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21.
G Kokotos V Theodorou V Constantinou-Kokotou WA Gibbons C Roussakis 《Canadian Metallurgical Quarterly》1998,8(12):1525-1530
A number of lipophilic platinum(II) complexes of the general structures cis-[Pt(LA)2Cl2] and [Pt(LD)Cl2] were synthesised. Long chain amines (LA) and diamines (LD), prepared from lipidic amino acids, were used as ligands. The in vitro cytotoxicity of the complexes was evaluated against four cell lines (P388, NSCLC-N6, E39, M96). cis-Dichloro-bis(2-aminohexadecanol)platinum(II) was the most active against P388, NSCLC-N6 and E39 (IC50: 11 micrograms/ml, 25 micrograms/ml, 31 micrograms/ml), while dichloro(1,3-heptadecanediamine)platinum(II) presented the highest activity against M96 (IC50: 13 micrograms/ml). 相似文献
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Eirini Anastasaki Fryni Drizou Panagiotis G. Milonas 《Journal of chemical ecology》2018,44(3):288-298
In response to attack by herbivorous insects, plants produce semiochemicals for intra- and interspecific communication. The perception of these semiochemicals by conspecifics of the herbivore defines their choice for oviposition and feeding. We aimed to investigate the role of herbivore-induced plant volatiles (HIPVs) by Tuta absoluta larvae on the oviposition choice of conspecific females on tomato plants. We performed two- choice and non-choice bioassays with plants damaged by larvae feeding and intact control plants. We also collected headspace volatiles of those plants and tested the response of female antennae on those blends with Gas Chromatography- Electro-Antennographical Detection (GC-EAD). In total 55 compounds were collected from the headspace of T. absoluta larvae-infested plants. Our results show that female moths preferred to oviposit on intact control plants instead of damaged ones. Herbivory induced the emission of hexanal, (Ζ)-3-hexen-1-ol, (E)-β-ocimene, linalool, (Z)-3-hexenyl butanoate, methyl salicylate, indole, nerolidol, guaidiene-6,9, β-pinene, β-myrcene, α-terpinene, hexenyl hexanoate, β-elemene, β-caryophyllene and (Ε-Ε)- 4,8,12-trimethyl-1,3,7,11-tridecatetraene (TMTT), one unidentified sesquiterpene and three unknown compounds. In Electroantennographic (EAG) assays, the antennae of T. absoluta females responded to hexanal, (Ζ)-3-hexen-1-ol, methyl salicylate and indole. The antennae of T. absoluta females exhibited a dose-response in EAG studies with authentic samples. Strong EAG responses were obtained for compounds induced on damaged tomato plants, as well as in nonanal, a compound emitted by both infested and control plants. These compounds could be utilized in integrated pest management of T. absoluta. 相似文献
24.
Interesting pattern mining in multi-relational data 总被引:1,自引:1,他引:0
Mining patterns from multi-relational data is a problem attracting increasing interest within the data mining community. Traditional data mining approaches are typically developed for single-table databases, and are not directly applicable to multi-relational data. Nevertheless, multi-relational data is a more truthful and therefore often also a more powerful representation of reality. Mining patterns of a suitably expressive syntax directly from this representation, is thus a research problem of great importance. In this paper we introduce a novel approach to mining patterns in multi-relational data. We propose a new syntax for multi-relational patterns as complete connected subsets of database entities. We show how this pattern syntax is generally applicable to multi-relational data, while it reduces to well-known tiles “ Geerts et al. (Proceedings of Discovery Science, pp 278–289, 2004)” when the data is a simple binary or attribute-value table. We propose RMiner, a simple yet practically efficient divide and conquer algorithm to mine such patterns which is an instantiation of an algorithmic framework for efficiently enumerating all fixed points of a suitable closure operator “Boley et al. (Theor Comput Sci 411(3):691–700, 2010)”. We show how the interestingness of patterns of the proposed syntax can conveniently be quantified using a general framework for quantifying subjective interestingness of patterns “De Bie (Data Min Knowl Discov 23(3):407–446, 2011b)”. Finally, we illustrate the usefulness and the general applicability of our approach by discussing results on real-world and synthetic databases. 相似文献
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K. Polychronopoulou C. Rebholz M.A. Baker L. Theodorou N.G. Demas S.J. Hinder A.A. Polycarpou C.C. Doumanidis K. Böbel 《Diamond and Related Materials》2008,17(12):2054-2061
This study describes the correlation between microstructure, mechanical and tribological properties of TiCx coatings (with x being in the range of 0–1.4), deposited by reactive magnetron sputtering from a Ti target in Ar/C2H2 mixtures at ~ 200 °C. The mechanical and tribological properties were found to strongly depend on the chemical composition and the microstructure present. Very dense structures and high hardness, combined with low wear rates and friction coefficients, were observed for coatings with chemical composition close to TiC. X-ray diffraction and X-ray photoelectron spectroscopy analysis, used to evaluate coating microstructure, composition and relative phase fraction, showed that low carbon contents in the coatings lead to sub-stoichiometric nanocrystalline TiCx coatings being deposited, whilst higher carbon contents gave rise to dual phase nanocomposite coatings consisting of stoichiometric TiC nanocrystallites and free amorphous carbon. Optimum performance was observed for nanocomposite TiC1.1 coatings, comprised of nanocrystalline nc-TiC (with an average grain size of ~ 15 nm) separated by 2–3 monolayers of an amorphous a-DLC matrix phase. 相似文献
27.
