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31.
Ren  Wuyang  Li  Handong  Gao  Lei  Li  Yong  Zhang  Zhongyang  Long  Chengjia  Ji  Haining  Niu  Xiaobin  Lin  Yuan  Wang  Zhiming 《Nano Research》2017,10(1):247-254
Nano Research - Thermal transport in superlattices is governed by various phonon-scattering processes. For extracting the phonon-scattering contribution of hetero-interfaces in chalcogenide...  相似文献   
32.
Owing to the strong affinity of thiols to Au and Ag, they are often employed to modify the surfaces of nanoparticles (NPs). Recently, these strong ligand-interface interactions have been employed to control NP growth, and this technique has emerged as a unique modulation strategy for creating unconventional plasmonic hybrid nanostructures. In these systems, the roles of the non-mercapto components of the thiol molecules and their structures are still unknown. Therefore, we herein present our investigation into this phenomenon. Primary amino (–NH2) groups in thiols are found to play a key role in regulating growth kinetics, i.e., in accelerating Ag deposition on Au NPs. The–NH2 groups are thought to bring Ag ions to the particle surface by coordinating to them, and thereby assist their reduction. The effect of molecular structure is non-trivial and thus provides the possibility of selective thiol detection. Based on the dependence of kinetic modulation on the non-mercapto components and molecular structures of molecules, we demonstrate the highly sensitive and specific detection of cysteine (limit of detection: 6 nM) in a mixture of 19 natural amino acids based on Ag growth on Au nanospheres. In addition, based on this modulation effect, we reveal the entrapping of chiral thiols within the growth layer through their plasmonic circular dichroism (PCD) responses. We believe that thiol-based growth regulation has great potential for creating plasmonic nanostructures with novel functionalities.
  相似文献   
33.
In this paper, we shall establish sufficient conditions for the existence of mild solutions for nonlocal impulsive differential inclusions. On the basis of the fixed point theorems for multivalued maps and the technique of approximate solutions, new results are obtained. Examples are also provided to illustrate our results.  相似文献   
34.
35.
International Journal of Control, Automation and Systems - This brief paper studies the stationary consensus of multiple Euler-Lagrange systems with nonlinear protocols. Two consensus protocols are...  相似文献   
36.
We compare the fixed parameter complexity of various variants of coloring problems (including List Coloring, Precoloring Extension, Equitable Coloring, L(p,1)-Labeling and Channel Assignment) when parameterized by treewidth and by vertex cover number. In most (but not all) cases we conclude that parametrization by the vertex cover number provides a significant drop in the complexity of the problems.  相似文献   
37.
大纯滞后过程的采样控制及其工程实现中的若干问题   总被引:1,自引:0,他引:1  
提出了采样控制机制的新观点,介绍控制器参数确定的新方法,分析了采样控制的质量,指出了在工程实施应考虑的若干问题。  相似文献   
38.
田吉  秦文明 《控制工程》2001,8(3):58-59
以实际应用的小型集散变频调速系统为例 ,介绍一种PC机与多AT89C2 0 51单片机之间串行通信的接口电路 ,并提出一种新的通信方法 ,即采用QBASIC语言提供通信语句来编写多机通信程序。该方法硬件紧凑 ,软件编程简单可靠。  相似文献   
39.
The fundamental issues of capability of robust and adaptive control in dealing with uncertainty are investigated in stochastic systems. It is revealed that to capture the intrinsic limitations of adaptive control, it is necessary to use supt types of transient and persistent performance, rather than lim supt types which reflect only asymptotic behavior of a system. For clarity and technical tractability, a simple first-order linear time-varying system is employed as a vehicle to explore performance lower bounds of robust and adaptive control. Optimal performances of nominal, robust and adaptive control are explicitly derived and their implications are discussed in an information framework. An adaptive strategy is scrutinized for its achievable performance bounds. The results indicate that intimate interaction and inherent conflict between identification and control result in a certain performance lower bound which does not approach the nominal performance even when the system varies very slowly. Explicit lower bounds are obtained when disturbances are either normally or uniformly distributed  相似文献   
40.
Recently, one-dimensional nanostructures have attracted extensive attention since they are potentially important for both applications and fundamental research. In this paper, we report the synthesis of ultra-long single crystal Si3N4 nanobelts via catalyst-assisted pyrolysis of polymeric precursors. The obtained products contain both α- and β-Si3N4 nanobelts, which are 50–100 nm in thickness, 400–1000 nm in width, and a few hundreds of micrometers to several millimeters in length. Different from previous techniques for synthesizing one-dimensional structures, the current nanobelts are synthesized through confined crystallization of an amorphous phase. A solid–liquid–gas–solid reaction/crystallization growth mechanism is proposed. The formation of nanobelts instead of nanowires is attributed to the anisotropy growth at an earlier stage.  相似文献   
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