全文获取类型
收费全文 | 1735篇 |
免费 | 86篇 |
国内免费 | 3篇 |
专业分类
电工技术 | 71篇 |
综合类 | 1篇 |
化学工业 | 499篇 |
金属工艺 | 37篇 |
机械仪表 | 49篇 |
建筑科学 | 19篇 |
矿业工程 | 1篇 |
能源动力 | 71篇 |
轻工业 | 175篇 |
水利工程 | 3篇 |
石油天然气 | 1篇 |
无线电 | 104篇 |
一般工业技术 | 302篇 |
冶金工业 | 294篇 |
原子能技术 | 59篇 |
自动化技术 | 138篇 |
出版年
2023年 | 27篇 |
2022年 | 55篇 |
2021年 | 82篇 |
2020年 | 43篇 |
2019年 | 44篇 |
2018年 | 61篇 |
2017年 | 51篇 |
2016年 | 63篇 |
2015年 | 54篇 |
2014年 | 45篇 |
2013年 | 110篇 |
2012年 | 85篇 |
2011年 | 106篇 |
2010年 | 69篇 |
2009年 | 66篇 |
2008年 | 78篇 |
2007年 | 63篇 |
2006年 | 48篇 |
2005年 | 42篇 |
2004年 | 32篇 |
2003年 | 34篇 |
2002年 | 23篇 |
2001年 | 28篇 |
2000年 | 31篇 |
1999年 | 33篇 |
1998年 | 102篇 |
1997年 | 67篇 |
1996年 | 57篇 |
1995年 | 20篇 |
1994年 | 26篇 |
1993年 | 30篇 |
1992年 | 10篇 |
1991年 | 9篇 |
1990年 | 14篇 |
1989年 | 11篇 |
1988年 | 8篇 |
1987年 | 8篇 |
1986年 | 7篇 |
1985年 | 4篇 |
1984年 | 5篇 |
1983年 | 8篇 |
1982年 | 7篇 |
1981年 | 11篇 |
1980年 | 6篇 |
1979年 | 3篇 |
1977年 | 3篇 |
1976年 | 12篇 |
1975年 | 8篇 |
1974年 | 3篇 |
1971年 | 2篇 |
排序方式: 共有1824条查询结果,搜索用时 31 毫秒
81.
Yuki Tanaka Takumi Sako Tatsuhiro Hiraoka Misaki Yamaguchi Masayuki Yamaguchi 《应用聚合物科学杂志》2020,137(46):49516
The structure and rheological properties of binary blends of polycarbonate (PC) and polystyrene (PS) were investigated using various PS samples with different molecular weights, namely PS1k (Mw = 1,000), PS53k (Mw = 53,000), and PS240k (Mw = 240,000). The blends with PS53k and PS240k show phase-separated structures, whereas the blend with PS1k is miscible. The shear viscosity decreases greatly on addition of PS53k and PS240k, especially at high shear rates, which would be a great advantage at processing operations. Because the nonlinear response occurs in the small strain region for multilayered films of PC and PS240k, the origin of the significant viscosity drop for the phase-separated system is interfacial slippage at the phase boundary. 相似文献
82.
Dr. Ivan A. Yaremenko Dr. Paolo Coghi Parichat Prommana Congling Qiu Peter S. Radulov Yuanqing Qu Yulia Yu. Belyakova Dr. Enrico Zanforlin Dr. Vladimir A. Kokorekin Yuki Yu Jun Wu Prof. Fabrice Fleury Dr. Chairat Uthaipibull Dr. Vincent Kam Wai Wong Prof. Alexander O. Terent'ev 《ChemMedChem》2020,15(13):1118-1127
This article discloses a new horizon for the application of peroxides in medical chemistry. Stable cyclic peroxides are demonstrated to have cytotoxic activity against cancer cells; in addition a mechanism of cytotoxic action is proposed. Synthetic bridged 1,2,4,5-tetraoxanes and ozonides were effective against HepG2 cancer cells and some ozonides selectively targeted liver cancer cells (the selectivity indexes for compounds 11 b and 12 a are 8 and 5, respectively). In some cases, tetraoxanes and ozonides were more selective than paclitaxel, artemisinin, and artesunic acid. Annexin V flow-cytometry analysis revealed that the active ozonides 22 a and 23 a induced cell death of HepG2 by apoptosis. Further study showed that compounds 22 a and 23 a exhibited a strong inhibitory effect on P-glycoprotein (P-gp/ABCB5)-overexpressing HepG2 cancer cells. ABCB5 is a key player in the multidrug-resistant phenotype of liver cancer. Peroxides failed to demonstrate a direct correlation between oxidative potential and their biological activity. To our knowledge this is the first time that peroxide diastereoisomers have been found to show stereospecific antimalarial action against the chloroquine-sensitive 3D7 strain of Plasmodium falciparum. Stereoisomeric ozonide 12 b is 11 times more active than stereoisomeric ozonide 12 a (IC50=5.81 vs 65.18 μm ). Current findings mean that ozonides merit further investigation as potential therapeutic agents for drug-resistant hepatocellular carcinoma. 相似文献
83.
本文摘录介绍了近年来日本在节能环保领域内,从国家的政策引导到地方政府和民间企业的积极参与建设新型智能社区的情况.并具体说明了一些关键应用,如新能源利用,能源管理系统,智能电网,EV电动车和新型交通系统在智能社区里的应用实例及日本在此领域内的标准化推进方面的情况. 相似文献
84.
