全文获取类型
收费全文 | 504篇 |
免费 | 19篇 |
国内免费 | 2篇 |
专业分类
电工技术 | 48篇 |
综合类 | 2篇 |
化学工业 | 173篇 |
金属工艺 | 13篇 |
机械仪表 | 27篇 |
建筑科学 | 12篇 |
能源动力 | 15篇 |
轻工业 | 35篇 |
水利工程 | 1篇 |
石油天然气 | 1篇 |
无线电 | 38篇 |
一般工业技术 | 79篇 |
冶金工业 | 16篇 |
原子能技术 | 20篇 |
自动化技术 | 45篇 |
出版年
2023年 | 7篇 |
2022年 | 7篇 |
2021年 | 18篇 |
2020年 | 5篇 |
2019年 | 7篇 |
2018年 | 14篇 |
2017年 | 6篇 |
2016年 | 10篇 |
2015年 | 13篇 |
2014年 | 19篇 |
2013年 | 36篇 |
2012年 | 21篇 |
2011年 | 38篇 |
2010年 | 22篇 |
2009年 | 14篇 |
2008年 | 25篇 |
2007年 | 16篇 |
2006年 | 13篇 |
2005年 | 20篇 |
2004年 | 17篇 |
2003年 | 17篇 |
2002年 | 16篇 |
2001年 | 16篇 |
2000年 | 9篇 |
1999年 | 9篇 |
1998年 | 7篇 |
1997年 | 4篇 |
1996年 | 6篇 |
1994年 | 6篇 |
1993年 | 5篇 |
1992年 | 6篇 |
1991年 | 6篇 |
1989年 | 6篇 |
1987年 | 4篇 |
1986年 | 8篇 |
1985年 | 5篇 |
1984年 | 4篇 |
1982年 | 5篇 |
1981年 | 5篇 |
1980年 | 4篇 |
1979年 | 4篇 |
1978年 | 5篇 |
1976年 | 6篇 |
1975年 | 4篇 |
1974年 | 4篇 |
1973年 | 3篇 |
1972年 | 4篇 |
1971年 | 3篇 |
1970年 | 5篇 |
1969年 | 3篇 |
排序方式: 共有525条查询结果,搜索用时 31 毫秒
71.
Florian Weyland Matias Acosta Malte Vögler Yoshitaka Ehara Jürgen Rödel Nikola Novak 《Journal of Materials Science》2018,53(13):9393-9400
The electric field–temperature phase diagrams of three bismuth sodium titanate-based relaxor ferroelectrics are reported, namely 0.94(Na1/2Bi1/2TiO3)–0.06(BaTiO3), 0.80(Na1/2Bi1/2TiO3)–0.20(K1/2Bi1/2TiO3) and 0.75(Na1/2Bi1/2TiO3)–0.25(SrTiO3). Relaxor behavior is demonstrated by temperature-dependent dielectric permittivity measurements in the unpoled and poled states, as well as by the field-induced phase transition into a ferroelectric phase from the relaxor phase. From temperature-dependent thermometry measurements, we identified the threshold electric field to induce the ferroelectric phase and obtained the released latent heat of the phase transition. We determined the nonergodic and ergodic relaxor phase temperature range based on the absence or presence of reversibility of the relaxor to ferroelectric transition. For all three compositions, the electric field–temperature phase diagram was constructed and a critical point was identified. The constructed electric field–temperature phase diagrams are useful to find optimum operational ranges of ferroelectrics and relaxors for electromechanical and electrocaloric applications. 相似文献
72.
