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281.
282.
Depletion-induced self-assembly is routinely used to separate plasmonic nanoparticles (NPs) of different shapes, but less often for its ability to create supercrystals (SCs) in suspension. Therefore, these plasmonic assemblies have not yet reached a high level of maturity and their in-depth characterization by a combination of in situ techniques is still very much needed. In this work, gold triangles (AuNTs) and silver nanorods (AgNRs) are assembled by depletion-induced self-assembly. Small Angle X-ray Scattering (SAXS) and scanning electron microscopy (SEM) analysis shows that the AuNTs and AgNRs form 3D and 2D hexagonal lattices in bulk, respectively. The colloidal crystals are also imaged by in situ Liquid-Cell Transmission Electron Microscopy. Under confinement, the affinity of the NPs for the liquid cell windows reduces their ability to stack perpendicularly to the membrane and lead to SCs with a lower dimensionality than their bulk counterparts. Moreover, extended beam irradiation leads to disassembly of the lattices, which is well described by a model accounting for the desorption kinetics highlighting the key role of the NP-membrane interaction in the structural properties of SCs in the liquid-cell. The results shed light on the reconfigurability of NP superlattices obtained by depletion-induced self-assembly, which can rearrange under confinement.  相似文献   
283.
Journal of Inorganic and Organometallic Polymers and Materials - A platinum(II) polyyne/diketopyrrolopyrole-containing polymer of two different chain lengths, P (short) and P’ (long chain),...  相似文献   
284.
This paper proposes an energy-harvesting-aware model that aims to assess the performances of wireless sensor networks. Our model uses generalized stochastic Petri nets to define a sensor–neighbors relationship abstraction. The novelty of the proposed formulation is taking into account several real-life considerations such as battery-over breakdowns, unavailability of neighbors, retrial attempts, and sleeping mechanism in a single model. We use TimeNet tool to simulate the network behavior in order to evaluate its performance throughout different formulas after it had reached its steady state. Finally, we present a case study featuring the different solar energy recovery capabilities of the vast Algerian territory. The aim is to show with the presented model how to determine the kind of resources to be acquired in order to cope with the sensor deployment project requirements. The proposed model allows us to ensure that the battery energy level of sensors deployed in Algiers province for example is almost equal to 80% for 100 messages per day and (1 min/2 min) for (awakening time/sleeping time) ratio.  相似文献   
285.
The design of car shapes requires a delicate balance between aesthetic and performance. While fluid simulation provides the means to evaluate the aerodynamic performance of a given shape, its computational cost hinders its usage during the early explorative phases of design, when aesthetic is decided upon. We present an interactive system to assist designers in creating aerodynamic car profiles. Our system relies on a neural surrogate model to predict fluid flow around car shapes, providing fluid visualization and shape optimization feedback to designers as soon as they sketch a car profile. Compared to prior work that focused on time-averaged fluid flows, we describe how to train our model on instantaneous, synchronized observations extracted from multiple pre-computed simulations, such that we can visualize and optimize for dynamic flow features, such as vortices. Furthermore, we architectured our model to support gradient-based shape optimization within a learned latent space of car profiles. In addition to regularizing the optimization process, this latent space and an associated encoder-decoder allows us to input and output car profiles in a bitmap form, without any explicit parameterization of the car boundary. Finally, we designed our model to support pointwise queries of fluid properties around car shapes, allowing us to adapt computational cost to application needs. As an illustration, we only query our model along streamlines for flow visualization, we query it in the vicinity of the car for drag optimization, and we query it behind the car for vortex attenuation.  相似文献   
286.
The design of infrared nanocrystals-based (NCs) photodiodes faces a major challenge related to the identification of barriers with a well-suited band alignment or strategy to finely control the carrier density. Here, this study explores a general complementary approach where the carrier density control is achieved by coupling an NC layer to a ferroelectric material. The up-and-down change in ferroelectric polarization directly impacts the NC electronic structure, resulting in the formation of a lateral pn junction. This effect is uncovered directly using nano X-ray photoemission spectroscopy, which shows a relative energy shift of 115 meV of the NC photoemission signal over the two different up- and down-polarized ferroelectric regions, a shift as large as the open circuit value obtained in the diode stack. The performance of this pn junction reveals enhanced responsivity and reduced noise that lead to a factor 40 increase in the detectivity value.  相似文献   
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