tree species (Acer pseudoplatanus L., Alnus glutinosa L. Gaertn., Fraxinus excelsior L., Populus alba L. and Robinia pseudoacacia L.) were planted on a mound constructed of dredged sediment. The sediment originated from a brackish river mouth and was slightly polluted with heavy metals. This preliminary study evaluated the use of trees for site reclamation by means of phytoextraction of metals or phytostabilisation. Although the brackish nature of the sediment caused slight salt damage, overall survival of the planted trees was satisfactory. Robinia and white poplar had the highest growth rates. Ash, maple and alder had the highest survival rates (>90%) but showed stunted growth. Ash, alder, maple and Robinia contained normal concentrations of Cd, Cu, Pb and Zn in their foliage. As a consequence these species reduce the risk of metal dispersal and are therefore suitable species for phytostabilisation under the given conditions. White poplar accumulated high concentrations of Cd (8.0 mg kg(-1)) and Zn (465 mg kg(-1)) in its leaves and might therefore cause a risk of Cd and Zn input into the ecosystem because of autumn litter fall. This species is thus unsuitable for phytostabilisation. Despite elevated metal concentrations in the leaves, phytoextraction of heavy metals from the soil by harvesting stem and/or leaf biomass of white poplar would not be a realistic option because it will require an excessive amount of time to be effective. 相似文献
995.
The rates of oxidation of Fe(II) by H(2)O(2) in the presence of sodium perchlorate, sodium nitrate, sodium chloride and sodium sulfate salts (0-1M) have been compared in the study. Experiments were carried out in a batch reactor, in the dark, at pH <3, 25+/-0.5 degrees C and at controlled ionic strength (< or =1M). The experimental results showed that the rates of oxidation of Fe(II) in the presence of chloride, nitrate and perchlorate were identical. In the presence of sulfate, the rate of oxidation of Fe(II) was faster and depended on the pH and the concentration of sulfate. The pseudo second-order rate constants for the reaction of H(2)O(2) with Fe(2+), FeCl(+) and FeSO(4) were determined as 55+/-1, 55+/-1 and 78+/-3 M(-1) s(-1), respectively. 相似文献
996.
997.
基于MCGS组态软件的上位机控制系统设计 总被引:8,自引:0,他引:8
文章以自动插件机为例,介绍了基于MCGS工业组态软件的上位机控制系统的开发与设计,阐述了该系统的构成、功能及MCGS组态软件在该系统中的应用。上位机采用嵌入式WINCE操作系统和MCGS嵌入式组态软件,下位机采用PLC来控制。人机界面的设计主要用MCGS提供的绘图工具箱来完成,各个控制窗口之间的逻辑控制、各个窗口内的功能实现以及各个按钮控件、文本框等图形对象的功能主要用MCGS的脚本语言来完成。上位机与PLC之间的通讯主要通过设备窗口来完成,在设备窗口中建立系统与PLC设备的连接关系,实现对工业过程的实时监控。 相似文献
998.
999.
1000.
研究了钨含量及固溶温度对超级双相不锈钢022Cr25Ni7Mo3.5WCuN耐点腐蚀性能的影响。通过化学浸泡失重法和电化学极化曲线法,测试了超级双相不锈钢022Cr25Ni7Mo3.5WCuN耐点腐蚀性能,并运用Thermo Calc热力学计算辅助分析。结果表明,固溶温度对超级双相不锈钢022Cr25Ni7Mo3.5WCuN耐点腐蚀性能影响效果显著,在1 100 ℃时,022Cr25Ni7Mo3.5WCuN 的耐腐蚀性能达到最佳;在理想的固溶条件下,钨元素有助于钝化膜的形成,钨含量的增加使得022Cr25Ni7Mo3.5WCuN的耐腐蚀性能增强,在钨质量分数为1.5%时,022Cr25Ni7Mo3.5WCuN获得最佳耐腐蚀性能,若钨含量继续增加,打破了α和γ两相的平衡,则耐蚀性能降低。 相似文献