Maximilian L. Eggersdorfer Eirini Goudeli 《American Institute of Chemical Engineers》2020,66(12):e17099
The growth of silica nanoparticles by agglomeration and viscous flow sintering is studied from free molecular to transition regime by off-lattice event-driven (ED) simulations. Coagulation by simultaneous agglomeration and sintering takes place at high temperature environments, where sintering and collision rates are comparable. The effect of temperature on aggregate mobility and gyration radii, particle morphology, and collisional enhancement is elucidated. The ratio between the characteristic sintering time and characteristic collision time controls the particle size and structure, quantified by the mass fractal dimension. The aggregate morphology depends solely on the ratio of characteristic times and is insensitive to the process temperature. When sintering is negligible, the overall collision frequency is 90% larger than that predicted by the classic Fuchs collision kernel for monodisperse agglomerates, in agreement with experiments. The ED-obtained quasi-self-preserving size distributions are consistent with mobility size distributions measured in hot-wall reactors and flame sprays. 相似文献
28.
Konstantinos Skobridis Prof. Maria Kinigopoulou Vassiliki Theodorou Prof. Emilia Giannousi Alison Russell Rakhee Chauhan Roberta Sala Nicola Brownlow Dr. Serafim Kiriakidis Dr. Jan Domin Dr. Andreas G. Tzakos Dr. Nick J. Dibb Dr. 《ChemMedChem》2010,5(1):130-139
Imatinib is a clinically important ATP analogue inhibitor that targets the tyrosine kinase domain of the intracellular Abl kinase and the PDGF receptor family. Imatinib has revolutionised the treatment of chronic myeloid leukaemia, which is caused by the oncogene Bcr–Abl and certain solid tumours that harbor oncogenic mutations of the PDGF receptor family. As a leading kinase inhibitor, imatinib also provides an excellent model system to investigate how changes in drug design impact biological activity, which is an important consideration for rational drug design. Herein we report a new series of imatinib derivatives that in general have greater activity against the family of PDGF receptors and poorer activity against Abl, as a result of modifications of the phenyl and N‐methylpiperazine rings. These new compounds provide a platform for further drug development against the therapeutically important PDGF receptor family and they also provide insight into the engineering of drugs with altered biological activity. 相似文献
29.
Athanasios K. Morozinis Christos Tzoumanekas Stefanos D. Anogiannakis Doros N. Theodorou 《Polymer Science Series C》2013,55(1):212-218
A molecular-level understanding of cavitation in polymer networks upon imposition of mechanical stress is still lacking. Molecular Dynamics simulations of crosslinked amorphous Polyethylene (PE) were conducted in order to study cavitation as a function of the prevailing stress. We first show that the characteristic relaxation times related to tube confinement and chain connectivity can be obtained by examining the mean square displacement of middle chain monomers. Then, we present a methodology for predicting the cavitation strength and understanding its dependence on cohesive interactions and entropic elasticity. Our simulations show that experimental observations and predictions of continuum mechanics analysis, which relate the critical stress for cavitation to the Young’s modulus of the rubber, are in agreement with the observed tensile triaxial stress below which a pre-existing cavity cannot survive in a cavitated sample. 相似文献
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