Yuichi Tominaga Keiji Fukushima Yoshitaka Takezawa Daisuke Shimamoto Yusuke Imai Yuji Hotta 《Advanced Powder Technology》2017,28(8):1911-1919
The exfoliation of layered muscovite with non-swelling property has been performed by combining various processes, such as heating, intercalation, and wet-jet milling. The c axis of muscovite was expanded from 2004.0 to 2022.8 pm at 800 °C without the destruction of crystallinity of muscovite. The heating at 800 °C led to the weak attraction force between potassium ions and silicate layers by hydroxylation of muscovite. The muscovite heated at 800 °C progressed the intercalation of dodecylammonium chloride (DDAC) into the layers effectively. Furthermore, the DDAC molecules were inserted to the interlayer of muscovite effectively by suppressing the formation of micelle of DDAC. The sedimentation test of wet-jet milled muscovite slurry showed that the relative packing density of muscovite was decreasing with increasing the amount of the intercalated DDAC. As results, the aspect ratio of muscovite prepared with combining the heating, the intercalation and the wet-jet milling was increased by 253% as compared to the raw muscovite. The aspect ratio was calculated from laser particle size distribution and thickness size distribution which was estimated from field emission-scanning electron microscopic images. The expansion of the interlayer led to the effective exfoliation of muscovite with high aspect ratio. 相似文献
73.
We consider the problem of mining web access patterns with super-pattern constraint. This constraint requires that the sequential patterns in the sequence database must contain a particular set of patterns as sub-patterns. One common application of this constraint is web usage mining which mines the user access behavior on the web. In this paper, we introduce an efficient strategy for mining web access patterns with super-pattern constraint that requires only one database scan. Firstly, we present the MWAPC (M ining W eb A ccess P atterns based on super-pattern C onstraint) algorithm, in which each frequent pattern has to be checked if it contains at least one pattern from a user-defined set of patterns. Then we develop an effective algorithm, called EMWAPC that prunes the search space at the beginning of mining process and avoids checking the constraints one by one based on three proposed propositions. We have conducted the experiments on real web log databases. The experimental results show that the proposed algorithms outperform the previous methods. 相似文献
74.
Eiichi Obataya Yuhzo Furuta Yoshitaka Ohno Misato Norimoto Bunichiro Tomita 《应用聚合物科学杂志》2002,83(11):2288-2294
The effects of aging and moisture on the dynamic viscoelastic properties of three oriental lacquer films were investigated. With aging over 1000 days at room temperature, the glass‐transition temperature of the lacquer films (Tα) shifted to higher temperatures, the maximum loss tangent (tanδα) decreased, and the storage modulus at 20°C (E) increased. These changes were analogous irrespective of lacquers. With increasing moisture content, E decreased and tanδ increased at room temperature. Although the equilibrium moisture content of the virgin lacquer (sap) film was higher than that of the clear lacquer film, its E and tanδ were more stable with an increase of moisture content. It was speculated that the polysaccharides aggregated in the sap film did not effectively contribute to the mechanical properties of the film, while their hygroscopicity resulted in higher moisture content. © 2002 Wiley Periodicals, Inc. J Appl Polym Sci 83: 2288–2294, 2002 相似文献
75.
Effect of water on vapor phase photografting on cellulose was investigated at 60°C. An activated grafting of methyl methacrylate by water contained in the sample was observed in the experiment. The effect of water was commonly recorded irrespective of the type of cellulose derivatives such as cellulose acetate (degree of substitution, DS = 0.18 and 0.33), cellulose nitrate (DS = 0.35 and 0.75), and carboxymethl cellulose (DS = 0.19 and 0.74). Organic solvents can also be used in place of water, indicating that the percent grafting decreases in the order, water > methanol > acetone > cyclohexane. From ESR studies, water in the sample was found to contribute to the decay of cellulose radicals rather than to the radical formation. The decay was accelerated by organic solvents, and the magnitude of the effect was in the order, water ≈ methanol > acetone > cyclohexane. Based on the above investigation, it was presumed that water contained in the sample cannot contribute directly to the formation of cellulose radicals which may initiate grafting, but mostly promotes the penetration of monomer into cellulose fibers. Such penetration could lead cellulose radicals to an effective initiation of grafting. 相似文献
76.
