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171.
Fangchao Li Xuliang Zhang Junwei Shi Lujie Jin Jiawei Qiao Junjun Guo Hang Yin Youyong Li Jianyu Yuan Wanli Ma 《Advanced functional materials》2023,33(40):2302542
Organic–inorganic formamidinium lead triiodide (FAPbI3) hybrid perovskite quantum dot (QD) is of great interest to photovoltaic (PV) community due to its narrow band gap, higher ambient stability, and long carrier lifetime. However, the surface ligand management of FAPbI3 QD is still a key hurdle that impedes the design of high-efficiency solar cells. Herein, this study first develops a solution-mediated ligand exchange (SMLE) for preparing FAPbI3 QD film with enhanced electronic coupling. By dissolving optimal methylammonium iodide (MAI) into antisolvent to treat the FAPbI3 QD solution, the SMLE can not only effectively replace the long-chain ligands, but also passivate the A- and X-site vacancies. By combining experimental and theoretical results, this study demonstrates that the SMLE engineered FAPbI3 QD exhibits lower defect density, which is beneficial for fabricating high-quality QD arrays with desired morphology and carrier transport. Consequently, the SMLE FAPbI3 QD based solar cell outputs a champion efficiency of 15.10% together with improved long-term ambient storage stability, which is currently the highest reported value for hybrid perovskite QD solar cells. These results would provide new design principle of hybrid perovskite QDs toward high-performance optoelectronic application. 相似文献
172.
173.
Qiang Chen Hang Li Xuan Lou Jianli Zhang Guangya Hou Jun Lu Yiping Tang 《Advanced functional materials》2023,33(17):2214920
Aqueous ammonium ion hybrid supercapacitor (A-HSC) combines the charge storage mechanisms of surface adsorption and bulk intercalation, making it a low-cost, safe, and sustainable energy storage candidate. However, its development is hindered by the low capacity and unclear charge storage fundamentals. Here, the strategy of phosphate ion-assisted surface functionalization is used to increase the ammonium ion storage capacity of an α-MoO3 electrode. Moreover, the understanding of charge storage mechanisms via structural characterization, electrochemical analysis, and theoretical calculation is advanced. It is shown that NH4+ intercalation into layered α-MoO3 is not dominant in the A-HSC system; rather, the charge storage mainly depends on the adsorption energy of surface “O” to NH4+. It is further revealed that the hydrogen bond chemistry of the coordination between “O” of surface phosphate ion and NH4+ is the reason for the capacity increase of MoO3. This study not only advances the basic understanding of rechargeable aqueous A-HSC but also demonstrates the promising future of surface engineering strategies for energy storage devices. 相似文献
174.
Hanfei Li Fei Han Lulu Wang Laixin Huang Oluwarotimi Williams Samuel Hang Zhao Ruijie Xie Ping Wang Qiong Tian Qingsong Li Yang Zhao Mei Yu Jing Sun Ruofan Yang Xiaomeng Zhou Fei Li Guanglin Li Yi Lu Peizhi Guo Zhiyuan Liu 《Advanced functional materials》2023,33(29):2300859
Stretchable ultra-narrow (e.g., 10 µm in width) microelectrodes are crucial for the electrophysiological monitoring of single cells providing the fundamental understanding to the working mechanism of neuro network or other electrically functional cells. Current fabrication strategies either focus on the preparation of normal stretchable electrodes with hundreds of micrometers or millimeters in width by using inorganic conductive materials or develop conductive organic polymer gel for ultra-narrow electrodes which suffer from low stretchability and instability for long-term implantation, therefore, it is still highly desirable to explore bio-interfacial ultra-narrow stretchable inorganic electrodes. Herein, a hybrid strategy is reported to prepare ultra-narrow multi-channel stretchable microelectrodes without using photolithography or laser-assisting etching. A 10 µm × 10 µm monitoring window is fabricated with enhanced interfacial impedance by the special rough surface. The stretchability achieves to 120% for this 10 µm-width stretchable electrode. Supported by these superior properties, it is demonstrated that the stretchable microelectrodes can detect electrophysiological signals of single cells in vitro and collect electrophysiological signals more precisely in vivo. The reported strategy will open up the accessible preparation of the fine-size stretchable microelectrode. It will significantly improve the resolution of monitoring and stimulation of inorganic stretchable electrodes. 相似文献
175.
