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91.
Anubhav Jain Ivano E. Castelli Geoffroy Hautier David H. Bailey Karsten W. Jacobsen 《Journal of Materials Science》2013,48(19):6519-6534
We examine the performance of genetic algorithms (GAs) in uncovering solar water light splitters over a space of almost 19,000 perovskite materials. The entire search space was previously calculated using density functional theory to determine solutions that fulfill constraints on stability, band gap, and band edge position. Here, we test over 2500 unique GA implementations in finding these solutions to determine whether GA can avoid the need for brute force search, and thereby enable larger chemical spaces to be screened within a given computational budget. We find that the best GAs tested offer almost a 6 times efficiency gain over random search, and are comparable to the performance of a search based on informed chemical rules. In addition, the GA is almost 10 times as efficient as random search in finding half the solutions within the search space. By employing chemical rules, the performance of the GA can be further improved to approximately 12–17 better than random search. We discuss the effect of population size, selection function, crossover function, mutation rate, fitness function, and elitism on the final result, finding that selection function and elitism are especially important to GA performance. In addition, we determine that parameters that perform well in finding solar water splitters can also be applied to discovering transparent photocorrosion shields. Our results indicate that coupling GAs to high-throughput density functional calculations presents a promising method to rapidly search large chemical spaces for technological materials. 相似文献
92.
Corneal collagen crosslinking (CXL) is a non invasive technique used in halting the progression of keratoconus. Complications with this modality are rare. We report a case of an 8-year-old child who developed sterile infiltrates in the immediate postoperative period after uneventful corneal collagen crosslinking for keratoconus. The infiltrates resolved with topical steroid therapy. There was also present coexisting vernal keratoconjunctivitis (VKC) which was controlled with topical 2% cyclosporine A eye drops prior to crosslinking treatment. This case highlights importance of controlling VKC prior to CXL in keratoconus as it adds to the risk of developing post operative sterile keratitis. 相似文献
93.
Bhawani Narayan Satyaprasad P. Senanayak Ankit Jain K. S. Narayan Subi J. George 《Advanced functional materials》2013,23(24):3053-3060
Oligo(p‐phenylenevinylenes) (OPVs) with amphiphilic character are synthesized and their self‐assembly characteristics studied. Careful studies point at two morphologically different states of assemblies, with one being two dimensional sheets and the other as rolled tubes. This is also the first time that self‐assembled sheets are achieved for OPVs. Morphological and photo‐physical studies reveal a unique aggregate to aggregate transition between rolled tubes and two dimensional sheets, which is outlined as a more thermodynamic aggregate. The thermodynamic aggregate (2D sheet) is better ordered and consists of chromophores that are better excitonically coupled. The mobilities of these aggregates are also studied for a field effect transistor device and as expected sheets supersede rolled tubes by a couple of orders. More interestingly, the mobility values obtained for the well ordered chromophores in sheets is three orders higher than any other self‐assembled OPV previously reported. It is hypothesized that the better π interactions enforced by the amphiphilic design and the resultant supramolecular organization is a prime factor for such a remarkable rise in mobilities. 相似文献
94.
G Venkata Ramana Balaji Padya Vadali V S S Srikanth P K Jain 《Bulletin of Materials Science》2014,37(3):585-588
Composite thin film containing polyaniline (PANI) coated small diameter carbon nanotubes (SDCNTs)/PANI nanofibres (NFs) has been prepared using an easy in situ rapid mixing chemical oxidative polymerization method. SDCNTs thin film was obtained using thermal chemical vapour deposition method in a separate experiment, whilst PANI NFs are formed in situ during the synthesis of composite. In the composite, PANI coated SDCNTs are uniformly distributed among PANI NFs. The presence of SDCNTs during the composite synthesis does not influence the nucleation and growth of PANI NFs. Raman analysis shows a good interaction between PANI and SDCNTs. Room temperature d.c. electrical sheet resistance of SDCNTs/PANI NFs composite thin film surface is three orders lesser than that of PANI NFs thin film (PANI NFs have the same morphology as in the composite) synthesized using the same method but without the presence of SDCNTs. 相似文献
95.
