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排序方式: 共有1239条查询结果,搜索用时 15 毫秒
941.
Zupeng Chen Sharon Mitchell Evgeniya Vorobyeva Rowan K. Leary Roland Hauert Tom Furnival Quentin M. Ramasse John M. Thomas Paul A. Midgley Dariya Dontsova Markus Antonietti Sergey Pogodin Núria López Javier Pérez‐Ramírez 《Advanced functional materials》2017,27(8)
Graphitic carbon nitride (g‐C3N4) exhibits unique properties as a support for single‐atom heterogeneous catalysts (SAHCs). Understanding how the synthesis method, carrier properties, and metal identity impact the isolation of metal centers is essential to guide their design. This study compares the effectiveness of direct and postsynthetic routes to prepare SAHCs by incorporating palladium, silver, iridium, platinum, or gold in g‐C3N4 of distinct morphology (bulk, mesoporous and exfoliated). The speciation (single atoms, dimers, clusters, or nanoparticles), distribution, and oxidation state of the supported metals are characterized by multiple techniques including extensive use of aberration‐corrected electron microscopy. SAHCs are most readily attained via direct approaches applying copolymerizable metal precursors and employing high surface area carriers. In contrast, although post‐synthetic routes enable improved control over the metal loading, nanoparticle formation is more prevalent. Comparison of the carrier morphologies also points toward the involvement of defects in stabilizing single atoms. The distinct metal dispersions are rationalized by density functional theory and kinetic Monte Carlo simulations, highlighting the interplay between the adsorption energetics and diffusion kinetics. Evaluation in the continuous three‐phase semihydrogenation of 1‐hexyne identifies controlling the metal–carrier interaction and exposing the metal sites at the surface layer as key challenges in designing efficient SAHCs. 相似文献
942.
Daniel Glasner Meirav Galun Sharon Alpert Ronen Basri Gregory Shakhnarovich 《Image and vision computing》2012
We describe an approach to category-level detection and viewpoint estimation for rigid 3D objects from single 2D images. In contrast to many existing methods, we directly integrate 3D reasoning with an appearance-based voting architecture. Our method relies on a nonparametric representation of a joint distribution of shape and appearance of the object class. Our voting method employs a novel parameterization of joint detection and viewpoint hypothesis space, allowing efficient accumulation of evidence. We combine this with a re-scoring and refinement mechanism, using an ensemble of view-specific support vector machines. We evaluate the performance of our approach in detection and pose estimation of cars on a number of benchmark datasets. Finally we introduce the “Weizmann Cars ViewPoint” (WCVP) dataset, a benchmark for evaluating continuous pose estimation. 相似文献
943.
Although advanced technologies are available for measuring and sampling fire intensity, their costs, limitations, or complexity often preclude general use in field experiments. The lack of quality measurements exacerbates the task of relating ecological responses directly to the fires that cause them. In this paper, a new technique for measuring flame height, describing its distribution, and relating it to fire intensity is presented. Flame pulsation in natural fuels is also examined. 相似文献
944.
Trung Dac Nguyen Carolyn L. Phillips Joshua A. Anderson Sharon C. Glotzer 《Computer Physics Communications》2011,(11):2307-2313
Molecular dynamics (MD) methods compute the trajectory of a system of point particles in response to a potential function by numerically integrating Newton?s equations of motion. Extending these basic methods with rigid body constraints enables composite particles with complex shapes such as anisotropic nanoparticles, grains, molecules, and rigid proteins to be modeled. Rigid body constraints are added to the GPU-accelerated MD package, HOOMD-blue, version 0.10.0. The software can now simulate systems of particles, rigid bodies, or mixed systems in microcanonical (NVE), canonical (NVT), and isothermal-isobaric (NPT) ensembles. It can also apply the FIRE energy minimization technique to these systems. In this paper, we detail the massively parallel scheme that implements these algorithms and discuss how our design is tuned for the maximum possible performance. Two different case studies are included to demonstrate the performance attained, patchy spheres and tethered nanorods. In typical cases, HOOMD-blue on a single GTX 480 executes 2.5–3.6 times faster than LAMMPS executing the same simulation on any number of CPU cores in parallel. Simulations with rigid bodies may now be run with larger systems and for longer time scales on a single workstation than was previously even possible on large clusters. 相似文献
945.
Harald Fecher Sharon Shoham 《International Journal on Software Tools for Technology Transfer (STTT)》2011,13(4):289-306
A key technique for the verification of programs is counterexample-guided abstraction–refinement (CEGAR). Grumberg et al.
