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41.
B. Nagy Y. N. Khaydukov L. F. Kiss S. Sajti D. G. Merkel F. Tanczikó A. S. Vasenko R. O. Tsaregorodsev A. Rühm T. Keller L. Bottyán 《Journal of Superconductivity and Novel Magnetism》2013,26(5):1957-1961
The thickness (d F) and concentration (x) dependence of the Curie temperature of Ni x Cu1?x (d F) ferromagnetic alloy layers (x=0.55, 0.65, d F=[4.5 nm÷12 nm]) in contact with a vanadium layer was studied. The Curie temperature of the ferromagnetic layers depends on the thickness when it is comparable with the transition layer between the F and the vanadium layers, which is attributed to the proximity coupling of the interface region with the rest of the F layer. The present study provides valuable information for fabrication of samples with controlled exchange coupling strength for studies of superconductor/ferromagnet proximity effects. 相似文献
42.
Vladimir V. Pushkarev Zhongwei Zhu Kwangjin An Antoine Hervier Gabor A. Somorjai 《Topics in Catalysis》2012,55(19-20):1257-1275
We aim to develop novel catalysts that exhibit high activity, selectivity and stability under real catalytic conditions. In the recent decades, the fast development of nanoscience and nanotechnology has allowed synthesis of nanoparticles with well-defined size, shape and composition using colloidal methods. Utilization of mesoporous oxide supports effectively prevents the nanoparticles from aggregating at high temperatures and high pressures. Nanoparticles of less than 2?nm sizes were found to show unique activity and selectivity during reactions, which was due to the special surface electronic structure and atomic arrangements that are present at small particle surfaces. While oxide support materials are employed to stabilize metal nanoparticles under working conditions, the supports are also known to strongly interact with the metals through encapsulation, adsorbate spillover, and charge transfer. These factors change the catalytic performance of the metal catalysts as well as the conductivity of oxides. The employment of new in situ techniques, mainly high-pressure scanning tunneling microscopy (HPSTM) and ambient-pressure X-ray photoelectron spectroscopy (APXPS) allows the determination of the surface structure and chemical states under reaction conditions. HPSTM has identified the importance of both adsorbate mobility to catalytic turnovers and the metal substrate reconstruction driven by gaseous reactants such as CO and O2. APXPS is able to monitor both reacting species at catalyst surfaces and the oxidation state of the catalyst while it is being exposed to gases. The surface composition of bimetallic nanoparticles depends on whether the catalysts are under oxidizing or reducing conditions, which is further correlated with the catalysis by the bimetallic catalytic systems. The product selectivity in multipath reactions correlates with the size and shape of monodisperse metal nanoparticle catalysts in structure sensitive reactions. 相似文献
43.
Valéria Nagy Roland Tengölics Gert Schansker Gábor Rákhely Kornél L. Kovács Győző Garab Szilvia Z. Tóth 《International Journal of Hydrogen Energy》2012
The green alga Chlamydomonas reinhardtii is capable of photoproducing molecular hydrogen following sulphur deprivation, which results in anaerobiosis and a suppression of oxygen evolution and thus an alleviation of the inhibitory effect of oxygen on the hydrogenase. At the same time it transiently maintains a limited supply of electrons arising from photosystem II (PSII) to the hydrogenase (Melis and Happe Plant Physiol 2001; 127:740–748). In this work, using fast chl a fluorescence and P700 measurements, we show that ascorbate (Asc), a naturally occurring PSII alternative electron donor, is capable of donating electrons to PSII in heat-treated and sulphur-deprived cells and this can be significantly accelerated by supplementing the culture with 10 mM Asc. It also enhances, about three-fold, the photoproduction of hydrogen in cells subjected to sulphur deprivation as shown by gas chromatography. Similar stimulation was obtained in the presence of diphenylcarbazide (DPC), an artificial PSII electron donor. Asc and DPC also facilitated the anaerobiosis of cells, probably via super reducing the oxygen evolving complex while feeding electrons to PSII reaction centres and the linear electron transport chain, and ultimately to the hydrogenase – as shown by the significant DCMU-sensitivity of the light-induced Asc- and DPC-dependent re-reduction of P700+ and hydrogen evolution. 相似文献
44.