Fe-Pt nanoparticles of 3.5 nm in average particle diameter are obtained with the simultaneous chemical reduction of platinum acetylacetonate and the thermal decomposition of iron pentacarbonyl. Because the as-synthesized particles are superparamagnetic at room temperature, they must be transformed to L10 ordered phase by annealing at temperatures above 773 K to apply to high-density magnetic recording media. However, the annealing at such high temperatures induces the coalescence and inter-particle sintering. In the present paper, to solve the problem caused by the annealing, we use ultraviolet-ozone treatment to modify particle surface. Even after annealing at 773 K, the crystalline size is kept at 4.4 nm. Furthermore, coercivity is higher than that without the ultraviolet-ozone treatment. 相似文献
77.
Koji Takahashi Kenichi Uchiide Yoshitaka Kimura Wataru Nakao Kotoji Ando Masahiro Yokouchi 《Journal of the American Ceramic Society》2007,90(7):2159-2164
A mullite/SiC whisker/SiC particle multi-composite, having excellent crack-healing ability and mechanical properties, was hot pressed in order to investigate the crack-healing behavior under stress and the resultant fatigue strength at the temperature of healing. A semi-elliptical surface crack 100 μm in surface length was introduced on each specimen. The pre-cracked specimens were crack healed under cyclic or constant stress by using a three-point bending stress at 1473 K, and the resultant bending strength and cyclic fatigue strength were measured at 1473 K. The pre-crack on the surface of the specimens could be healed even under stress. The threshold stresses for crack healing, as determined by evaluating the strengths of crack-healed specimens at a healing temperature of 1473 K, were 170 MPa for both constant and cyclic stresses, corresponding to 77% of the bending strength of the pre-cracked specimens. The static and cyclic fatigue behaviors of crack-healed specimens were also investigated at a healing temperature of 1473 K. 相似文献
78.
Yoshitaka Uchiyama 《Wear》1981,74(2):247-262
To obtain information about the basic processes involved in the formation of wear particles of polytetrafluoroethylene (PTFE), the rubbing surface of a PTFE pin was observed through a glass disk.In the initial stages of rubbing, small PTFE fragments transferred to the glass disk from the PTFE pin but did not necessarily adhere strongly to the glass disk. Some wear fragments were observed moving against the PTFE pin at a speed lower than the sliding speed of the glass disk. The fragments at higher travelling speeds combined with the fragments at lower travelling speeds and increased in size. The fragments also increased in size by scratching the surface of the PTFE pin.In steady state rubbing, large and small fragments were observed and the enlarged fragments were successively detached from the glass disk. The variation in the volume and the travelling speed of the fragments with rubbing was also examined. The total increase in the volume of transferred fragments in a definite sliding distance was found to be similar to the volume of removed fragments. 相似文献
79.
Uichiro Mizutani Takashi Yamaguchi Hiroshi Ikuta Tetsuya Tomofuji Yosuke Yanagi Yoshitaka Itoh Tetsuo Oka 《Materials Science and Engineering: B》2008,151(1):84
We have developed the two-cathode magnetron sputtering apparatus equipped with superconducting permanent magnet to produce Mo/Si multi-layer films, which would potentially serve as a high-quality optical mirror at extreme ultraviolet (EUV) wavelength of 13.5 nm. The best deposition condition was searched by analyzing the structure of the inter-diffusion layer formed in the Mo/Si bi-layer film prepared under different deposition conditions. It was found that (1) Xe gas should be used as inert gas species, (2) its pressure is lower than 4 × 10−2 Pa, (3) a throw distance is longer than 250 mm and (4) discharge voltage around 2 kV. By making full use of these data, we synthesized Mo/Si multi-layer films and analyzed the structure and its effect on the reflectivity. The highest EUV-reflectivity so far obtained is 67% in the normal incident condition. 相似文献
80.