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排序方式: 共有1627条查询结果,搜索用时 15 毫秒
21.
Allemann C Gordillo R Clemente FR Cheong PH Houk KN 《Accounts of chemical research》2004,37(8):558-569
Computational studies have led to models to understand some classic and contemporary asymmetric reactions involving organocatalysts. The Hajos-Parrish-Eder-Sauer-Wiechert reaction and intermolecular aldol reactions as well as Mannich reactions and oxyaminations catalyzed by proline and other amino acids, and Diels-Alder reactions catalyzed by MacMillan's chiral amine organocatalysts have been studied with density functional theory. Quantitative predictions for several new catalysts and reactions are provided. 相似文献
22.
The compatibilizing effect of the triblock copolymer poly(styrene‐b‐ethylene‐co‐butylene‐b‐styrene) (SEBS) on the morphological and mechanical properties of virgin and recycled polypropylene (PP)/high‐impact polystyrene (HIPS) blends was studied, with the properties optimized for rigid composite films. The components of the blend were obtained from municipal plastic waste, PP being acquired from mineral water bottles (PPb) and HIPS from disposable cups. These materials were preground, washed only with water, dried with hot air, and ground again (PPb) or agglutinated (HIPS). Blends with three different weight ratios of PPb and HIPS (6:1, 6:2, and 6:3) were prepared, and three different concentrations of SEBS (5, 6, and 7 wt %) were used for investigations of its compatibilizing effect. Scanning electron microscopy showed that SEBS reduced the diameter of dispersed HIPS particles in the globular and fibril shapes and improved the adhesion between the disperse phase and the matrix. However, SEBS interactions with PPb and HIPS influenced the mechanical properties of the compatibilized PPb/HIPS/SEBS blends. An adequate composition of PP/HIPS, for both virgin and recycled blends, for applications in composite films with characteristics similar to those of synthetic paper was obtained with a minimal amount of SEBS and a maximal HIPS/PP ratio in the range of concentrations studied. © 2003 Wiley Periodicals, Inc. J Appl Polym Sci 88: 2861–2867, 2003 相似文献
23.
Cleide Borsoi Betina Hansen Ruan Ezequiel Gemmer Marcos Aurélio Dahlem Júnior Edson Luiz Francisquetti Ademir José Zattera Ruth Marlene Campomanes Santana André Luis Catto 《应用聚合物科学杂志》2021,138(45):51350
This study presents the preparation of post-consumer polypropylene (r-PP) composites filled with 30 wt% yerba mate (YM) stick particles. To improve the fiber–matrix adhesion, three surface treatments were performed: alkaline treatment with sodium hydroxide (NaOH) and use of 3-aminopropyltriethoxysilane (APTS) and maleic anhydride graft polypropylene copolymer (PP-g-MA) as coupling agents. Mechanical properties including tensile, flexural, and impact resistance were determined, and chemical (Fourier transform infrared spectroscopy [FTIR]), physical (water absorption), and morphological analyses were performed. The main findings show that the treatments were efficient in improving the mechanical properties of the composites, with emphasis on the r-PP/YM30/APTS and r-PP/YM30/PP-g-MA composites, which proved to be superior in tensile, flexion and impact strength and absorption of water compared to the untreated composite. The morphological analysis showed a better interaction between the fiber and the polymeric matrix for the composites with YM/APTS and YM/PP-g-MA, which corroborates the results of tensile and flexural strength, as well as with the spectra of FTIR in which the chemical modification of the fibers is observed. However, the results show that these treatments are promising in obtaining composites with recycled matrix with better properties. 相似文献
24.
Samuel Mascarenhas Nick Degens Ana Paiva Rui Prada Gert Jan Hofstede Adrie Beulens Ruth Aylett 《Autonomous Agents and Multi-Agent Systems》2016,30(5):931-962
This work addresses the challenge of creating virtual agents that are able to portray culturally appropriate behavior when interacting with other agents or humans. Because culture influences how people perceive their social reality it is important to have agent models that explicitly consider social elements, such as existing relational factors. We addressed this necessity by integrating culture into a novel model for simulating human social behavior. With this model, we operationalized a particular dimension of culture—individualism versus collectivism—within the context of an interactive narrative scenario that is part of an agent-based tool for intercultural training. Using this scenario we conducted a cross-cultural study in which participants from a collectivistic country (Portugal) were compared with participants from an individualistic country (the Netherlands) in the way they perceived and interacted with agents whose behavior was either individualistic or collectivistic, according to the configuration of the proposed model. In the obtained results, Portuguese subjects rated the collectivistic agents more positively than the Dutch but both countries had a similarly positive opinion about the individualistic agents. This experiment sheds new light on how people from different countries differ when assessing the social appropriateness of virtual agents, while also raising new research questions on this matter. 相似文献
25.