Sanjay Kumar Ankur Jain Hiroki Miyaoka Takayuki Ichikawa Yoshitsugu Kojima 《International Journal of Hydrogen Energy》2017,42(27):17178-17183
Bis(cyclopentadienyl) nickel II is one of the best precursors of nickel catalyst which remarkably improved the hydrogen absorption-desorption of Mg–MgH2 system. The X-ray photoelectron spectroscopy (XPS) and Furrier Transformed Infrared Spectroscopy (FTIR) analyses revealed that bis (cyclopentadienyl) nickel II decomposed into metallic nickel during ball milling with MgH2. The nickel thus formed has homogeneously doped over the Mg - MgH2 surface. The Ni-doped Mg-MgH2 have shown the excellent catalytic effect on hydrogen absorption-desorption. The catalyzed MgH2 could desorb hydrogen below 225 °C (Tonset) under Ar flow, and absorb hydrogen at 50 °C under 1.5 MPa H2 pressure. The hydrogen absorption-desorption temperatures are remarkably decreased as compared to the uncatalyzed Mg-MgH2 system under the identical experimental conditions. 相似文献
96.
R. K. Jain S. Datta S. Majumder A. Dutta 《Journal of Intelligent and Robotic Systems》2014,74(3-4):547-569
This paper presents a new design of multi micro manipulation system using ionic polymer metal composite (IPMC) micro grippers for robotic micro assembly where IPMC is used as a light weight actuator for developing the micro grippers. It has the potential of large displacement, low mass force generation and misalignment compensation ability during micro manipulation. These capabilities are utilized for handling of miniature parts like pegs. The analysis of IPMC micro gripper and manipulator are carried out for developing a multi micro manipulation system that can handle pegs in micro assembly operation for shifting one to another hole position in a large work space (100 mm × 100 mm). By developing a prototype, it is demonstrated that IPMC based micro grippers are capable of handling the peg-in-hole assembly tasks in a multi micro manipulation system. 相似文献
97.
Resonant ultrasound spectroscopy (RUS) is an NDE technique that evaluates a sample based on its predicted resonant behavior, but RUS is limited by lack of spatial resolution and small specimen size. Air-coupled ultrasonic resonance imaging (ACURI) is a new NDE technique that is based on RUS but introduces a spatial resolution by generating an image of the flexural vibration modes. This paper presents experimental results of ACURI applied to hexagonal silicon carbide tiles. Frequency sweep scans demonstrate the ability of air-coupled transducers to detect resonance modes. Several mode shapes are imaged and compared to Finite Element simulations with good agreement. Visual comparison allows for easy detection of material differences such as density variations. 相似文献
98.
Jitendra Sharma Prabhakaran Ponnusamy Pazhaniandi Vinay Kumar Tanwar Sudip Kumar Das Meena Goswami 《International Journal of Food Science & Technology》2012,47(1):61-66
This investigation was carried out to evaluate the antioxidant effect of turmeric (turmeric 1000 ppm, turmeric 5000 ppm), nitrite (nitrite 200 ppm) and ascorbic acid (ascorbic acid 500 ppm) on raw minced chicken stored at 4 ± 1 °C. Physicochemical properties [pH, water activity, cooking loss, thiobarbituric acid (TBA) value, peroxide value (PV), free fatty acid (FFA)] were evaluated on 0, 2, 4 and 6th day of storage. Highly significant differences (P < 0.01) in pH, TBA value, PV and FFA value were noticed between treatments and between storage periods. TBA values were observed to be lowest for nitrite 200 ppm and then turmeric 5000 ppm, and there was no significant difference between nitrite 200 ppm and turmeric 5000 ppm, and both were superior to ascorbic acid 500 ppm and turmeric 1000 ppm. Among different treatments, PV was found to be lowest in turmeric 5000 ppm and highest in nitrite 200 ppm. FFA value was found to be lowest in turmeric 5000 ppm and highest in ascorbic acid 500 ppm among all treated samples. It can be concluded that turmeric has potential to replace synthetic antioxidants presently used in meat processing with many added advantages. 相似文献
99.
100.
The design of rolling element bearings has been a challenging task in the field of mechanical engineering. While most of the real aspects of the design are never disclosed by bearing manufacturers, the common engineer is left with no other alternative than to refer to standard tables and charts containing the bearing performance characteristics. This paper presents a more viable method to solve this problem using genetic algorithms (GAs). Since the algorithm is basically a guided random search, it weakens the chances of getting trapped in local maxima or minima. The method used has yielded improved performance parameters than those catalogued in standard tables. 相似文献