Yi Wei Wei Wang Zhennan Wang Hang Yang Xinyu You Yunna Zhao Peipei Dang Hongzhou Lian Jianhua Hao Guogang Li Jun Lin 《Advanced functional materials》2023,33(2):2205829
Bismuth (Bi3+)-included lead-free metal halide (LFMH) materials attract much attention in lighting, display, photodetectors, X-ray detectors, and photovoltaic fields, due to the tunable luminescence and optoelectronic performance in response to crystal and electronic structure, morphology, and particle sizes. This review summarizes Bi3+-included LFMH materials about their preparation approach, crystal and electronic structure properties, luminescence performance, and emerging applications. Notably, Bi3+ ions not only can act as framework cation to construct stable LFMH structure, but can also incorporate into LFMH materials as activators or sensitizers to generate remarkable luminescence tuning and band engineering. The Bi3+ effect on the luminescence and optoelectronic properties of LFMH materials, including, promotion of exciton localization, enhancement of light absorption in near-ultraviolet region, action as sensitizer ions to transfer energy to rare earth or transition metal ions and emission of highly-efficient light is systematically summarized. The proposed structure-luminescence relationship offers guidance for the optimization of current Bi3+-included LFMH materials and the exploitation of new LFMH derivatives. 相似文献
176.
ZnO1-xSx thin films modified by sulfur doping were prepared on glass substrates by chemical bath deposition (CBD) for studying the effect of thiourea concentration on the thin film properties. The obtained ZnO1-xSx thin films were characterized by scanning electron microscopy (SEM), which shows the surfaces of ZnO1-xSx thin films deposited under the thiourea concentration of 0.14 M are more compact. X-ray diffraction (XRD) measurement shows that the ZnO1-xSx thin films with hexagonal crystal structure had strong diffraction peaks and better crystallinity. The optical transmittance of the ZnO1-xSx thin films with 0.14 M thiourea concentration is above 80% in the wavelength range of 300—900 nm. According to the measurement results from spectrophotometer, the ZnO1-xSx band gap energy value Eg varies nonlinearly with different S/(S+O) ratio x, and increases with the increase of x. There is a band gap value of 2.97 eV in the ZnO1-xSx thin films deposited under 0.14 M thiourea concentration. Therefore, the thin films have better structural, optical and electric properties, and are more suitable for the buffer layers of copper indium gallium selenide (CIGS) thin film solar cells. 相似文献
177.
城市绿植为城市生态系统提供自净功能, 起到净化空气以及滞尘降尘等多种环境保护作用, 而滞尘等因素也
会对绿植产生影响。为了研究滞尘对城市绿植叶片光谱特征的影响, 采集了四种常绿绿植 (八角金盘、石楠、香樟和
玉兰) 叶片样本, 使用高光谱激光雷达系统获取高光谱点云数据, 分析了滞尘对叶片光谱特征的影响。分析结果表明:
对于不同种类叶片, 滞尘对可见光波段反射率均有较大影响; 对于同种类叶片, 滞尘对近红外波段的反射率差异影响
较大, 可见光波段的反射率差异为 1.21%∼3.41%, 近红外为 1.76%∼8.49%; 线性四点内插法计算和光谱导数分析表明
滞尘对四种叶片的红边位置无显著影响; 四种叶片的叶面水含量指数 (LWI) 对滞尘的响应程度最小 (均小于 3.7%), 而
比值植被指数 (RVI) 对滞尘的响应程度最大 (除香樟外, 均大于 20.0%), 红边指数 (SDr)、简单比值指数 (SR) 和叶面叶
绿素指数 (LCI) 的响应程度稳定性较差。进一步建立了滞尘植被指数和响应程度的线性相关性拟合模型并进行了检
验, 其中以 LCI 为自变量建立的模型为最稳定拟合模型, 可表示为 y = −1.527x + 0.6597, 决定系数约为 0.88。 相似文献
178.
Wan Hang Mao Yingzhu Cai Yanpeng Li Ran Feng Jingjie Yang Huixia 《Engineering with Computers》2022,38(4):3169-3184
Engineering with Computers - Aerated flow characterized by complex mass transfer processes with multiple hydraulic properties is a common enviro-hydraulics phenomenon, which have a variety of... 相似文献
179.
Chen Rongxin Wang Zhijin Su Hang Xie Shutong Wang Zongyue 《The Journal of supercomputing》2022,78(4):5420-5449
The Journal of Supercomputing - The performance of XPath query is the key factor to the capacity of XML processing. It is an important way to improve the performance of XPath by making full use of... 相似文献
180.
Farrugia Russell Portelli Barnaby Grech Ivan Camilleri Duncan Casha Owen Micallef Joseph Gatt Edward 《Microsystem Technologies》2022,28(6):1451-1465
Microsystem Technologies - The maximum scan angle amplitude of resonating micro-mirrors, intended for micro-projection display applications is limited by air damping. Three-dimensional transient... 相似文献