IT infrastructure is definitely going green. From significant new regulations for IT equipment disposal to stringent energy-efficiency specifications for PCs and monitors to national standards for data center power savings, Green IT is an "in" topic. But many problems are unsolved. Will telecommuting make a difference or is it too difficult to manage? Will cloud computing reduce the number of large data centers? Can legislation diminish e-waste challenges? 相似文献
26.
Mohammed Mahmoud Yuqiong Liu Holly Hartmann Steven Stewart Thorsten Wagener Darius Semmens Robert Stewart Hoshin Gupta Damian Dominguez Francina Dominguez David Hulse Rebecca Letcher Brenda Rashleigh Court Smith Roger Street Jenifer Ticehurst Mark Twery Hedwig van Delden Ruth Waldick Denis White Larry Winter 《Environmental Modelling & Software》2009,24(7):798-808
Scenarios are possible future states of the world that represent alternative plausible conditions under different assumptions. Often, scenarios are developed in a context relevant to stakeholders involved in their applications since the evaluation of scenario outcomes and implications can enhance decision-making activities. This paper reviews the state-of-the-art of scenario development and proposes a formal approach to scenario development in environmental decision-making. The discussion of current issues in scenario studies includes advantages and obstacles in utilizing a formal scenario development framework, and the different forms of uncertainty inherent in scenario development, as well as how they should be treated. An appendix for common scenario terminology has been attached for clarity. Major recommendations for future research in this area include proper consideration of uncertainty in scenario studies in particular in relation to stakeholder relevant information, construction of scenarios that are more diverse in nature, and sharing of information and resources among the scenario development research community. 相似文献
27.
Jens Hauslage Medea Abbrecht Lars Hanke Ruth Hemmersbach Claudia Koch Wolfgang Hanke Florian P. M. Kohn 《Microgravity science and technology》2016,28(6):633-638
All life on earth has been established under conditions of stable gravity of 1g. Nevertheless, in numerous experiments the direct gravity dependence of biological processes has been shown on all levels of organization, from single molecules to humans. To study the effects especially of microgravity on biological systems, a variety of platforms are available, from drop towers to the ISS. Due to the costs of these platforms and their limited availability, as an alternative, numerous simulators have been developed for so called “simulated” microgravity. A classical systems is a clinostat, basically rotating a sample around one axis, and by integration of the gravity vector for 360° arguing that thus the effects of gravity are depleted. Indeed, a variety of studies has shown that taking out the direction of gravity from a biological system often results in consequences similar to the exposure of the system to real microgravity. Nevertheless, the opposite has been shown, too, and as a consequence the relevance of clinostats in microgravity research is still under discussion. To get some more insight into this problem we have constructed a small fluorescence clinostat and have studied the effects of clinorotation on the cytosolic calcium concentration of neuroglioma cells. The results have been compared to experiments with identical cells in real microgravity, utilizing parabolic flight missions. Our results show that in case of a cell suspension used in a small florescence clinostat within a tube diameter of 2mm, the effects of clinorotation are comparable to those under real microgravity, both showing a significant increase in intracellular calcium concentration. 相似文献
28.
29.
Manoli Pifarre Ruth Cobos 《International Journal of Computer-Supported Collaborative Learning》2010,5(2):237-253
This paper aims to better understand the development of students’ metacognitive learning processes when participating actively
in a CSCL system called KnowCat. To this end, a longitudinal case study was designed, in which 18 university students took
part in a 12-month (two semesters) learning project. The students followed an instructional process, using specific features
of the KnowCat design to support and improve their interaction processes, especially peer-learning processes. Our research
involved both supervising the students’ collaborative learning processes throughout the learning project and focusing our
analysis on the qualitative evolution of their interaction processes and of their metacognitive learning processes. The results
of the current research suggest that the pedagogical use of the KnowCat system may favour and improve the development of the
students’ metacognitive learning processes. In addition, the implications of the design of CSCL networks and related pedagogical
issues are discussed. 相似文献
30.
Dolors Costal Cristina Gómez Anna Queralt Ruth Raventós Ernest Teniente 《Software and Systems Modeling》2008,7(4):469-486
An important aspect in the specification of conceptual schemas is the definition of general constraints that cannot be expressed
by the predefined constructs provided by conceptual modeling languages. This is generally achieved by using general-purpose
languages like OCL. In this paper we propose a new approach that facilitates the definition of such general constraints in
UML. More precisely, we define a profile that extends the set of predefined UML constraints by adding certain types of constraints
that are commonly used in conceptual schemas. We also show how our proposal facilitates reasoning about the constraints and
their automatic code generation, study the application of our ideas to the specification of two real-life applications, and
present a prototype tool implementation.
相似文献
Ernest TenienteEmail: |