Enhanced Light Storage of SrAl2O4 Glass‐Ceramics Controlled by Selective Europium Reduction
下载免费PDF全文
![点击此处可从《Journal of the American Ceramic Society》网站下载免费的PDF全文](/ch/ext_images/free.gif)
Takayuki Nakanishi Kazune Watanabe Jumpei Ueda Koji Fushimi Setsuhisa Tanabe Yasuchika Hasegawa 《Journal of the American Ceramic Society》2015,98(2):423-429
A luminescent Eu, Dy: SrAl2O4 glass‐ceramics with high transparency in the visible region was successfully synthesized using the frozen sorbet technique with the control of O2 partial pressure () for the oxidation of Eu2+ ions. The glass‐ceramics include Eu2+, Eu3+, and Dy3+ ions, and thus exhibits three characteristic types of emission bands, 4f–5d at around 520 nm (Eu2+ ions), 4f–4f at 610 nm (Eu3+ ions), and 480 nm (Dy3+ ions). The Eu, Dy: SrAl2O4 glass‐ceramics provide remarkable long‐persistent luminescence under dark condition. The glass‐ceramics also exhibits color‐changing luminescence in the visible region based on their remarkable light storage properties. The luminescent Eu, Dy: SrAl2O4 glass‐ceramics using the frozen sorbet technique with control of are promising materials for application in novel photonic and light storage materials. 相似文献
85.
Feng B Morita M Imanaka H Imamura K Nakanishi K 《Journal of Bioscience and Bioengineering》2006,102(5):470-473
We identified 22 genes from Aspergillus oryzae that are preferentially expressed in membrane-surface liquid culture (MSLC), among which Ser/Thr protein kinase (aopk1) and phosphatase (aoppt) genes were cloned. We also revealed that aopk1 encodes a protein with an N-terminal sequence 150 amino acid residues longer than that predicted from the registered sequence in GenBank. 相似文献
86.
Murakami M Imamura E Shinohara H Kiri K Muramatsu Y Harada A Takada H 《Environmental science & technology》2008,42(17):6566-6572
We analyzed perfluorinated surfactants (PFSs) in 20 river samples and 5 wastewater secondary effluent samples in Japan to reveal their occurrence and sources. Nine PFS species were determined: perfluorooctanesulfonate (PFOS), perfluorooctane sulfonamide (FOSA), perfluoroheptanoate (PFHpA), perfluorooctanoate (PFOA), perfluorononanoate (PFNA), perfluorodecanoate (PFDA), perfluoroundecanoate (PFUA), perfluorododecanoate (PFDDA), and perfluorotridecanoate (PFTDA). PFSs were detected in all rivers, revealing nationwide contamination of rivers. In particular, 11 out of 20 river samples exceeded New Jersey guidance for PFOA in drinking water (40 ng/L). PFOS, PFHpA, PFOA, and PFNA were major species in Japan. Concentrations of PFOS, PFHpA, and PFNA in rivers were strongly correlated with population density, suggesting that the chemicals were derived from urban activities. PFOA showed a significant but weak correlation. We used crotamiton, a marker of sewage effluent, for further source analysis. Concentrations of PFOS, PFHpA, and PFNAwere strongly correlated with those of crotamiton, and plots of secondary effluents fell near the regression lines of rivers, indicating that the PFOS, PFHpA, and PFNA in rivers were derived from sewage effluent. On the other hand, PFOA was found at remarkably high levels (54-192 ng/L) in seven river samples containing low levels of crotamiton, suggesting that it was derived from nonsewage point sources, as well as sewage effluent. The total fluxes of sewage-derived PFOS, PFHpA, PFOA, and PFNA from Japan were estimated to be 3.6, 2.6, 5.6, and 2.6 t/year, respectively. This is the first report to identify PFOA in several rivers, derived from nonsewage point sources, by using a marker of sewage effluent. 相似文献
87.
Atsushi Nakanishi Takashi Yasuda Kazuki Horita Hironori Takahashi 《Journal of Infrared, Millimeter and Terahertz Waves》2018,39(1):36-44
We measured the thermal dependencies of the refractive index and the absorption coefficient of high-resistivity silicon. We found that the refractive index varied slightly with temperature, and the absorption coefficient was very low and remained approximately constant as the temperature was changed. As a result, the conditions for terahertz propagation in silicon could be controlled by changing the refractive index without any absorption loss. As one application of this effect, we developed a terahertz time delay generator that can generate a terahertz time delay by changing the temperature of the medium through which the terahertz beam passes, without the need for any mechanical delay. We demonstrated generation of a terahertz time delay of approximately 6.6 ps. 相似文献
88.
89.
Shoya Ueno Yuki Nakamura Ken-Ichi Sugioka Masaki Kubo Takao Tsukada Masahito Uchikoshi Hiroyuki Fukuyama 《International Journal of Thermophysics》2017,38(2):16
The normal spectral emissivity of molten Cu–Co alloy with different compositions was measured in the wavelength range of 780 nm to 920 nm and in the temperature range of 1430 K to 1770 K including the undercooled condition by an electromagnetic levitator superimposed with a static magnetic field. The emissivity was determined as the ratio of the radiance from a levitated molten Cu–Co droplet measured by a spectrometer to the radiance from a blackbody calculated by Planck’s law at a given temperature, where a static magnetic field of 2.5 T to 4.5 T was applied to the levitated droplet to suppress the surface oscillation and translational motion of the sample. We found little temperature dependence of the normal spectral emissivity of molten Cu–Co alloy. Concerning the composition dependence, the emissivity decreased markedly above 80 at%Cu and reached that of pure Cu, although its dependence was low between 20 at%Cu and 80 at%Cu. In addition, this composition dependence of the emissivity of molten Cu–Co alloy can be explained well by the Drude free-electron model. 相似文献
90.