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排序方式: 共有811条查询结果,搜索用时 31 毫秒
61.
Valentin Magn Florent Blanchard Angela Marinetti Arnaud Voituriez Xavier Guinchard 《Advanced Synthesis \u0026amp; Catalysis》2016,358(21):3355-3361
N‐Propargyl‐ and N‐homoallenyl‐2‐bromo‐β‐tryptamines undergo gold(I)‐catalyzed dearomatizing cyclizations to afford 2‐bromospiroindolenines that are in situ hydrolyzed to furnish spirooxindoles in a one‐pot process. Tryptophane derivatives (R2=CO2Et) led upon cyclization to chiral spirooxindoles in excellent diastereoselectivities.
62.
Bacterial-based additives for the production of artificial snow: What are the risks to human health?
Arnaud Lagriffoul Rafik Absi Jean-Marc Berjeaud Edmond E. Creppy Jean-Pierre Gadonna Cindy E. Morris 《The Science of the total environment》2010,408(7):1659-1666
For around two decades, artificial snow has been used by numerous winter sports resorts to ensure good snow cover at low altitude areas or more generally, to lengthen the skiing season. Biological additives derived from certain bacteria are regularly used to make artificial snow. However, the use of these additives has raised doubts concerning the potential impact on human health and the environment. In this context, the French health authorities have requested the French Agency for Environmental and Occupational Health Safety (Afsset) to assess the health risks resulting from the use of such additives. The health risk assessment was based on a review of the scientific literature, supplemented by professional consultations and expertise. Biological or chemical hazards from additives derived from the ice nucleation active bacterium Pseudomonas syringae were characterised. Potential health hazards to humans were considered in terms of infectious, toxic and allergenic capacities with respect to human populations liable to be exposed and the means of possible exposure. Taking into account these data, a qualitative risk assessment was carried out, according to four exposure scenarios, involving the different populations exposed, and the conditions and routes of exposure. It was concluded that certain health risks can exist for specific categories of professional workers (mainly snowmakers during additive mixing and dilution tank cleaning steps, with risks estimated to be negligible to low if workers comply with safety precautions). P. syringae does not present any pathogenic capacity to humans and that the level of its endotoxins found in artificial snow do not represent a danger beyond that of exposure to P. syringae endotoxins naturally present in snow. However, the risk of possible allergy in some particularly sensitive individuals cannot be excluded. Another important conclusion of this study concerns use of poor microbiological water quality to make artificial snow. 相似文献
63.
Coplanar waveguide (CPW) and thin film microstrip (TFMS) lines integrating porous ultra low-k as inter-metal dielectric layers (k = 2.5) and copper as metal, are for the first time experimentally measured up to 110 GHz and under different temperature conditions, up to 200 °C. The extracted attenuation and propagation coefficients of those transmission lines are compared to simulations performed with MAGWEL software, a frequency domain 3-D Maxwell solver. Based on the characterization results some guidelines related to interconnect design are presented for future applications. 相似文献
64.
ABSTRACT Vacuum drying, j,e drying under absolute gas pressure of about 10? Pa. is an efficient means of reducing the process period and of producing good quality wood. We will examine here continuous vacuum drying where the plank surfaces are kept at a constant temperature, which remains above the boiling point, and moisture flowing to the surface is extracted from the kiln. We have carried out an experimental study of oak drying under such conditions. The drying rate and moisture content profile of the sample (40 mm thick) are recorded during the whole drying period. A model of continuous drying is established from general conservation equations with the main approximation that the air is rapidly extracted. The two constitutive equations of the model which describe temperature and water content fields are of a diffusive type and coupled through coefficients. The adequate boundary equation is not a convective one, but expresses a hygroscopic equilibrium between the vapour in the chamber and the wood surface. The mass diffusive coefficient can be adjusted to the drying rates through capillary pressure and bound water diffusion functions. The wood heterogeneity (seasonal growth) is the main factor of discrepancy in these functions. The simulated drying rates correspond with the experimental ones. 相似文献
65.
N. Arnaud J.Y. Cognard P. Davies P.Y. Le Gac 《Journal of Adhesion Science and Technology》2013,27(21):2355-2380
The objective of the study is to identify the 3D behaviour of an adhesive in an assembly, and to take into account the effect of ageing in a marine environment. To that end, three different tests were employed. Gravimetric analyses were used to determine the water diffusion kinetics in the adhesive. Bulk tensile tests were performed to highlight the effects of humid ageing on the adhesive behaviour. Modified Arcan tests were performed for several ageing times to obtain the experimental database which was necessary to identify constitutive models. A Mahnken–Schlimmer type model was determined for the unaged state according to a procedure developed in a previous study. This identification used inverse techniques. It was based on the unaged modified Arcan results and on a coupling between an optimisation routine and finite-element analysis. Then, a global inverse identification procedure was developed. Its aim was to relate the unaged parameters to the moisture concentration and overcome the difficulties usually associated with ageing of bonded assemblies in a humid environment: a non-uniformity of the stress state and a gradient of mechanical properties in the adhesive. This procedure was similar to the one used in the first part but needed modified Arcan results for several ageing times. It also required an initial assumption for the evolution of the Mahnken–Schlimmer parameters with the moisture concentration. 相似文献
66.
Yannick Raoul des Essarts Mohamad Sabbah Arnaud Comte Laurent Soulère Yves Queneau Yves Dessaux Valérie Hélias Denis Faure 《International journal of molecular sciences》2013,14(10):19976-19986
Bacteria belonging to the Pectobacterium genus are the causative agents of the blackleg and soft-rot diseases that affect potato plants and tubers worldwide. In Pectobacterium, the expression of the virulence genes is controlled by quorum-sensing (QS) and N-acylhomoserine lactones (AHLs). In this work, we screened a chemical library of QS-inhibitors (QSIs) and AHL-analogs to find novel QSIs targeting the virulence of Pectobacterium. Four N,N′-bisalkylated imidazolium salts were identified as QSIs; they were active at the μM range. In potato tuber assays, two of them were able to decrease the severity of the symptoms provoked by P. atrosepticum. This work extends the range of the QSIs acting on the Pectobacterium-induced soft-rot disease. 相似文献
67.
68.
Arnaud Duchosal René Leroy Laurent Vecellio Christophe Louste N. Ranganathan 《The International Journal of Advanced Manufacturing Technology》2013,66(5-8):1003-1014
In this study, a method is developed to determine the oil mist characteristics for the minimal quantity lubricant process. The oil mist is characterized by the size, velocity, and volume flow rate of its particles. In each case, a specific measurement process is used: the laser diffraction granulometry method, the particle image velocimetry, and the gravimetric method. These methods are used in the case of static and simple models with different inner channels. Experimental tests have been done with the same inner channel as the existing spindle inner channel. Different output models with different inner canalizations have been tested, using these experimental processes. The main goal is to control the characteristics of output oil mist as a function of the input oil mist device parameters. 相似文献
69.
70.
Y Z Gunata C L Bayonove R E Cordonnier A Arnaud P Galzy 《Journal of the science of food and agriculture》1990,50(4):499-506
The exocellular β-glucosidases of Candida molischiana and Candida wickerhamii are able to hydrolyse geranyl, neryl, citronellyl, linalyl and α-terpinyl-β-D -glucopyranosides. The nature of the aglycone residue greatly affects the rate of hydrolysis. Glucosides with a tertiary alcohol as aglycone residue are more slowly hydrolysed than those with a primary alcohol. The β-glucosidase from C molischiana is also able to hydrolse α-L-arabinofuranosides. This results in the release of monoterpenols from a glycoside extract from grape juice. 相似文献