Kristof Molnar David Juriga Peter M Nagy Katalin Sinko Angela Jedlovszky‐Hajdu Miklos Zrinyi 《Polymer International》2014,63(9):1608-1615
Biocompatible synthetic polymer gel scaffolds for tissue engineering and regenerative medicine were prepared by reactive electrospinning. Protein‐like nano‐ and microfibres from chemically crosslinked polysuccinimide were obtained. Fibrous poly(aspartic acid) gels with size similar to that of extracellular matrix were obtained by hydrolysis of the polysuccinimide gel fibres. The effects of process parameters on fibre morphology (diameter, swelling degree) and chemical structure were investigated. Sub‐micrometre‐sized biocompatible fibrous scaffolds from a poly(amino acid) is a novel approach with great promise in several biomedical applications due to the tailor‐made synthetic nature, extreme purity and possibility of production on a large scale. © 2014 Society of Chemical Industry 相似文献
45.
David W. Embley Mukkai S. Krishnamoorthy George Nagy Sharad Seth 《International Journal on Document Analysis and Recognition》2016,19(2):119-138
Much of the world’s quantitative data reside in scattered web tables. For a meaningful role in Big Data analytics, the facts reported in these tables must be brought into a uniform framework. Based on a formalization of header-indexed tables, we proffer an algorithmic solution to end-to-end table processing for a large class of human-readable tables. The proposed algorithms transform header-indexed tables to a category table format that maps easily to a variety of industry-standard data stores for query processing. The algorithms segment table regions based on the unique indexing of the data region by header paths, classify table cells, and factor header category structures of two-dimensional as well as the less common multidimensional tables. Experimental evaluations substantiate the algorithmic approach to processing heterogeneous tables. As demonstrable results, the algorithms generate queryable relational database tables and semantic-web triple stores. Application of our algorithms to 400 web tables randomly selected from diverse sources shows that the algorithmic solution automates end-to-end table processing. 相似文献
46.
Robert C. Mathews Irving M. Lane Lewis G. Roussel Mark S. Nagy Dawn E. Haptonstahl Drew B. Brock 《人工智能实验与理论杂志》2013,25(3-4):259-276
Three experiments investigated procedures derived from research on knowledge acquisition, group processes, and artificial intelligence for facilitating the development of expertise. In each experimental session, subjects learned to control a simulated sugar production factory. Then they formulated written policies for controlling sugar production either alone as individuals or in small groups. An adaptive AI system provided feedback on policy quality. The research also investigated the use of forced reflective practice in which learners attempted to predict what their policy would do while performing the task. The AI system provided feedback about what their policy would have done in each situation and the outcome based on their policy's response or their suggested alternative response. Results indicated that group interaction and feedback from the AI system improved policy quality. However, only when all three procedures were employed, group interaction, AI feedback, and forced reflective practice, was the development of individual expertise on the task enhanced. 相似文献
47.
Lately, demand for fast failure recovery in IP networks has become compelling. The Loop-Free Alternates (LFA) specification is a simple IP Fast ReRoute (IPFRR) scheme proposed by the IETF that does not require profound changes to the network infrastructure before deployment. However, this simplicity comes at a severe price, because LFA does not provide complete protection for all possible failure cases in a general topology. This is even more so if network components are prone to fail jointly. In this paper, we study an important network optimization problem arising in this context, the so called LFA graph extension problem, which asks for augmenting the topology with new links in an attempt to improve the LFA failure case coverage. Unfortunately, this problem is NP-complete. The main contributions of the paper are a novel extension of the bipartite graph model for the LFA graph extension problem to the multiple-failure case using the model of Shared Risk Groups, and a suite of accompanying heuristics to obtain approximate solutions. We also compare the performance of the algorithms in extensive numerical studies and we conclude that the optimum can be approximated well in most cases relevant to practice. 相似文献
48.
Francesco
Borgioli David Hajdu Tamas Insperger Gabor Stepan Wim Michiels 《International journal for numerical methods in engineering》2020,121(16):3505-3528
The article presents a pseudospectral approach to assess the stability robustness of linear time-periodic delay systems, where periodic functions potentially present discontinuities and the delays may also periodically vary in time. The considered systems are subject to linear real-valued time-periodic uncertainties affecting the coefficient matrices, and the presented method is able to fully exploit structure and potential interdependencies among the uncertainties. The assessment of robustness relies on the computation of the pseudospectral radius of the monodromy operator, namely, the largest Floquet multiplier that the system can attain within a given range of perturbations. Instrumental to the adopted novel approach, a solver for the computation of Floquet multipliers is introduced, which results into the solution of a generalized eigenvalue problem which is linear w.r.t. (samples of) the original system matrices. We provide numerical simulations for popular applications modeled by time-periodic delay systems, such as the inverted pendulum subject to an act-and-wait controller, a single-degree-of-freedom milling model and a turning operation with spindle speed variation. 相似文献
49.
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