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31.
The introduction of of web services has led to web service composition being a focus of many researchers. Composing web services using workflows is seen as the most realistic method from an industrial viewpoint. Amongst other method, the use of natural computing methods has been proposed previously to automate web service composition. The need for a fast response when computing the most suitable sequence of services is addressed in this paper. In particular, we propose a novel heuristic immune algorithm with an efficient encoding and mutation method. The algorithm involves two steps: an immune selection operation, which is maintaining antibody population diversity and the clonal selection. The use of a vaccine during the evolution provides heuristic information that accelerates the convergence. Our experimental results illustrate that the proposed heuristic immune algorithm is very effective in improving the convergence speed. We also provide a schema analysis for this method. 相似文献
32.
Ting Tian Shanshan Yin Suo Tu Christian L. Weindl Kerstin S. Wienhold Suzhe Liang Matthias Schwartzkopf Stephan V. Roth Peter Müller-Buschbaum 《Advanced functional materials》2021,31(46):2105644
Cooperative self-assembly (co-assembly) of diblock copolymers (DBCs) and inorganic precursors that takes inspiration from the rich phase separation behavior of DBCs can enable the realization of a broad spectrum of functional nanostructures with the desired sizes. In a DBC assisted sol–gel chemistry approach with polystyrene-block-poly(ethylene oxide) and ZnO, hybrid films are formed with slot-die coating. Pure DBC films are printed as control. In situ grazing-incidence small-angle X-ray scattering measurements are performed to investigate the self-assembly and co-assembly process during the film formation. Combining complementary ex situ characterizations, several distinct regimes are differentiated to describe the morphological transformations from the initially solvent-dispersed to the ultimately solidified films. The comparison of the assembly pathway evidences that the key step in the establishment of the pure DBC film is the coalescence of spherical micelles toward cylindrical domains. Due to the presence of the phase-selective precursor, the formation of cylindrical aggregates in the solution is crucial for the structural development of the hybrid film. The pre-existing cylinders in the ink impede the domain growth of the hybrid film during the subsequent drying process. The precursor reduces the degree of order, prevents crystallization of the PEO block, and introduces additional length scales in the hybrid films. 相似文献
33.
A procedure for producing arrays of self-aligned carbon nanotubes (CNTs) using standard chemical vapor deposition (CVD) is
reported. Using UV photolithography, silicon substrates are patterned with a thin layer of thermally evaporated iron as a
CNT catalyst. The CVD synthesis was carried out over a small temperature range (700°C–800°C) using acetylene and methane gasses,
producing aligned CNT towers. Scanning electron microscopy (SEM) analysis shows a relationship between CNT tower height and
synthesis time. Additionally, results show that impurity particles dramatically effect CNT tower growth. These results indicate
that aligned CNTs can be produced in a desired pattern with height control. 相似文献
34.
Christian Stephan Bernd 《AEUE-International Journal of Electronics and Communications》2006,60(1):20-24
Security for ad hoc network environments has received a lot of attention as of today. Previous work has mainly been focussing on secure routing, fairness issues, and malicious node detection. However, the issue of introducing and conserving trust relationships has received considerably less attention. In this article, we present a scalable method for the use of public key certificates and their revocation in mobile ad hoc networks (MANETs). With the LKN-ad hoc security framework (LKN-ASF) a certificate management protocol has been introduced, bringing PKI technology to MANETs. In addition a performance analysis of two different revocation approaches for MANETs will be presented. 相似文献
35.
36.
Avalanche‐Discharge‐Induced Electrical Forming in Tantalum Oxide‐Based Metal–Insulator–Metal Structures 下载免费PDF全文
Katharina Skaja Christoph Bäumer Oliver Peters Stephan Menzel Marco Moors Hongchu Du Manuel Bornhöfft Christoph Schmitz Vitaliy Feyer Chun‐Lin Jia Claus Michael Schneider Joachim Mayer Rainer Waser Regina Dittmann 《Advanced functional materials》2015,25(46):7154-7162
Oxide‐based metal–insulator–metal structures are of special interest for future resistive random‐access memories. In such cells, redox processes on the nanoscale occur during resistive switching, which are initiated by the reversible movement of native donors, such as oxygen vacancies. The formation of these filaments is mainly attributed to an enhanced oxygen diffusion due to Joule heating in an electric field or due to electrical breakdown. Here, the development of a dendrite‐like structure, which is induced by an avalanche discharge between the top electrode and the Ta2O5‐x layer, is presented, which occurs instead of a local breakdown between top and bottom electrode. The dendrite‐like structure evolves primarily at structures with a pronounced interface adsorbate layer. Furthermore, local conductive atomic force microscopy reveals that the entire dendrite region becomes conductive. Via spectromicroscopy it is demonstrated that the subsequent switching is caused by a valence change between Ta4+ and Ta5+, which takes place over the entire former Pt/Ta2O5‐x interface of the dendrite‐like structure. 相似文献
37.
