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11.
Template‐Free Fabrication of Mesoporous Alumina Nanospheres Using Post‐Synthesis Water‐Ethanol Treatment of Monodispersed Aluminium Glycerate Nanospheres for Molybdenum Adsorption 下载免费PDF全文
Indra Saptiama Yusuf Valentino Kaneti Yoshitaka Suzuki Kunihiko Tsuchiya Nobuyoshi Fukumitsu Takeji Sakae Jeonghun Kim Yong‐Mook Kang Katsuhiko Ariga Yusuke Yamauchi 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(21)
This work reports the template‐free fabrication of mesoporous Al2O3 nanospheres with greatly enhanced textural characteristics through a newly developed post‐synthesis “water‐ethanol” treatment of aluminium glycerate nanospheres followed by high temperature calcination. The proposed “water‐ethanol” treatment is highly advantageous as the resulting mesoporous Al2O3 nanospheres exhibit 2–4 times higher surface area (up to 251 m2 g?1), narrower pore size distribution, and significantly lower crystallization temperature than those obtained without any post‐synthesis treatment. To demonstrate the generality of the proposed strategy, a nearly identical post‐synthesis “water treatment” method is successfully used to prepare mesoporous monometallic (e.g., manganese oxide (MnO2)) and bimetallic oxide (e.g., CuCo2O4 and MnCo2O4) nanospheres assembled of nanosheets or nanoplates with highly enhanced textural characteristics from the corresponding monometallic and bimetallic glycerate nanospheres, respectively. When evaluated as molybdenum (Mo) adsorbents for potential use in molybdenum‐99/technetium‐99m (99Mo/99mTc) generators, the treated mesoporous Al2O3 nanospheres display higher molybdenum adsorption performance than non‐treated Al2O3 nanospheres and commercial Al2O3, thereby suggesting the effectiveness of the proposed strategy for improving the functional performance of oxide materials. It is expected that the proposed method can be utilized to prepare other mesoporous metal oxides with enhanced textural characteristics and functional performance. 相似文献
12.
Since the control methods of a transport system between processing machines are specialized for each layout of the system,
it is difficult to design prompt schedules and control logic for new complicated systems, especially in cases of machine faults
or restructuring the system to modify the layout. In this article, we describe a multiagent transport control system which
utilizes pheromone information. Each element of the system acts as an agent and estimates the appropriate path and time to
drive out the products using information obtained by communication with other elements as well as pheromone information deposited
on the tracks of the products. 相似文献
13.
Yoshitaka Sawa Kenji Yamashita Takeshi Kitadani Daiji Noda Tadashi Hattori 《Microsystem Technologies》2010,16(8-9):1369-1375
The nickel electroforming method using a high-concentration nickel sulfamate bath is commonly used to fabricate micro metal molds in the LIGA process; however, this method does not produce micro metal molds of sufficient hardness. One means of improving the hardness of micro metal molds made using the nickel electroforming method is to include additives in the nickel plating solution. Another method is nickel alloy plating or a similar technique. In this research, we used a nickel–boron (Ni–B) electroless alloy plating method to obtain a hard nickel plated film having hardness of 832 Hv. It was also ascertained that Ni–B electroless alloy plated film retains its high hardness even during heat treatment in conditions of 250°C for 1 h. To deal with the high stresses developed in high-hardness plated films, we proposed double-layer nickel electroforming. This method is covered and used on conventional nickel electroforming layer by high hardness micro mold. High hardness micro metal mold using double-layer was fabricated by nickel electroforming and Ni–B electroless alloy plating method. 相似文献
14.
Hossein Tehrani Nik Nejad Nobuhiro Sugimura Koji Iwamura Yoshitaka Tanimizu 《Journal of Intelligent Manufacturing》2010,21(4):487-499
Due to rapid changes of markets and pressures of competitions, industries are adopting their production ways to support diversity
of customer’s needs and increase of new product developments. This paper deals with development of an agent-based architecture
of dynamic systems for process planning in the manufacturing systems. In consideration of alternative manufacturing processes
and machine tools, the process plans and the schedules of the manufacturing resources are generated incrementally and dynamically.
A previously proposed negotiation protocol is customized and improved to generate suitable process plans for the target products
real-timely and dynamically, based on the alternative manufacturing processes. The alternative manufacturing processes are
presented by the process plan networks and the suitable process plans are searched and generated to cope with both the dynamic
status and disturbances of the manufacturing systems. We initiatively combine the heuristic search algorithms of the process
plan networks with the negotiation protocols, in order to generate suitable process plans. 相似文献
15.
Implementation of a decision support system using an interactive large-scale high-resolution display
Tomoyuki Ishida Yusuke Hirohara Nobuyuki Kukimoto Yoshitaka Shibata 《Artificial Life and Robotics》2017,22(3):385-390
In this research, we propose and evaluate a decision support system using an interactive large-scale high-resolution display. This decision support system supports the summarization and decision-making of a large amount of disaster information during the occurrence of a large-scale natural disaster. Municipal employees at the disaster control headquarters can display disaster information on the large-scale display with a touch or flick on a laptop or tablet. To evaluate the operability, readability, functionality, and necessity of the decision support system, we surveyed 23 municipal employees in the disaster prevention division using a questionnaire. The system received a great evaluation in all the evaluation items. 相似文献
16.
