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Hongbing Song Lei Liu Bingxiao Feng Haozhong Wang Meng Xiao Hengjun Gai Yubao Tang Xiaofei Qu Tingting Huang 《中国化学工程学报》2021,40(12):293-303
In this work, modified g-C3N4 was fabricated successfully by calcination of ionic liquid (IL) and urea. The addition of IL changed the polymerization mode of urea, induced the self-assembly of urea molecules, modified the morphological structure of the tightly packed g-C3N4, and extended the electron conjugation system. When using 1-butyl-3-methylimidazolium chloride ([Bmim]Cl) as a modifier, the heteroatom Cl could be inserted into the g-C3N4 to optimize the electronic structure. The results of characterizations indicate that the unique structure of modified g-C3N4 has an expanded electron delocalization range, introduces an interlayer charge transmission channel, promotes the charge transmission, reduces the band gap, enhances the absorption of visible light, and inhibits electron-hole recombination. Modified g-C3N4 showed excellent photocatalytic performance for the degradation of rhodamine B and tetracycline. Furthermore, the effect of different anions in 1-butyl-3-methylimidazolium salts ([Bmim]Cl, [Bmim]Br, [Bmim][BF4], and [Bmim][PF6]) on the structure and function of g-C3N4 are discussed. 相似文献
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Chung-Kuan Wu Ji-Fan Lin Tzong-Shyuan Lee Yu Ru Kou Der-Cherng Tarng 《International journal of molecular sciences》2021,22(7)
TRPA1, a nonselective cation channel, is expressed in sensory afferent that innervates peripheral targets. Neuronal TRPA1 can promote tissue repair, remove harmful stimuli and induce protective responses via the release of neuropeptides after the activation of the channel by chemical, exogenous, or endogenous irritants in the injured tissue. However, chronic inflammation after repeated noxious stimuli may result in the development of several diseases. In addition to sensory neurons, TRPA1, activated by inflammatory agents from some non-neuronal cells in the injured area or disease, might promote or protect disease progression. Therefore, TRPA1 works as a molecular sentinel of tissue damage or as an inflammation gatekeeper. Most kidney damage cases are associated with inflammation. In this review, we summarised the role of TRPA1 in neurogenic or non-neurogenic inflammation and in kidney disease, especially the non-neuronal TRPA1. In in vivo animal studies, TRPA1 prevented sepsis-induced or Ang-II-induced and ischemia-reperfusion renal injury by maintaining mitochondrial haemostasis or via the downregulation of macrophage-mediated inflammation, respectively. Renal tubular epithelial TRPA1 acts as an oxidative stress sensor to mediate hypoxia–reoxygenation injury in vitro and ischaemia–reperfusion-induced kidney injury in vivo through MAPKs/NF-kB signalling. Acute kidney injury (AKI) patients with high renal tubular TRPA1 expression had low complete renal function recovery. In renal disease, TPRA1 plays different roles in different cell types accordingly. These findings depict the important role of TRPA1 and warrant further investigation. 相似文献
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Margarida Taborda Duarte H. Y. Liu S. Q. Kou P. -A. Lindqvist K. Miskovsky 《Journal of Materials Engineering and Performance》2005,14(1):104-111
The importance of the microstructural parameters in rock mechanical behavior has been investigated by several authors. Moreover,
the Weibull statistical model has been used to characterize the heterogeneity of several materials on the basis of the concept
that the microscopic defects within the material determine their mechanical strength. The modeling of different rocks is a
topic that is fundamental for the prediction of rock fragmentation. In this article, the analysis of rock microstructure is
performed using the microstructural modeling approach, which consists of the simplification, quantification, and modeling
of the main properties of rock microstructure. The grain size, grain shape, and microcracks are modeled by means of statistical
density functions, namely, Cauchy, chi-squared, exponential, extreme value, gamma, Laplace, normal, uniform, and Weibull.
It is found that the Weibull distribution is the most appropriate statistical model of the grain size and grain shape, when
compared with the other eight statistical models. Regarding microcracks, the results show that the gamma distribution is the
most appropriate model. The Weibull and gamma distributions are then used to analyze the heterogeneity of the microstructure.
This is done by comparison of the statistical models of each microstructural property evaluated in several thin sections of
the same rock. It is found that with respect to grain size and grain shape, the rock is homogeneous, while the size distribution
of the microcracks shows a clear trend toward less homogeneity. The microstructural modeling approach is important for modeling,
characterizing, and analyzing the microstructure of rock material. Among other applications, it can be used to explain differences
in the mechanical behavior obtained in testing several specimens. 相似文献
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采用渗流铸造工艺制备了钨丝增强不同Nb含量的Zr基金属玻璃复合材料,利用X-Ray衍射、扫描电镜以及电子探针考察了复合材料界面反应和界面扩散情况,研究了基体合金中的Nb含量对复合材料界面反应和界面扩散的影响。结果表明:对Zr55Al10Ni5Cu30基复合材料,渗流时,钨丝与液相中的Zr发生界面包晶反应,生成W5Zr3界面相,并使界面位置向液相方向移动。在Zr55Al10Ni5Cu30合金的基础上添加Nb,发现Nb优先在钨丝界面偏聚,降低了Zr在钨丝界面的偏聚和活度,抑制钨丝与液相中的Zr包晶反应的发生,没有生成W5Zr3界面相,界面处只存在简单的扩散层。同时发现Zr元素在钨丝中的扩散系数降低,此时界面位置向钨丝方向移动。 相似文献
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以带有同步组装技术的分离式Hopkinson压杆装置作为热模拟装置,采用基于MTS(Mechanical Threshold Stress)模型建立的FCC晶体结构的动态本构方程,确定了定向凝固水平连铸多晶铜动态本构方程参数,研究了其动态冲击特性,获得高温段(685K-1085K)的理论应力-应变曲线与实验曲线相当吻合,而在低温段(低于685K)的理论曲线与实验曲线出入较大。结果也表明定向凝固水平连铸多晶铜在485K和685K之间有一温度能使其回复能达到阀值。 相似文献
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