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81.
Hexabromocyclododecane: current understanding of chemistry, environmental fate and toxicology and implications for global management 总被引:2,自引:0,他引:2
Marvin CH Tomy GT Armitage JM Arnot JA McCarty L Covaci A Palace V 《Environmental science & technology》2011,45(20):8613-8623
Hexabromocyclododecane (HBCD) is a globally produced brominated flame retardant (BFR) used primarily as an additive FR in polystyrene and textile products and has been the subject of intensified research, monitoring and regulatory interest over the past decade. HBCD is currently being evaluated under the Stockholm Convention on Persistent Organic Pollutants. HBCD is hydrophobic (i.e., has low water solubility) and thus partitions to organic phases in the aquatic environment (e.g., lipids, suspended solids). It is ubiquitous in the global environment with monitoring data generally exhibiting the expected relationship between proximity to known sources and levels; however, temporal trends are not consistent. Estimated degradation half-lives, together with data in abiotic compartments and long-range transport potential indicate HBCD may be sufficiently persistent and distributed to be of global concern. The detection of HBCD in biota in the Arctic and in source regions and available bioaccumulation data also support the case for regulatory scrutiny. Toxicity testing has detected reproductive, developmental and behavioral effects in animals where exposures are sufficient. Recent toxicological advances include a better mechanistic understanding of how HBCD can interfere with the hypothalamic-pituitary-thyroid axis, affect normal development, and impact the central nervous system; however, levels in biota in remote locations are below known effects thresholds. For many regulatory criteria, there are substantial uncertainties that reduce confidence in evaluations and thereby confound management decision-making based on currently available information. 相似文献
82.
Adrian R. Brough Christopher M. Dobson Ian G. Richardson Geoffrey W. Groves 《Journal of the American Ceramic Society》1994,77(2):593-596
Selective isotopic enrichment of SiO2 with 29 Si in a mixture with tricalcium silicate (C3 S) has allowed the Si from this phase to be effectively labeled during the course of the hydration reaction, thus isolating its contribution to the reaction. A double Q2 signal has been observed in 29 SI solid-state MAS NMR spectroscopy of C-S-H gels of relatively low Ca/Si ratio, prepared by hydration or by carbonation of a C3 S paste. The origin of the weaker, downfield peak is discussed and tentatively attributed to bridging tetrahedra of a dreierkette silicate chain structure. 相似文献
83.
López Steven R.; Lara Ma. del Carmen; Kopelowicz Alex; Solano Susana; Foncerrada Hector; Aguilera Adrian 《Canadian Metallurgical Quarterly》2009,77(4):763
The authors developed and tested a 35-min psychoeducational program with the goal of increasing Spanish-speaking persons’ literacy of psychosis. The program uses popular cultural icons derived from music, art, and videos, as well as a mnemonic device—La CLAve (The Clue)—to increase (a) knowledge of psychosis, (b) efficacy beliefs that one can identify psychosis in others, (c) attributions to mental illness, and (d) professional help-seeking. Assessments were conducted before and after administering the program to both community residents (n = 57) and family caregivers of persons with schizophrenia (n = 38). For community residents, the authors observed increases across the 4 domains of symptom knowledge, efficacy beliefs, illness attributions, and recommended help-seeking. For caregivers, increases were observed in symptom knowledge and efficacy beliefs. La CLAve is a conceptually informed psychoeducational tool with a developing empirical base aimed at helping Spanish-speaking Latinos with serious mental illness obtain care in a timely manner. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
84.
Adrian Postelnicu 《International Journal of Heat and Mass Transfer》2009,52(11-12):2466-2470
The onset of convection in a horizontal layer filled with a fluid-saturated porous medium is studied in this paper. On the lower wall there is an exothermic surface reaction, described by the Arrhenius kinetics, while the upper wall is subjected to uniform temperature and concentration. The problem, cast in dimensionless form, is governed by three dimensionless parameters pertaining to the exothermic reaction and the Lewis number. Once the basic state is solved, a linearized stability analysis is then performed and the resulting eigenvalue problem is solved using a conventional shooting method. One determines numerically the critical Rayleigh and wave numbers at the onset of convection, for various values of the problem parameters. 相似文献
85.
