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91.
Abstract Under 24-GHz millimetre-wave irradiation heating ionic conductivity of zirconia base ceramics was up to 20 times higher than that of a conventionally-heated sample at the same temperature of 400 °C. The degree of enhancement could be altered by changing the stabilising atom from Y to Yb. Enhancement of ionic conduction was prominent in the setup condition of larger self-heating ratio and larger MMW absorbing materials. The isothermal improvement of ionic conductivity under MMW irradiation would be ascribed to the non-thermal effect. 相似文献
92.
Kenji Imai Koji Takai Tatsunori Hanai Makoto Shiraki Yusuke Suzuki Hideki Hayashi Takafumi Naiki Youichi Nishigaki Eiichi Tomita Masahito Shimizu Hisataka Moriwaki 《International journal of molecular sciences》2014,15(7):11294-11306
Obesity-related metabolic abnormalities, including adipokine imbalance and chronic inflammation, are involved in liver carcinogenesis. Chemerin, a novel adipokine, plays a critical role in adipogenesis, energy metabolism, and inflammation. We evaluated the impact of serum chemerin levels on liver functional reserves in hepatocellular carcinoma (HCC) patients and on the recurrence and prognosis of HCC. This study included 44 patients with any stage of HCC who underwent curative treatment at Gifu Municipal Hospital (Gifu, Japan) between 2006 and 2007. Recurrence-free survival and overall survival were estimated using the Kaplan-Meier method. Serum albumin levels (Pearson’s correlation coefficient; r = 0.3110, p = 0.0399), platelet counts (r = 0.4159, p = 0.0050), and prothrombin times (r = 0.3775, p = 0.0115) were significantly correlated with serum chemerin levels in patients with HCC, and they were inversely correlated with Child-Pugh scores (r = −0.3732, p = 0.0126), serum alanine aminotransferase levels (r = −0.3864, p = 0.0105), and total bilirubin levels (r = −0.4023, p = 0.0068). Among these variables, a multiple comparison test identified that platelet counts and total bilirubin levels were associated with serum chemerin levels (p < 0.0083). No significant correlation was found between serum chemerin levels and recurrence-free survival (p = 0.3691) or overall survival (p = 0.7916). In HCC patients, serum chemerin concentrations were correlated with liver functional reserves and platelet counts, but not with recurrence or prognosis. 相似文献
93.
Yoshihiro Hayashi Takuya Oishi Kaede Shirotori Yuki Marumo Atsushi Kosugi Shungo Kumada 《Drug development and industrial pharmacy》2018,44(7):1090-1098
Objectives: The aim of this study was to explore the potential of boosted tree (BT) to develop a correlation model between active pharmaceutical ingredient (API) characteristics and a tensile strength (TS) of tablets as critical quality attributes.Methods: First, we evaluated 81 kinds of API characteristics, such as particle size distribution, bulk density, tapped density, Hausner ratio, moisture content, elastic recovery, molecular weight, and partition coefficient. Next, we prepared tablets containing 50% API, 49% microcrystalline cellulose, and 1% magnesium stearate using direct compression at 6, 8, and 10?kN, and measured TS. Then, we applied BT to our dataset to develop a correlation model. Finally, the constructed BT model was validated using k-fold cross-validation.Results: Results showed that the BT model achieved high-performance statistics, whereas multiple regression analysis resulted in poor estimations. Sensitivity analysis of the BT model revealed that diameter of powder particles at the 10th percentile of the cumulative percentage size distribution was the most crucial factor for TS. In addition, the influences of moisture content, partition coefficients, and modal diameter were appreciably meaningful factors.Conclusions: This study demonstrates that BT model could provide comprehensive understanding of the latent structure underlying APIs and TS of tablets. 相似文献
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96.
Shunsuke Kato Prof. Akira Onoda Naomasa Taniguchi Prof. Ulrich Schwaneberg Prof. Takashi Hayashi 《Chembiochem : a European journal of chemical biology》2021,22(4):679-685
Directed evolution of Cp*RhIII-linked nitrobindin (NB), a biohybrid catalyst, was performed based on an in vitro screening approach. A key aspect of this effort was the establishment of a high-throughput screening (HTS) platform that involves an affinity purification step employing a starch-agarose resin for a maltose binding protein (MBP) tag. The HTS platform enables efficient preparation of the purified MBP-tagged biohybrid catalysts in a 96-well format and eliminates background influence of the host E. coli cells. Three rounds of directed evolution and screening of more than 4000 clones yielded a Cp*RhIII-linked NB(T98H/L100K/K127E) variant with a 4.9-fold enhanced activity for the cycloaddition of acetophenone oximes with alkynes. It is confirmed that this HTS platform for directed evolution provides an efficient strategy for generating highly active biohybrid catalysts incorporating a synthetic metal cofactor. 相似文献
97.