Quick-freeze deep-etch replica electron microscopy gives high contrast snapshots of individual protein molecules under physiological conditions in vitro or in situ. The images show delicate internal pattern, possibly reflecting the rotary-shadowed surface profile of the molecule. As a step to build the new system for the "Structural analysis of single molecules", we propose a procedure to quantitatively characterize the structural property of individual molecules; e.g. conformational type and precise view-angle of the molecules, if the crystallographic structure of the target molecule is available. This paper presents a framework to determine the observed face of the protein molecule by analyzing the surface profile of individual molecules visualized in freeze-replica specimens. A comprehensive set of rotary-shadowed views of the protein molecule was artificially generated from the available atomic coordinates using light-rendering software. Exploiting new mathematical morphology-based image filter, characteristic features were extracted from each image and stored as template. Similar features were extracted from the true replica image and the most likely projection angle and the conformation of the observed particle were determined by quantitative comparison with a set of archived images. The performance and the robustness of the procedure were examined with myosin head structure in defined configuration for actual application. 相似文献
17.
Yukimitsu Okano Tamio Kohriyama Yoshitaka Yoshida Michio Murase 《Nuclear Engineering and Design》2003,223(2):145-158
For severe accident assessment in a light water reactor, heat transfer models in a narrow annular gap between the overheated core debris and the reactor pressure vessel (RPV) are important for evaluating RPV integrity and emergency procedures. Using existing data, the authors developed heat transfer models on the average critical heat flux (CHF) restricted by countercurrent flow limitation (CCFL) and local boiling heat fluxes, and showed that the average CHF depended on the steam–water flow pattern in the narrow gap and that the local heat fluxes were similar to the pool boiling curve. We evaluated the validity of heat transfer models by simple calculations for ALPHA experiments performed at Japan Atomic Energy Research Institute. Calculated results showed that heat fluxes on the crust surface were restricted mainly by thermal resistance of the crust after the crust formation, and emissivity on the crust surface did not have much effect on the heat fluxes. The calculated vessel temperature during the heat-up process and peak vessel temperature agreed well with the measurements, which confirmed the validity of the average CHF correlation. However, the vessel cooling rate was underestimated mainly due to underestimation of the gap size. 相似文献
18.
Yoshitaka Shingaya Tomonobu Nakayama Masakazu Aono 《Science and Technology of Advanced Materials》2004,5(5-6):647
Nanorods of substoichiometric tungsten oxide (WOx) were grown on W(001) substrates. Two methods for the growth of nanorods were used: oxidation of the substrate under appropriate conditions and the deposition of tungsten oxide from a tungsten foil heated in the presence of oxygen. The grown nanorods were observed using a scanning electron microscope and an atomic force microscope. The diameters of the nanorods were 5–20 nm. The nanorods were slightly inclined from the directions parallel or normal to the surface. The inclination of nanorods was explained in terms of the epitaxial relationship between WO3 crystals and the W(001) substrate. The WO3 crystals formed at the initial stage of growth act as the nuclei of WOx nanorods. We observed selective enhancement of the growth in a certain epitaxial direction depending on the method of growth, and an array of WOx nanorods was produced on the W(001) substrate. 相似文献
19.
One-step route to a hybrid TiO2/TixW1?xN nanocomposite by in situ selective carbothermal nitridation
Zo? Schnepp Martin J Hollamby Masahiko Tanaka Yoshitaka Matsushita Yoshio Katsuya Yoshio Sakka 《Science and Technology of Advanced Materials》2012,13(3)
Metal oxide/nitride nanocomposites have many existing and potential applications, e.g. in energy conversion or ammonia synthesis. Here, a hybrid oxide/nitride nanocomposite (anatase/TixW1−xN) was synthesized by an ammonia-free sol–gel route. Synchrotron x-ray diffraction, complemented with electron microscopy and thermogravimetric analysis, was used to study the structure, composition and mechanism of formation of the nanocomposite. The nanocomposite contained nanoparticles (<5 nm diameter) of two highly intermixed phases. This was found to arise from controlled nucleation and growth of a single oxide intermediate from the gel precursor, followed by phase separation and in situ selective carbothermal nitridation. Depending on the preparation conditions, the composition varied from anatase/TixW1−xN at low W content to an isostructural mixture of Ti-rich and W-rich TixW1−xN at high W content. In situ selective carbothermal nitridation offers a facile route to the synthesis of nitride-oxide nanocomposites. This conceptually new approach is a significant advance from previous methods, which generally require ammonolysis of a pre-synthesized oxide. 相似文献
20.
Sango Matsuzaki Kimitoshi Yamazaki Yoshitaka Hara Takashi Tsubouchi 《Journal of Intelligent and Robotic Systems》2018,92(3-4):453-463
This paper describes a novel method to estimate appropriate traversable regions from an outdoor scene image. The traversable regions output by the proposed method reflect the common sense of people. For example, a candidate traversable region is “a paved road somewhat distant from the side ditch.” The input to the traversable region estimation is one color image. First, category is assigned to each pixel in the image. The categorization result is then input to the region estimator. Finally, the traversable region are estimated on the input image. An important aspect of this method is the application of two score functions in region estimation process. One score function places high value on categories selected as traversable paths by subjects. The other function places high value on categories that are not selected as traversable regions but are adjacent to categories with traversable paths. A combination of these two functions produces feasible estimation results. The effectiveness of the combined score functions was evaluated by experiments and a questionnaire. 相似文献