A new analytical method has been developed for the quantification of polybrominated diphenyl ethers (PBDEs) in human adipose tissue samples. After Soxhlet extraction and a cleanup procedure using two successive solid-phase extraction cartridges containing acid silica and acid silica: neutral silica:deactivated basic alumina (from top to bottom), detection can been achieved by narrow-bore (0.10-mm i.d.) capillary gas chromatography/electron impact low-resolution mass spectrometry using a large-volume injection technique. Using narrow-bore capillaries, it is possible to analyze complex mixtures in a short time (up to 10 min), saving 50% or more of the analysis time of conventional columns while maintaining a similar resolution power. The method allows the determination of five major PBDE congeners (BDE 28, 47, 99, 100, and 153) at concentrations below 1 ng/g lipid weight. Detection limits in the selected ion mode varied between 0.05 and 0.30 ng/g lipid weight, depending on the degree of bromination. The sensitivity of this method can compete with low-resolution mass spectrometry with electron capture ionization, while a much better selectivity is obtained. Levels of PBDEs in 20 Belgian human adipose tissue samples ranged between 2.18 and 11.70 ng/g lipid weight and were similar to previously reported values from Europe. 相似文献
86.
Reduction Incorporated (RI) recognisers and parsers deliver high performance by suppressing the stack activity except for those rules that generate fully embedded recursion. Automaton constructions for RI parsing have been presented by Aycock and Horspool [John Aycock and Nigel Horspool. Faster generalised LR parsing. In Compiler Construction, 8th Intnl. Conf, CC'99, volume 1575 of Lecture Notes in Computer Science, pages 32 – 46. Springer-Verlag, 1999] and by Scott and Johnstone [Adrian Johnstone and Elizabeth Scott. Generalised regular parsers. In Gorel Hedin, editor, Compiler Construction, 12th Intnl. Conf, CC'03, volume 2622 of Lecture Notes in Computer Science, pages 232–246. Springer-Verlag, Berlin, 2003] but both can yield very large tables. An unusual aspect of the RI automaton is that the degree of stack activity suppression can be varied in a fine-grained way, and this provides a large family of potential RI automata for real programming languages, some of which have manageable table size but still show high performance. We give examples drawn from ANSI-C, Cobol and Pascal; discuss some heuristics for guiding manual specification of stack activity suppression; and describe work in progress on the automatic construction of RI automata using profiling information gathered from running parsers: in this way we propose to optimise our parsers' table size against performance on actual parsing tasks. 相似文献
87.
Forward directivity effects in the near-fault region produce pulse-type motions that differ significantly from ordinary ground motions that occur at greater distances from the causative fault. Current code site factors are based on empirical observations and analyses involving less intense nonpulse ordinary ground motions. Nonlinear site response analyses with bidirectional shaking are performed using representative site profiles to quantify seismic site response effects for intense near-fault motions resulting from forward directivity. Input rock motions are represented with simplified velocity pulses that characterize the amplitude and period of forward directivity motions. Results indicate that site response affects both the amplitude and period of forward directivity pulses, and hence, local site conditions should be considered when evaluating seismic designs in the near-fault region. Stiff soil sites tend to amplify the peak ground velocity and increase the period of pulse-type motions, particularly, when the period of the rock motion coincides with the degraded period of the site. Amplification is limited at soft soil sites by the dynamic strength of the weak soil, so attenuation occurs for intense input motions. This nonlinearity is not reflected in the site factors in current building codes. Guidance is provided for estimating the amplitude and pulse period for velocity pulses at soil sites. 相似文献
88.
Adrian David Cheok Xubo Yang Zhou Zhi Ying Mark Billinghurst Hirokazu Kato 《Personal and Ubiquitous Computing》2002,6(5-6):430-442
This paper presents a novel computer entertainment system which recaptures human touch and physical interaction with the
real-world environment as essential elements of the game play, whilst also maintaining the exciting fantasy features of traditional
computer entertainment. Our system called ‘Touch-Space’ is an embodied (ubiquitous, tangible, and social) computing based
Mixed Reality (MR) game space which regains the physical and social aspects of traditional game play. In this novel game space,
the real-world environment is an essential and intrinsic game element, and the human’s physical context influences the game
play. It also provides the full spectrum of game interaction experience ranging from the real physical environment (human
to human and human to physical world interaction), to augmented reality, to the virtual environment. It allows tangible interactions
between players and virtual objects, and collaborations between players in different levels of reality. Thus, the system re-invigorates
computer entertainment systems with social human-to-human and human-to-physical touch interactions.
Correspondence to: Professor A. Cheok, National University of Singapore, 10 Kent Ridge Crescent, Singapore 119260. Email: adriancheok@nus.edu.sg 相似文献
89.
90.
A new mean-value type of algorithm is developed for analyzing multi-facility blocking models with state-dependent arrival rates. It can be applied to a broad class of blocking systems with simultaneous resource possession including, for example, circuit-switched networks. The underlying recursion is cast in terms of blocking probabilities and marginal state probabilities. The developments made here generalize previous results that were restricted to the case of constant arrival rates. 相似文献