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71.
Reinhard Miller Dmitri Grigoriev Jürgen Krägel Alexander V. Makievski Valentin B. Fainerman Volodymyr I. Kovalchuk Libero Liggieri Francesca Ravera Michele Ferrari Eva Santini Giuseppe Loglio Victoria Dutschk Thodoris Karapantsios 《Microgravity science and technology》2006,18(3-4):104-107
The utilisation of particle-surfactants nanostructures as stabilising agents represents today the technologic and scientific frontier in the stabilisation of liquid films in emulsion and foams. This topic will be addressed by the proposal STEFAN (STabilisation of Emulsions and FoAms by Nanoparticles), proposed by European groups in the framework of the ESA AO-2004 for Life and Physical Sciences and Applied Research projects Similarly to what can be observed for surfactant-stabilised emulsions and foams, microgravity provides ideal conditions for the investigation of the hierarchy of involved objects: interfacial layer, liquid film, dispersed systems foam or emulsion. Microgravity experiments are planned by refurbishing the Experimental Container FASES for the ISS Fluid Science Laboratory and the facility FASTER for the European Drawer Rack, already under development in existing research programmes. Here the scientific guidelines of the project are presented together with examples and preliminary results on the effect of nano-particle-surfactant structures adsorbed at liquid interfaces. First experimental results have been achieved for particle monolayers at the water/air interface and a thermodynamic model was derived to describe the obtained surface pressure-area isotherms. 相似文献
72.
Before analysing machinery operation in fields, it has to be coped with the problem that the GPS signals of GPS receivers located on the machines contain measurement noise, are time-discrete, and the underlying physical system describing the positions, axial and absolute velocities, angular rates and angular orientation of the operating machines during the whole working time are unknown. This research work presents a new three-dimensional mathematical approach using kinematic relations based on control variables as Euler angular velocities and angles and a discrete target control problem, such that the state control function is given by the sum of squared residuals involving the state and control variables to get such a physical system, which yields a noise-free and piecewise analytic representation of the positions, velocities, angular rates and angular orientation. It can be used for a further detailed study and analysis of the problem of why agricultural vehicles operate in practice as they do. 相似文献
73.
Twinned Growth of Metal‐Free,Triazine‐Based Photocatalyst Films as Mixed‐Dimensional (2D/3D) van der Waals Heterostructures 下载免费PDF全文
Dana Schwarz Yu Noda Jan Klouda Karolina Schwarzová‐Pecková Ján Tarábek Jiří Rybáček Jiří Janoušek Frank Simon Maksym V. Opanasenko Jiří Čejka Amitava Acharjya Johannes Schmidt Sören Selve Valentin Reiter‐Scherer Nikolai Severin Jürgen P. Rabe Petra Ecorchard Junjie He Miroslav Polozij Petr Nachtigall Michael J. Bojdys 《Advanced materials (Deerfield Beach, Fla.)》2017,29(40)
Design and synthesis of ordered, metal‐free layered materials is intrinsically difficult due to the limitations of vapor deposition processes that are used in their making. Mixed‐dimensional (2D/3D) metal‐free van der Waals (vdW) heterostructures based on triazine (C3N3) linkers grow as large area, transparent yellow‐orange membranes on copper surfaces from solution. The membranes have an indirect band gap (E g,opt = 1.91 eV, E g,elec = 1.84 eV) and are moderately porous (124 m2 g?1). The material consists of a crystalline 2D phase that is fully sp2 hybridized and provides structural stability, and an amorphous, porous phase with mixed sp2–sp hybridization. Interestingly, this 2D/3D vdW heterostructure grows in a twinned mechanism from a one‐pot reaction mixture: unprecedented for metal‐free frameworks and a direct consequence of on‐catalyst synthesis. Thanks to the efficient type I heterojunction, electron transfer processes are fundamentally improved and hence, the material is capable of metal‐free, light‐induced hydrogen evolution from water without the need for a noble metal cocatalyst (34 µmol h?1 g?1 without Pt). The results highlight that twinned growth mechanisms are observed in the realm of “wet” chemistry, and that they can be used to fabricate otherwise challenging 2D/3D vdW heterostructures with composite properties. 相似文献
74.
Jens Laube Valentin Baric Samir Salameh Lutz Mädler Lucio Colombi Ciacchi 《Granular Matter》2018,20(2):28
We develop a novel coarse-grained contact model for Discrete Element Method simulations of \(\hbox {TiO}_2\) nanoparticle films subjected to mechanical stress. All model elements and parameters are derived in a self-consistent and physically sound way from all-atom Molecular Dynamics simulations of interacting particles and surfaces. In particular, the nature of atomic-scale friction and dissipation effects is taken into account by explicit modelling of the surface features and water adsorbate layers that strongly mediate the particle-particle interactions. The quantitative accuracy of the coarse-grained model is validated against all-atom simulations of \(\hbox {TiO}_2\) nanoparticle agglomerates under tensile stress. Moreover, its predictive power is demonstrated with calculations of force-displacement curves of entire nanoparticle films probed with force spectroscopy. The simulation results are compared with Atomic Force Microscopy and Transmission Electron Microscopy experiments. 相似文献
75.
We derive explicit expressions in the frame of the optical indicatrix for the second-order effective nonlinearity in biaxial crystals with point groups 2, m, and 1, governing the conversion efficiency in three-wave nonlinear optical interactions. The tabulated expressions for the monoclinic symmetry classes 2 and m are valid for all possible orientations of the optical indicatrix relative to the crystallographic frame and for propagation along an arbitrary direction outside the principal planes. They can be used for direct estimation of the effective nonlinearity in the same frame where the phase-matching loci are calculated. The relevant properties and conventions used for the newly emerging acentric monoclinic crystals belonging to the borate family are summarized and tabulated. The derivations are expected to help establish adherence to uniform nomenclature and conventions for these novel inorganic nonlinear crystals, and to eliminate ambiguity and increasing confusion in the literature and in the industrial specifications. The general expressions for the effective nonlinearity are reduced for triclinic crystals of point group 1 to simplified forms in the principal planes. 相似文献
76.
The temperature dependence has been determined for the wetting by molten aluminum of materials based on aluminum oxide (polycor and corundum). A temperature range has been identified in which the wetting increases significantly. There is no effect on the wetting characteristics of these oxide materials from the addition to the aluminum of up to 25% silicon, 33% copper, or 6% nickel. 相似文献
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