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41.
42.
Methanol decomposition to synthesis gas over supported Pd catalysts prepared from synthetic anionic clays 总被引:2,自引:0,他引:2
Ryuji Shiozaki Takashi Hayakawa Yan-yong Liu Tomoko Ishii Mikio Kumagai Satoshi Hamakawa Kunio Suzuki Tatehiko Itoh Tetsuya Shishido Katsuomi Takehira 《Catalysis Letters》1999,58(2-3):131-140
Supported Pd or Rh catalysts were prepared by the solid-phase crystallization method starting from hydrotalcite anionic clay
minerals based on [Mg6Al2(OH)16CO
2
2−
]·4H2O as the precursors. The precursors were prepared by a coprecipitation method from the raw materials containing Pd2+ and various trivalent metal ions which can replace each site of Mg2+ and Al3+ in the hydrotalcite. Rh3+ was also used for preparing the catalyst as comparison. The precursors were then thermally decomposed and reduced to form
supported Pd or Rh catalysts and used for the methanol decomposition to synthesis gas. Among the precursors tested, use of
Mg–Cr hydrotalcite containing Pd2+ resulted in the formation of efficient Pd supported catalysts for the production of synthesis gas by selective decomposition
of methanol at low temperature. Although Pd2+ cannot well replace the Mg2+ site in the hydrotalcite, the Pd supported catalyst (Pd/Mg–Cr) prepared by the solid-phase crystallization method formed
highly dispersed Pd metal particles and showed much higher activity than that prepared by the conventional impregnation method.
When the precursor was prepared under mild conditions, more fine particles of Pd metal were formed over the catalyst, resulting
in high activity. It is likely that the high activity may be due to the highly dispersed and stable Pd metal particles assisted
by the role of Cr as the co-catalyst.
This revised version was published online in November 2006 with corrections to the Cover Date. 相似文献
43.
Masugi Inoue Khaled Mahmud Homare Murakami Mikio Hasegawa Hiroyuki Morikawa 《Wireless Personal Communications》2005,35(1-2):53-70
A context-based adaptive communication system is introduced for use in heterogeneous networks. Context includes the user's
presence, location, available network interfaces, network availability, network priority, communication status, terminal features,
and installed applications. An experimental system was developed to clarify the feasibility of using context information to
flexibly control networks and applications. The system operates on a seamless networking platform we developed for heterogeneous
networks. By using contexts, the system can inform the caller and callee of applications they can access, which are available
through the network before communication occurs. Changes in contexts can switch an on-going application to another during
actual communication. These functions provide unprecedented styles of communication. A business scenario for a seamless networking
provider is also presented.
Dr. Morikawa has also been in charge of NICT's Mobile Networking Group.
Masugi Inoue received his B.E. from Kyoto University in 1992 and his M.E. and D.E. from the University of Tokyo in 1994 and 1997, all
in the field of Electrical Engineering. He is currently a senior researcher at the Yokosuka Radio Communications Research
Center under the National Institute of Information and Communications Technology (NICT), Japan, and has been engaged in R&D
on ultrahigh-speed WLANs and mobile networking. He joined the Communications Research Laboratory (CRL) of the Ministry of
Posts and Telecommunications, Japan, in 1997, which was reorganized as NICT in April 2004. He was a visiting researcher at
Polytechnic University in Brooklyn, New York in 2000.
Khaled Mahmud received his B.Sc. (Eng.) in Electrical and Electronics Engineering from the Bangladesh University of Engineering and Technology
in Dhaka in 1991. He received his M.E. and Ph.D. in the same field from Shizuoka University in Japan, in 1997 and 2000, respectively.
He was a research fellow at NICT, Japan, from 2000 to 2004. He is currently an Assistant Professor in the Department of Computer
Science and Engineering at North South University, Bangladesh. His research interests include modulation-demodulation techniques,
software radio, mobile communication systems, wireless Internet, and IP mobility technologies.