Yanhui Gu Zhenglu Yang Guandong Xu Miyuki Nakano Masashi Toyoda Masaru Kitsuregawa 《World Wide Web》2014,17(4):595-626
Measuring the semantic similarity between sentences is an essential issue for many applications, such as text summarization, Web page retrieval, question-answer model, image extraction, and so forth. A few studies have explored on this issue by several techniques, e.g., knowledge-based strategies, corpus-based strategies, hybrid strategies, etc. Most of these studies focus on how to improve the effectiveness of the problem. In this paper, we address the efficiency issue, i.e., for a given sentence collection, how to efficiently discover the top-k semantic similar sentences to a query. The previous methods cannot handle the big data efficiently, i.e., applying such strategies directly is time consuming because every candidate sentence needs to be tested. In this paper, we propose efficient strategies to tackle such problem based on a general framework. The basic idea is that for each similarity, we build a corresponding index in the preprocessing. Traversing these indices in the querying process can avoid to test many candidates, so as to improve the efficiency. Moreover, an optimal aggregation algorithm is introduced to assemble these similarities. Our framework is general enough that many similarity metrics can be incorporated, as will be discussed in the paper. We conduct extensive experimental evaluation on three real datasets to evaluate the efficiency of our proposal. In addition, we illustrate the trade-off between the effectiveness and efficiency. The experimental results demonstrate that the performance of our proposal outperforms the state-of-the-art techniques on efficiency while keeping the same high precision as them. 相似文献
98.
Samuel L. Manzello Seul-Hyun Park Sayaka SuzukiJohn R. Shields Yoshihiko Hayashi 《Fire Safety Journal》2011,46(8):568-578
Attempting to experimentally quantify the vulnerabilities of structures to ignition from firebrand showers has remained elusive. The coupling of two facilities has begun to unravel this difficult problem. The NIST Firebrand Generator (NIST Dragon) is an experimental device that can generate a firebrand shower in a safe and repeatable fashion. Since wind plays a critical role in the spread of WUI fires in the USA and urban fires in Japan, NIST has established collaboration with the Building Research Institute (BRI) in Japan. BRI maintains one of the only full scale wind tunnel facilities in the world designed specifically for fire experimentation; the Fire Research Wind Tunnel Facility (FRWTF). The present investigation is aimed at extensively quantifying firebrand penetration through building vents using full scale tests. A structure was placed inside the FRWTF and firebrand showers were directed at the structure using the NIST Dragon. The structure was fitted with a generic building vent, consisting of only a frame fitted with a metal mesh. Six different mesh sizes openings were used for testing. Behind the mesh, four different materials were placed to ascertain whether the firebrands that were able to penetrate the building mesh assembly could ignite these materials. Reduced scale test methods afford the capability to test new vent technologies and may serve as the basis for new standard testing methodologies. As a result, a new experimental facility developed at NIST is presented and is known as the NIST Dragon's LAIR (Lofting and Ignition Research). The NIST Dragon's LAIR has been developed to simulate a wind driven firebrand attack at reduced scale. The facility consists of a reduced scale Firebrand Generator (Baby Dragon) coupled to a bench scale wind tunnel. Finally, a series of full scale experiments were conducted to visualize the flow of firebrands around obstacles placed downstream of the NIST Dragon. Firebrands were observed to accumulate in front of these obstacles at a stagnation plane, as was observed when the structure was used for firebrand penetration through building vent experiments, due to flow recirculation. The accumulation of firebrands at a stagnation plane presents a severe threat to ignitable materials placed near structures. 相似文献
99.
Katsuki Hirabayashi Yoshiya Tashiro Nobuhiro Kondo Sachio Hayashi 《Journal of Applied Glycoscience》2017,64(2):33
We report production of the functional disaccharide gentiobiose β-D-Glcp-(1→6)-D-Glc by a hydrolysis reaction of hydrothermally treated Aureobasidium pullulans β-1,3-1,6-glucan as the substrate and Kitalase as the enzyme. Gentiobiose was produced over the pH range 4−6 and the concentration of gentiobiose produced decreased above pH 7. The maximum value of gentiobiose production was unaffected by the enzyme concentration. The maximum concentration of gentiobiose produced was dependent on the substrate concentration whereas the maximum ratio of gentiobiose to glucose was not. The production of gentiobiose from yeast β-1,3-1,6-glucan was lower than that from A. pullulans β-1,3-1,6-glucan. 相似文献
100.
Masahiko Hayashi Kazuya Yoshimoto Naohito Hirata Kiyoshi Tanaka Nobuki Oguni Katsumasa Harada Akio Matsushita Yasuhiro Kawachi Hiroshi Sasaki 《Israel journal of chemistry》2001,41(4):241-246
Highly enantioselective addition of diketene to aldehydes was achieved by using novel Schiff base—titanium alkoxide complexes. Up to 92% ee of 5-hydroxy-3-oxoesters was obtained. This procedure provides an efficient method for the asymmetric synthesis of potential inhibitors of HMG coenzyme reductase. 相似文献