(LNCS, vol 3385, pp. 233–249. Springer, Berlin, 2005; Inf Comput 205(8):1130–1148, 2007) developed a CEGAR-based algorithm for the modal μ-calculus. There, every abstract state is split in a refinement step. In this paper, the work of Grumberg et al. is generalized
by presenting a new CEGAR-based algorithm for the μ-calculus. It is based on a more expressive abstract model and applies refinement only locally (at a single abstract state),
i.e., the lazy abstraction technique for safety properties is adapted to the μ-calculus. Furthermore, it separates refinement determination from the (3-valued based) model checking. Three different heuristics
for refinement determination are presented and illustrated. 相似文献
946.
947.
Bell JL Collins JW Wolf L Gronqvist R Chiou S Chang WR Sorock GS Courtney TK Lombardi DA Evanoff B 《Ergonomics》2008,51(12):1906-1925
In 2007, the Bureau of Labor Statistics reported that the incidence rate of lost workday injuries from slips, trips and falls (STFs) on the same level in hospitals was 35.2 per 10,000 full-time equivalents (FTE), which was 75% greater than the average rate for all other private industries combined (20.2 per 10,000 FTEs). The objectives of this 10-year (1996-2005) longitudinal study were to: 1) describe occupational STF injury events in hospitals; 2) evaluate the effectiveness of a comprehensive programme for reducing STF incidents among hospital employees. The comprehensive prevention programme included analysis of injury records to identify common causes of STFs, on-site hazard assessments, changes to housekeeping procedures and products, introduction of STF preventive products and procedures, general awareness campaigns, programmes for external ice and snow removal, flooring changes and slip-resistant footwear for certain employee subgroups. The hospitals' total STF workers' compensation claims rate declined by 58% from the pre-intervention (1996-1999) rate of 1.66 claims per 100 FTE to the post-intervention (2003-2005) time period rate of 0.76 claims per 100 FTE (adjusted rate ratio = 0.42, 95% CI: 0.33-0.54). STFs due to liquid contamination (water, fluid, slippery, greasy and slick spots) were the most common cause (24%) of STF claims for the entire study period 1996-2005. Food services, transport/emergency medical service and housekeeping staff were at highest risk of a STF claim in the hospital environment. Nursing and office administrative staff generated the largest numbers of STF claims. STF injury events in hospitals have a myriad of causes and the work conditions in hospitals are diverse. This research provides evidence that implementation of a broad-scale prevention programme can significantly reduce STF injury claims. 相似文献
948.
Joss Moorkens Sharon O’Brien Igor A. L. da Silva Norma B. de Lima Fonseca Fabio Alves 《Machine Translation》2015,29(3-4):267-284
Human rating of predicted post-editing effort is a common activity and has been used to train confidence estimation models. However, the correlation between human ratings and actual post-editing effort is under-measured. Moreover, the impact of presenting effort indicators in a post-editing user interface on actual post-editing effort has hardly been researched. In this study, ratings of perceived post-editing effort are tested for correlations with actual temporal, technical and cognitive post-editing effort. In addition, the impact on post-editing effort of the presentation of post-editing effort indicators in the user interface is also tested. The language pair involved in this study is English-Brazilian Portuguese. Our findings, based on a small sample, suggest that there is little agreement between raters for predicted post-editing effort and that the correlations between actual post-editing effort and predicted effort are only moderate, and thus an inefficient basis for MT confidence estimation. Moreover, the presentation of post-editing effort indicators in the user interface appears not to impact on actual post-editing effort. 相似文献
949.
Stilts are elevated tools that are frequently used by construction workers to raise workers 18-40 inches above the ground. The objective of this laboratory study was to evaluate the potential loss of postural stability associated with the use of stilts in various foot placements. Twenty construction workers with at least 1 year of experience in the use of stilts participated in this study. One Kistler™ force platform was used to collect kinetic data. Participants were tested under six-foot-placement conditions. These 6 experimental conditions were statically tested under all combinations of 3 levels of elevation: 0″ (no stilts), 24″ stilt height and 40″ stilt height. SAS mixed procedure was used to evaluate the effect of different experimental conditions. The results of the multivariate analysis of variance (MANOVA) and repeated measures of univariate analyses of variance (ANOVAs) demonstrated that stilt height, foot-placement direction, and foot-placement width all had significant effects on the whole-body postural stability. This study found that the higher the stilts were elevated, the greater the postural instability. A stance position with one foot placed forward of the other foot produced greater postural instability than a position with the feet parallel and directly beneath the body. This study found that placement of the feet parallel and directly beneath the body, with the feet positioned a half shoulder width apart, caused a greater amount of postural sway and instability than one and one-and-half shoulder width. This study also found that construction workers using the stilts could perceive the likely postural instability due to the change in foot placements. 相似文献
950.