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11.
Siqi Yu Qin Wang Jianwei Wang Yong Xiang Xiaobin Niu Tingshuai Li 《International Journal of Hydrogen Energy》2021,46(27):14331-14337
Artificial nitrogen fixation is emerging as a promising approach for synthesis of ammonia at mild conditions. Inspired by biological nitrogen fixation based on bacteria containing iron, zinc doped Fe2O3 nanoparticles are proposed as an efficient and earth abundant electrocatalyst for converting N2 to NH3. In neutral media, it achieves a maximum Faradaic efficiency (FE) of 10.4% and a large NH3 yield rate of 15.1 μg h?1 mg?1cat. at ?0.5 V vs. reversible hydrogen electrode. This catalyst also exhibits excellent selectivity and stability. Theoretical calculations suggest the reaction follows the associative enzymatic mechanism and it has a barrier of as low as 0.68 eV. 相似文献
12.
通过工程实例及理论分析 ,对横向风振“锁住区”问题进行了探讨 ,对《建筑结构荷载规范》(GB5 0 0 0 9— 2 0 0 1 )中有关这一方面内容存在的一些问题进行了分析 ,希望对工程设计人员能有所帮助 相似文献
13.
14.
M.Y. Shen Z.B. ZhangX.L. Niu 《Computer Methods in Applied Mechanics and Engineering》2003,192(25):2703-2725
The generalized compact (GC) schemes and some of their important properties are presented. And a new way for constructing high order accuracy and high-resolution GC schemes is presented. The schemes constructed by using this way could satisfy some principles and demands prescribed in advance to ensure some desired properties to the schemes, such as the principle about suppression of the oscillations, the principle of stability, the order of accuracy and number of scheme points, etc. As two examples, a three-point third-order compact scheme and a three-point fifth-order GC scheme satisfying the principle about suppression of the oscillations and the principle of stability are described in this paper. Numerical results show that these schemes are shock-capturing. The time-dependent boundary conditions proposed by Thompson are well employed when the algorithm is applied to the Euler equations of gas dynamics. Fourier analysis shows that the resolution characteristics are spectral-like. 相似文献
15.
Prolog逻辑程序设计语言具有不同于传统程序设计语言的特点.本文根据测试Prolog程序的实践,提出了一系列为Prolog程序生成测试用例的准则.按这些准则测试实际程序效果良好.这是在逻辑程序测试新领域迈出的一步. 相似文献
16.
通过正交试验研究了各工艺量数以钢/铝合金液固相复合性能的影响,最佳工艺条件为铝合金液体温度790℃,钢板表面处理为酸洗+钢刷+5%的氟钛酸钾助焊剂,复合压力为39.2MPa,组织观察表面界面脆性化合物的形成是导致结合强度降低的一个重要因素。 相似文献
17.
18.
Y. Xun R. Rodriguez E. J. Lavernia F. A. Mohamed 《Metallurgical and Materials Transactions A》2005,36(10):2849-2859
The present article deals with the processing and microstructural evolution of powder metallurgy (PM) Zn-22Al pct eutectoid
alloy. The powder material was produced through inert gas atomization and then cryomilled in liquid nitrogen. The milled powder
particles were consolidated by hot isostatic pressing (“hipping”) followed by thermomechanical treatment, resulting in a two-phase
microstructure. The microstructures were characterized using scanning electron microscopy (SEM) and transmission electron
microscopy (TEM). The principal processing factors and microstructural characteristics associated with the major processing
steps, including spray atomization, mechanical milling (MM), consolidation, and heat treatment, were evaluated and discussed.
Hot isostatic pressing and extrusion followed by heat treatment to produce the superplastic structure (Al-rich phase and Zn-rich
phase) are effective in elimination porosity. A TEM examination of the microstructure of the alloy after processing reveals
the presence of nanodispersion particles that are not uniformly distributed. The formation of the dispersions was attributed
to the interaction between the powder material (primarily Al phase) and environmental elements such as oxygen and nitrogen
during milling. Moreover, the size and distribution of the dispersions present in the bulk material met the anticipated requirements
for serving as inhibitors for grain growth and barriers for dislocation movement. The TEM observations on crept specimens
reveal extensive dislocation/dispersion interactions. 相似文献
19.
In order to study water-gas transport processes in the gas-diffusion-layer (GDL) of a proton exchange membrane (PEM) fuel cell system, a multiphase, multiple-relaxation-time lattice Boltzmann model is presented in this work. The model is based on the mean-field diffuse interface theory and can handle the multiphase flows with large density ratios and various viscosities. By using the standard bounce back boundary condition and an approximate average scheme for the non-slip and wetting boundary walls, respectively, detailed liquid-gas transportation in the GDL, in which exact boundary condition is difficult to be implemented, can be simulated. Unlike most of lattice Boltzmann methods based on the Bhatnagar–Gross–Krook collision operator, the present model shows a viscosity-independent velocity field, which is very important in simulating multiphase flows where various viscosities coexist. We validate our model by simulating a static droplet on a wetting wall and compare with theoretical predictions. Then, we simulate a water-gas flow in the GDL of a PEM fuel cell and investigate the saturation-dependent transport properties under different conditions. The results are shown to be qualitatively consistent with the previous numerical and theoretical works. 相似文献
20.
一、从政府采购相关利益人心态分析当前治理商业贿赂的难点当前治理政府采购领域商业贿赂采取的主要工作方法是通过调查摸底、对照检查、处理整改和评估验收来进行,这种方式有效与否在很大程度上取决于相关利益人(主体)对此项工作的关注度和认识程度。然而.简单分析政府采购全过程中相关利益人的心态不难看出,单靠这种方法较难使商业贿赂的治理取得实质性效果。 相似文献