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91.
In this paper, we develop and validate a method to identify computationally efficient site- and patient-specific models of ultrasound thermal therapies from MR thermal images. The models of the specific absorption rate of the transduced energy and the temperature response of the therapy target are identified in the reduced basis of proper orthogonal decomposition of thermal images, acquired in response to a mild thermal test excitation. The method permits dynamic reidentification of the treatment models during the therapy by recursively utilizing newly acquired images. Such adaptation is particularly important during high-temperature therapies, which are known to substantially and rapidly change tissue properties and blood perfusion. The developed theory was validated for the case of focused ultrasound heating of a tissue phantom. The experimental and computational results indicate that the developed approach produces accurate low-dimensional treatment models despite temporal and spatial noises in MR images and slow image acquisition rate. 相似文献
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94.
Sisi Liu Chongjian Zhang Shuangyuan Li Yong Xia Kang Wang Kao Xiong Haodong Tang Linyuan Lian Xinxing Liu Ming-Yu Li Manlin Tan Liang Gao Guangda Niu Huan Liu Haisheng Song Daoli Zhang Jianbo Gao Xinzheng Lan Kai Wang Xiao Wei Sun Ye Yang Jiang Tang Jianbing Zhang 《Advanced functional materials》2021,31(9):2006864
Lead chalcogenide quantum dot (QD) infrared (IR) solar cells are promising devices for breaking through the theoretical efficiency limit of single-junction solar cells by harvesting the low-energy IR photons that cannot be utilized by common devices. However, the device performance of QD IR photovoltaic is limited by the restrictive relation between open-circuit voltages (VOC) and short circuit current densities (JSC), caused by the contradiction between surface passivation and electronic coupling of QD solids. Here, a strategy is developed to decouple this restriction via epitaxially coating a thin PbS shell over the PbSe QDs (PbSe/PbS QDs) combined with in situ halide passivation. The strong electronic coupling from the PbSe core gives rise to significant carrier delocalization, which guarantees effective carrier transport. Benefited from the protection of PbS shell and in situ halide passivation, excellent trap-state control of QDs is eventually achieved after the ligand exchange. By a fine control of the PbS shell thickness, outstanding IR JSC of 6.38 mA cm−2 and IR VOC of 0.347 V are simultaneously achieved under the 1100 nm-filtered solar illumination, providing a new route to unfreeze the trade-off between VOC and JSC limited by the photoactive layer with a given bandgap. 相似文献
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96.
We report on room temperature continuous-wave optically pumped InAs/GaAs quantum dot whispering gallery mode microdisk lasers,heterogeneously integrated on silica/silicon chips.The microdisks are fabricated by photolithography and inductively coupled plasma etching.The lasing wavelength is approximately 1200 nm and the obtained lowest laser threshold is approximately 28μW.The experimental results show an approach of possible integrated Ⅲ-Ⅴ optical active materials on silica/silicon chip for low threshold WGM microdisk lasers. 相似文献
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98.
A 1.65-μm three-section distributed Bragg reflector(DBR) laser for CH4 gas sensors is reported.The DBR laser has a wide tunable range covering the R3 and R4 methane absorption line manifolds.The wavelength tunability properties,temperature stability and laser linewidth are characterized and analyzed.Several advantages were demonstrated compared with traditional DFB lasers in harmonic detection. 相似文献
99.
Hongqiang Li Kaining Gan Ran Li Huawei Huang Jiabao Niu Zhipeng Chen Jian Zhou Yan Yu Jieshan Qiu Xiaojun He 《Advanced functional materials》2023,33(1):2208622
Oxygen-regulated Ni-based single-atom catalysts (SACs) show great potential in accelerating the kinetics of electrocatalytic CO2 reduction reaction (CO2RR). However, it remains a challenge to precisely control the coordination environment of Ni O moieties and achieve high activity at high overpotentials. Herein, a facile carbonization coupled oxidation strategy is developed to mass produce NiO clusters-decorated Ni N C SACs that exhibit a high Faradaic efficiency of CO (maximum of 96.5%) over a wide potential range (−0.9 to −1.3 V versus reversible hydrogen electrode) and a high turnover frequency for CO production of 10 120 h−1 even at the high overpotential of 1.19 V. Density functional theory calculations reveal that the highly dispersed NiO clusters induce electron delocalization of active sites and reduce the energy barriers for *COOH intermediates formation from CO2, leading to an enhanced reaction kinetics for CO production. This study opens a new universal pathway for the construction of oxygen-regulated metal-based SACs for various catalytic applications. 相似文献
100.
Zijin Zhao Chunyu Xu Yao Ma Xiaoling Ma Xixiang Zhu Lianbin Niu Liang Shen Zhengji Zhou Fujun Zhang 《Advanced functional materials》2023,33(9):2212149
Filter-free narrowband photomultiplication-type planar heterojunction (PHJ) organic photodetectors (PM-PHOPDs) are first realized by employing a thick front donor layer and an ultrathin PC71BM layer. The thick front donor layer is employed as an optical field adjusting (OFA) layer. The sequentially coated PC71BM will diffuse slightly into OFA layer, which works as interfacial electron traps to capture photogenerated electrons for assisting hole tunneling injection. The P3HT/PC71BM-based PM-PHOPDs exhibit narrowband response with full-width of half-maximum of 32 nm and external quantum efficiency (EQE) of 1700% at 650 nm under −20 V bias. Due to the enhanced hole transport and reduced charge recombination in PHJ compared to those in bulk heterojunction (BHJ), the EQE of P3HT/PC71BM-based narrowband PM-PHOPDs is twice as P3HT:PC71BM BHJ-based narrowband PM-OPDs under the same bias. The response peak of PM-PHOPDs is adjusted from 650 to 695 or 745 nm by incorporating SMPV1 or DRCN5T in OFA layers due to the red-shifted absorption edge. The EQEs of 3600% at 695 nm and 870% at 745 nm are obtained for P3HT:SMPV1 and P3HT:DRCN5T-based PM-PHOPDs under −20 V bias, respectively. This work provides a smart strategy to achieve narrowband PM-OPDs by designing different OFA layers. 相似文献