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排序方式: 共有9807条查询结果,搜索用时 31 毫秒
141.
Lingping Kong Jue Gong Qingyang Hu Francesco Capitani Anna Celeste Takanori Hattori Asami Sano-Furukawa Nana Li Wenge Yang Gang Liu Ho-kwang Mao 《Advanced functional materials》2021,31(9):2009131
The soft nature of organic–inorganic halide perovskites renders their lattice particularly tunable to external stimuli such as pressure, undoubtedly offering an effective way to modify their structure for extraordinary optoelectronic properties. Here, using the methylammonium lead iodide as a representative exploratory platform, it is observed that the pressure-driven lattice disorder can be significantly suppressed via hydrogen isotope effect, which is crucial for better optical and mechanical properties previously unattainable. By a comprehensive in situ neutron/synchrotron-based analysis and optical characterizations, a remarkable photoluminescence (PL) enhancement by threefold is convinced in deuterated CD3ND3PbI3, which also shows much greater structural robustness with retainable PL after high peak-pressure compression–decompression cycle. With the first-principles calculations, an atomic level understanding of the strong correlation among the organic sublattice and lead iodide octahedral framework and structural photonics is proposed, where the less dynamic CD3ND3+ cations are vital to maintain the long-range crystalline order through steric and Coulombic interactions. These results also show that CD3ND3PbI3-based solar cell has comparable photovoltaic performance as CH3NH3PbI3-based device but exhibits considerably slower degradation behavior, thus representing a paradigm by suggesting isotope-functionalized perovskite materials for better materials-by-design and more stable photovoltaic application. 相似文献
142.
Tian Dong Shaoxian Li Manukumara Manjappa Peidi Yang Jiangping Zhou Deyin Kong Baogang Quan Xieyu Chen Chen Ouyang Fei Dai Jiaguang Han Chunmei Ouyang Xueqian Zhang Junjie Li Yang Li Jungang Miao Yutong Li Li Wang Ranjan Singh Weili Zhang Xiaojun Wu 《Advanced functional materials》2021,31(24):2100463
Extreme terahertz (THz) science and technologies, the next disruptive frontier in nonlinear optics, provide multifaceted capabilities for exploring strong light-matter interactions in a variety of physical systems. However, current techniques involve the need for an extremely high-field free space THz source that is difficult to generate and has limited investigations to a rather weak and linear regime of light-matter interactions. Therefore, new approaches are being sought for the tight confinement of THz waves that can induce nonlinear effects. Here, a nonlinear “tera-nano” metasurface is demonstrated exhibiting extremely large THz nonlinearity and sensitive self-modulation of resonances at moderate incident THz field strengths. A record deep-subwavelength (≈λ/33 000) confinement of strongly enhanced (≈3200) THz field in a nano-gap (15 nm) exhibits remarkable THz field-tailored nonlinearity. Further, ultrafast injection of photocarriers reveals a competition between nonlinear THz field-induced intervalley scattering and optically driven interband excitations. The results on “tera-nano” metasurfaces enable a novel platform to realize enhanced nonlinear nano/micro composites for field-sensitive extreme THz nonlinear applications without the need for intense THz light sources. 相似文献
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We consider large-scale wireless sensor networks with η nodes, out of which κ are in possession, (e.g., have sensed or collected in some other way) κ information packets. In the scenarios in which network nodes are vulnerable because of, for example, limited energy or a hostile environment, it is desirable to disseminate the acquired information throughout the network so that each of the η nodes stores one (possibly coded) packet so that the original κ source packets can be recovered, locally and in a computationally simple way from any κ(1 + ϵ) nodes for some small ϵ > 0. We develop decentralized Fountain codes based algorithms to solve this problem. Unlike all previously developed schemes, our algorithms are truly distributed, that is, nodes do not know η, κ or connectivity in the network, except in their own neighborhoods, and they do not maintain any routing tables. 相似文献
146.
熔石英玻璃激光损伤的三维应力场研究 总被引:1,自引:0,他引:1
为了研究CO2激光损伤后熔石英玻璃内部的三维应力场分布,采用脉冲CO2激光与熔石英玻璃相互作用的有限元数值模型,计算了脉冲激光停止时熔石英玻璃内部的温度分布,并研究了材料冷却后的内部三维应力分布和表面初始损伤形貌,计算结果与实验结果吻合。以该模型为基础,详细分析了径向和环向应力的三维分布,结果表明,在损伤凹坑附近,径向应力表现为压应力,且在凹坑底部附近取得最大值后,径向应力沿深度方向逐渐转化为拉应力;损伤凹坑附近的环向应力与径向应力相似,均表现为压应力,但压应力沿径向逐渐转化为拉应力,不同深度处的环向应力沿轴向增至最大后逐渐减小。另外,脉冲激光能量的增大导致径向应力与环向应力及其影响范围均有明显增加。研究结果有助于分析激光损伤熔石英玻璃内部的三维应力场,为CO2激光修复工艺的改进提供了理论依据。 相似文献
147.
将脑-机接口(brain-computer interface,BCI)技术与虚拟现实(virtual reality,VR)相结合构成基于虚拟现实的脑-机接口(BCI-VR)新技术是最近在多媒体和娱乐领域出现的一种BCI应用新模式。BCI-VR兼取两者优势互补,同时又相互促进创新,显示出广阔应用前景。本文从BCI-VR系统基本构成、BCI对VR控制和VR对BCI影响等方面,较详细介绍了近年来BCI-VR的主要研究方法、研究进展和成就,并根据作者体会小结了目前存在的难点与未来的可能发展动向,以与读者交流、共同促进BCI-VR新技术的快速发展。 相似文献
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计算无圈有向网络ST可靠性的一个新方法 总被引:3,自引:1,他引:3
本文考虑计算无圈有向网络的ST可靠性问题(至少存在一条从源点s到汇点t的正常运行道路的概率)。文章引进了深度优先搜索(Depth-FirstSearch)有序根树的概念并提出一个新的计算无圈有向网络ST可靠性的拓扑公式。以该公式为基础,我们利用DFS方法提出一个新的计算无圈有向网络ST可靠性算法,它能生成简洁的可靠性表达式,进而有效地计算无圈有向网络的ST可靠性。两个例子例证了我们的结论 相似文献
150.
A novel stacked folded shorted patch antenna for dual-band operation is presented. It has impedance bandwidths (SWR<2) of 22.9 and 20.3% in the lower and the upper bands, respectively. It is 0.0461lambdaL in height and 0.27lambdaL in length, where lambdaL is the free space wavelength at the centre frequency of the lower band. Therefore, it is very suitable for today's multi-band wireless communication systems. 相似文献