Shiro Nishiwaki Andreas Burn Stephan Buecheler Martin Muralt Snke Pilz Valerio Romano Reiner Witte Lukas Krainer Gabriel J. Spühler Ayodhya N. Tiwari 《Progress in Photovoltaics: Research and Applications》2015,23(12):1908-1915
Monolithically integrated Cu(In,Ga)Se2 mini‐modules were fabricated in order to reduce the width of patterning related dead area. The Cu(In,Ga)Se2 layers were prepared on soda‐lime glasses using the multistage process at low substrate temperature below 500 °C. A picosecond laser with a wavelength of 532 nm was used for all of the structuring processes (P1, P2, and P3) for the monolithic integration. A “lift‐off” type structuring was applied for P1 and P3, and an “ablation” type was for P2. The laser structuring was optimized to be minimizing the dead area width, and the width of about 70 µm was successfully achieved. A mini‐module, in which the optimized structuring processes were applied for the integration, demonstrated a certified efficiency of 16.6%. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
38.
Petr Kovaricek Peter Nadazdy Eva Pluharova Alica Brunova Riyas Subair Karol Vegso Valentino Libero Pio Guerra Oleksandr Volochanskyi Martin Kalbac Alexander Krasnansky Pallavi Pandit Stephan Volker Roth Alexander Hinderhofer Eva Majkova Matej Jergel Jianjun Tian Frank Schreiber Peter Siffalovic 《Advanced functional materials》2021,31(13):2009007
2D hybrid organic–inorganic perovskites are valued in optoelectronic applications for their tunable bandgap and excellent moisture and irradiation stability. These properties stem from both the chemical composition and crystallinity of the layer formed. Defects in the lattice, impurities, and crystal grain boundaries generally introduce trap states and surface energy pinning, limiting the ultimate performance of the perovskite; hence, an in-depth understanding of the crystallization process is indispensable. Here, a kinetic and thermodynamic study of 2D perovskite layer crystallization on transparent conductive substrates are provided—fluorine-doped tin oxide and graphene. Due to markedly different surface structure and chemistry, the two substrates interact differently with the perovskite layer. A time-resolved grazing-incidence wide-angle X-ray scattering (GIWAXS) is used to monitor the crystallization on the two substrates. Molecular dynamics simulations are employed to explain the experimental data and to rationalize the perovskite layer formation. The findings assist substrate selection based on the required film morphology, revealing the structural dynamics during the crystallization process, thus helping to tackle the technological challenges of structure formation of 2D perovskites for optoelectronic devices. 相似文献
39.
Matthias A. Ruderer Shuai Guo Robert Meier Hsin‐Yin Chiang Volker Körstgens Johannes Wiedersich Jan Perlich Stephan V. Roth Peter Müller‐Buschbaum 《Advanced functional materials》2011,21(17):3382-3391
Studies on the influence of four different solvents on the morphology and photovoltaic performance of bulk‐heterojunction films made of poly(3‐hexylthiophene) (P3HT) and [6,6]‐phenyl‐C61 butyric acid methyl ester (PCBM) via spin‐coating for photovoltaic applications are reported. Solvent‐dependent PCBM cluster formation and P3HT crystallization during thermal annealing are investigated with optical microscopy and grazing‐incidence wide‐angle X‐ray scattering (GIWAXS) and are found to be insufficient to explain the differences in device performance. A combination of atomic force microscopy (AFM), X‐ray reflectivity (XRR), and grazing‐incidence small‐angle X‐ray scattering (GISAXS) investigations results in detailed knowledge of the inner film morphology of P3HT:PCBM films. Vertical and lateral phase separation occurs during spin‐coating and annealing, depending on the solvent used. The findings are summarized in schematics and compared with the IV characteristics. The main influence on the photovoltaic performance arises from the vertical material composition and the existence of lateral phase separation fitting to the exciton diffusion length. Absorption and photoluminescence measurements complement the structural analysis. 相似文献
40.
概述了采用一个激光源能够加工刚性和挠性板的一种新型激光技术,PCB制造商可能采用最小的投资和提高生产率而进入HDI市场。 相似文献