Homare Murakami received his B.E. and M.E. in Electronic Engineering from Hokkaido University in 1997 and 1999. In 2004, he received the
Young Investigators Award from IEICE. He is currently a researcher at NICT's Mobile Networking Group. He is also an industrial
PhD student in Aalborg University since 2003. His interest areas are naming scheme, wireless TCP and new transport protocol,
IP mobility, fast handover method, and location management.
Mikio Hasegawa received his B. Eng, M. Eng., and Dr. Eng. in 1995, 1997, and 2000 from Science University of Tokyo. From 1997 to 2000, he
was a Research Fellow of the Japan Society for the Promotion of Science (JSPS). He is currently a senior researcher in Mobile
Networking Group, National Institute of Information and Communications Technology, and a technical advisor in ChaosWare Inc.
His research interests include applications of chaotic dynamical theory, combinatorial optimization, mobile networks, and
ubiquitous computing.
Hiroyuki Morikawa received his B.E., M.E., and D.E. in Electrical Engineering from the University of Tokyo in 1987, 1989, and 1992. He is currently
an Associate Professor in the Department of Frontier Informatics at the University of Tokyo and is in charge of NICT's Mobile
Networking Group. His research interests are in the areas of computer networks, mobile computing/networks, ubiquitous computing,
and network services. He serves as Editor of Transactions of the IEICE and has been on the technical program committees of
IEEE/ACM conferences and workshops. He sits on numerous telecommunications advisory committees and frequently serves as a
consultant to the government. 相似文献
44.
Preliminary Flight Test Program on Telecom and Broadcasting Using High Altitude Platform Stations 总被引:4,自引:0,他引:4
Telecommunication and broadcasting systems using radio-relay/base stations on board the high altitude platforms are expected
to create the largest business market among its possible applications. They could also be integrated with satellite- and terrestrial-based
systems in the future to construct the more powerful mobile and/or broadband networks. Prototype onboard equipment and ground
equipment are being developed on schedule in the fixed, mobile, and broadcasting services. The performance of them will be
demonstrated and evaluated in the preliminary flight tests planned in 2002 using alternative aerial vehicles: a helicopter,
a jet, and a solar-powered unmanned aerial vehicle (UAV), before flight tests using the high altitude airships. This paper
presents activity in Japan on the R&D of wireless access systems using high altitude platform stations and the detail of the
preliminary flight test program.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
45.
Oodo Masayuki Miura Ryu Hori Teruhisa Morisaki Takayuki Kashiki Kanshiro Suzuki Mikio 《Wireless Personal Communications》2002,23(1):3-14
In the World Radiocommunication Conference 2000 (WRC-2000), use of the 31 GHzand 28 GHz bands was permitted for the fixed service (FS) by using highaltitude platform stations (HAPS) in some countries. This paper examines thesharing and compatibility of the HAPS-based FS with the other services usingthe same and adjacent frequency bands and establishes the conditions of thecoexistence with those services. Feasibility of dynamic channel assignment(DCA) scheme among the different communication systems to facilitate thecoexistence is also studied. 相似文献
46.
Identification and field evaluation ofAnomala octiescostata (Coleoptera: Scarabaeidae) sex pheromone
Walter Soares Leal Makoto Hasegawa Masaaki Sawada Mikio Ono Yasuo Ueda 《Journal of chemical ecology》1994,20(7):1643-1655
Using GC-EAD, the sex pheromone of the scarab beetleAnomala octiescostata was identified to be a 8:2 binary mixture of (R,Z)-5-(–)-(oct-1-enyl)oxacyclopentan-2-one and (R,Z)-5-(–)-(dec-1-enyl)oxacyclopentan-2-one. These semiochemicals have been also reported as sex pheromone constituents of otherAnomala species, either geographically or seasonally isolated fromA. octiescostata. Synthetic sex pheromone was highly attractive in the field; 0.1 mg captured significantly more males than two virgin females. Buried traps were significantly more attractive than those positioned at 30, 90, and 150 cm above the ground. In a dose-response test (0.1–100 mg), no saturation due to overdose of pheromone was observed, but in most cases, two dosages differing by 10-fold were not significantly different. Response of males to traps baited with different ratios of the two components was tested in two experiments with randomized blocks and Latin-square designs. Deviation from the natural ratio (8:2) of sex pheromone did not significantly diminish the response of males. Peak flight activity of beetle was recorded at 9:00–10:00 AM JST on sunny days in the end of April 1993.Presented in part at the 10th Annual ISCE Meeting, July 31–August 4, 1993, Clearwater Beach, Florida. 相似文献
47.
