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991.
Son Ha Daesin Kim Hyung-Kyu Lim Chong Min Koo Seon Joon Kim Young Soo Yun 《Advanced functional materials》2021,31(32):2101261
The positive effects of a lithiophilic substrate on the electrochemical performance of lithium metal anodes are confirmed in several reports, while the understanding of lithiophilic substrate-guided lithium metal nucleation and growth behavior is still insufficient. In this study, the effect of a lithiophilic surface on lithium metal nucleation and growth behaviors is investigated using a large-area Ti3C2Tx MXene substrate with a large number of oxygen and fluorine dual heteroatoms. The use of the MXene substrate results in a high lithium-ion concentration as well as the formation of uniform solid–electrolyte-interface (SEI) layers on the lithiophilic surface. The solid–solid interface (MXene-SEI layer) significantly affects the surface tension of the deposited lithium metal nuclei as well as the nucleation overpotential, resulting in the formation of uniformly dispersed lithium nanoparticles ( ≈ 10–20 nm in diameter) over the entire MXene surface. The primary lithium nanoparticles preferentially coalesce and agglomerate into larger secondary particles while retaining their primary particle shapes. Subsequently, they form close-packed structures, resulting in a dense metal layer composed of particle-by-particle microstructures. This distinctive lithium metal deposition behavior leads to highly reversible cycling performance with high Columbic efficiencies > 99.0% and long cycle lives of over 1000 cycles. 相似文献
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994.
Qing Pan Timon Rabczuk Chong Chen 《International journal for numerical methods in engineering》2022,123(2):610-633
We present a new isogeometric analysis (IGA) approach based on extended Loop subdivision scheme for solving various geometric flows defined on subdivision surfaces. The studied flows include the second-order, fourth-order, and sixth-order geometric flows, such as averaged mean curvature flow, constant mean curvature flow, and minimal mean-curvature-variation flow, which are generally derived by minimizing the associate energy functionals with -gradient flow respectively. The geometric flows are discretized by means of subdivision based IGA, where the finite element space is formulated by the limit form of the extended Loop subdivision for different initial control meshes. The basis functions, consisting of quartic box-splines corresponding to each subdivided control mesh, are utilized to represent the geometry exactly. For the cases of the evolution of open surfaces with any shape boundary, high-order continuous boundary conditions derived from the mixed variational forms of the geometric flows should be implemented to be consistent with the isogeometric concept. For time discretization, we adopt an adaptive semi-implicit Euler scheme. By several numerical experiments, we study the convergence behaviors of the proposed approach for solving the geometric flows with high-order boundary conditions. Moreover, the numerical results also show the accuracy and efficiency of the proposed method. 相似文献
995.
Dunying Deng Chong Huang Jin Ma Shuxin Bai 《Journal of Materials Science: Materials in Electronics》2018,29(13):10834-10840
Low temperature silver pastes can be widely applied on thin-film switch, flexible printing line and touch screen. In this article, we investigated printability and conductivity of silver pastes with silver wires of different diameters and content, and the conductivity of the silver pastes cured at different temperatures filled with different types silver powders and silver wires. The sheet resistance of silver pastes cured at 100 °C with Ag1 powders and Ag2 powders filled with 10 wt% silver wires of 100 nm diameters is 21.93?±?1.63 and 23.16?±?1.44 Ω/□, which is lower than the same samples cured at 135 °C without silver wire fillers. Tap density of Ag1 and Ag2 powders mixed with silver nanowires is higher than that of Ag3 powders mixed with nanowires, due to a higher filling ratio of Ag1 and Ag2 powders with silver nanowires. SEM results show silver pastes filled with Ag1 and Ag2 powders formed network when silver nanowires were added. 相似文献
996.
Wenyan Ma Lian-Wei Luo Peihua Dong Peiyun Zheng Xiuhua Huang Chong Zhang Jia-Xing Jiang Yong Cao 《Advanced functional materials》2021,31(45):2105027
Recent studies have demonstrated that dihydrophenazine (Pz) with high redox-reversibility and high theoretical capacity is an attractive building block to construct p-type polymer cathodes for dual-ion batteries. However, most reported Pz-based polymer cathodes to date still suffer from low redox activity, slow kinetics, and short cycling life. Herein, a donor–acceptor (D–A) Pz-based conjugated microporous polymer (TzPz) cathode is constructed by integrating the electron-donating Pz unit and the electron-withdrawing 2,4,6-triphenyl-1,3,5-triazine (Tz) unit into a polymer chain. The D–A type structure enhances the polymer conjugation degree and decreases the band gap of TzPz, facilitating electron transportation along the polymer skeletons. Therefore the TzPz cathode for dual-ion battery shows a high reversible capacity of 192 mAh g−1 at 0.2 A g−1 with excellent rate performance (108 mAh g−1 at 30 A g−1), which is much higher than that of its counterpart polymer BzPz produced from 1,3,5-triphenylbenzene (Bz) and Pz (148 and 44 mAh g−1 at 0.2 and 10 A g−1, respectively). More importantly, the TzPz cathode also shows a long and stable cyclability of more than 10 000 cycles. These results demonstrate that the D–A structural design is an efficient strategy for developing high-performance polymer cathodes for dual-ion batteries. 相似文献
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999.
Sichen Gu Si-Wei Zhang Junwei Han Yaqian Deng Chong Luo Guangmin Zhou Yanbing He Guodan Wei Feiyu Kang Wei Lv Quan-Hong Yang 《Advanced functional materials》2021,31(28):2102128
Lithium metal anodes (LMAs) are promising for next-generation batteries but have poor compatibility with the widely used carbonate-based electrolytes, which is a major reason for their severe dendrite growth and low Coulombic efficiency (CE). A nitrate additive to the electrolyte is an effective solution, but its low solubility in carbonates is a problem that can be solved using a crown ether, as reported. A rubidium nitrate additive coordinated with 18-crown-6 crown ether stabilizes the LMA in a carbonate electrolyte. The coordination promotes the dissolution of NO3− ions and helps form a dense solid electrolyte interface that is Li3N-rich which guides uniform Li deposition. In addition, the Rb (18-crown-6)+ complexes are adsorbed on the dendrite tips, shielding them from Li deposition on the dendrite tips. A high CE of 97.1% is achieved with a capacity of 1 mAh cm−2 in a half cell, much higher than when using the additive-free electrolyte (92.2%). Such an additive is very compatible with a nickel-rich ternary cathode at a high voltage, and the assembled full battery with a cathode material loading up to 10 mg cm−2 shows an average CE of 99.8% over 200 cycles, indicating a potential for practical use. 相似文献
1000.
导航传感器在探险、应急、精确制导武器、船舶、航空器导航和定位系统中起着关键作用。针对偏振光罗盘在倾斜状态下误差较大的问题,提出了一种利用加速度计和陀螺仪对偏振光罗盘进行图像校正的方法,设计了一种基于陀螺仪校正的偏振光罗盘系统。首先利用加速度计和陀螺仪计算得到载体姿态角,对偏振光图像数据进行图像校正,采用Stokes矢量法解算大气偏振模式分布,进而提取导航特征点,最后对特征点进行拟合解算出航向角信息。并且进行了静态和动态测试实验,实验结果表明,该算法能够有效的对偏振光罗盘姿态变化引起的误差进行补偿,可以将偏振光罗盘的航向角测量误差控制在1.86°之内,平均误差为0.09°。 相似文献