48.
Masaaki Hirayama Noriyuki Sonoyama Takeshi Abe Machiko Minoura Masumi Ito Daisuke Mori Atsuo Yamada Ryoji Kanno Takahito Terashima Mikio Takano Kazuhisa Tamura Jun’ichiro Mizuki 《Journal of power sources》2007
A new experimental technique was developed for detecting structure changes at electrode/electrolyte interface of lithium cell using X-ray reflectometry and two-dimensional model electrodes with a restricted lattice-plane. The electrodes were constructed with an epitaxial film of LiCoO2 synthesized by pulsed laser deposition method. The orientation of the epitaxial film depends on the substrate plane; the 2D layer of LiCoO2 is parallel to the SrTiO3 (1 1 1) substrate ((0 0 3)LiCoO2//(1 1 1)SrTiO3), while the 2D layer is perpendicular to the SrTiO3 (1 1 0) substrate ((1 1 0)LiCoO2//(1 1 0)SrTiO3). The anisotropic properties were confirmed by electrochemical measurements. Ex situ X-ray reflectivity measurements indicated that the impurity layer existed on the as-grown LiCoO2 was dissolved and a new SEI layer with lower density was formed after soaking into the electrolyte. In situ X-ray reflectivity measurements indicated that the surface roughness of the intercalation (1 1 0) plane increased with applying voltages, while no significant changes in surface morphology were observed for the intercalation non-active (0 0 3) plane during the pristine stage of the charge–discharge process. 相似文献
49.
The narrow-gap compound semiconductor PbTe has high Hall mobility. The Fermi surface at the L-point in the Brillouin zone
has large anisotropy. In this work, we measured thermomagnetic effects in PbTe thin films to confirm anisotropy of the Nernst
coefficient A
Ne and show Nernst mobility from the ratio of A
Ne and the Seebeck coefficient S: μ
Ne = A
Ne/S. Angular dependences of the Nernst voltage show that A
Ne is independent of the angle between the temperature gradient and the magnetic field, because of the high L-point symmetry.
The calculated Nernst mobility was compared with the Hall mobility. Because the former is smaller, the Mott equation cannot
explain the Seebeck coefficient at room temperature. 相似文献
50.
Yu-Bai Pan Jian-Hui Qiu Mikio Morita Shou-Hong Tan Dongliang Jiang 《Journal of Materials Science》1998,33(5):1233-1237
Silicon carbide (SiC) and aluminium nitride (AlN) were found to form a solid solution at temperatures above 1800°C. Based on this interesting result, the composite was fabricated by mechanical mixing of the SiC and AlN powders, and hot pressed under 40 MPa at 1950°C in an argon atmosphere. The objective was to achieve full density and minimize solid solution formation. During the sintering process, the SiC–AlN system passed through three steps to form the solid solution at the end. First, the AlN particle is vaporized from its surface; next, the evaporated AlN is deposited on the surface of the SiC grains and the AlN particle, accompanied by a reduction in its size, and finally, partial SiC and AlN solid-solution formation on the boundary of the SiC grains. Because of the AlN deposition and solid-solution formation at the boundary of SiC grains, a barrier layer was present on the surface of SiC grains. This leads to the formation of fine grains. The toughening mechanism is thought to be by thermal residual stresses, due to the difference between the coefficients of thermal expansion of the matrix SiC and that of the dispersed AlN particles, and crack deflection around the SiC grains. Therefore, it is that which improves the mechanical properties of the SiC–AlN composite. © 1998 Chapman & Hall 相似文献