全文获取类型
收费全文 | 170篇 |
免费 | 14篇 |
专业分类
电工技术 | 3篇 |
化学工业 | 70篇 |
金属工艺 | 1篇 |
建筑科学 | 8篇 |
能源动力 | 3篇 |
轻工业 | 32篇 |
水利工程 | 2篇 |
无线电 | 11篇 |
一般工业技术 | 15篇 |
冶金工业 | 20篇 |
原子能技术 | 2篇 |
自动化技术 | 17篇 |
出版年
2023年 | 5篇 |
2022年 | 5篇 |
2021年 | 13篇 |
2020年 | 7篇 |
2019年 | 5篇 |
2018年 | 2篇 |
2017年 | 6篇 |
2016年 | 11篇 |
2015年 | 5篇 |
2014年 | 6篇 |
2013年 | 7篇 |
2012年 | 5篇 |
2011年 | 15篇 |
2010年 | 13篇 |
2009年 | 12篇 |
2008年 | 9篇 |
2007年 | 5篇 |
2006年 | 13篇 |
2005年 | 7篇 |
2004年 | 4篇 |
2003年 | 5篇 |
2002年 | 4篇 |
2001年 | 2篇 |
2000年 | 3篇 |
1999年 | 1篇 |
1997年 | 2篇 |
1996年 | 1篇 |
1994年 | 1篇 |
1993年 | 2篇 |
1992年 | 3篇 |
1989年 | 2篇 |
1986年 | 1篇 |
1976年 | 2篇 |
排序方式: 共有184条查询结果,搜索用时 578 毫秒
21.
Rancière F Dassonville C Roda C Laurent AM Le Moullec Y Momas I 《The Science of the total environment》2011,409(20):4480-4483
Indoor aldehydes may result from ozone-initiated chemistry, mainly documented by experimental studies. As part of an environmental investigation included in the PARIS birth cohort, the aim of this study was to examine ozone contribution to airborne aldehyde formation in Paris homes. Formaldehyde, acetaldehyde and hexaldehyde levels, as well as styrene, nitrogen dioxide and nicotine concentrations, comfort parameters and carbon dioxide levels, were measured twice during the first year of life of the babies. Ambient ozone concentrations were collected from the closest background station of the regional air monitoring network. Traffic-related nitrogen oxide concentrations in front of the dwellings were estimated by an air pollution dispersion model. Home characteristics and families' way of life were described by questionnaires. Stepwise multiple linear regression models were used to link aldehyde levels with ambient ozone concentrations and a few aldehyde precursors involved in oxidation reactions, adjusting for other indoor aldehyde sources, comfort parameters and traffic-related nitrogen oxides. A 4 and 11% increase in formaldehyde and hexaldehyde levels was pointed out when 8-hour ozone concentrations increased by 20 μg/m3. The influence of potential precursors such as indoor styrene level and frequent use of air fresheners, containing unsaturated volatile organic compounds as terpenes, was also found. Thus, our results suggest that ambient ozone can significantly impact indoor air quality, especially with regard to formaldehyde and hexaldehyde levels. 相似文献
22.
Due to their nutrient recycling function and their importance in food-webs, macroinvertebrates are essential for the functioning of aquatic ecosystems. These organisms also constitute an important component of biodiversity.Sediment evaluation and monitoring is an essential aspect of ecosystem monitoring since sediments represent an important component of aquatic habitats and are also a potential source of contamination. In this study, we focused on macroinvertebrate communities within run-of-river dams, that are prime areas for sediment and pollutant accumulation. Little is known about littoral macroinvertebrate communities within run-of-river dam or their response to sediment levels and pollution. We therefore aimed to evaluate the following aspects: the functional and structural composition of macroinvertebrate communities in run-of-river dams; the impact of pollutant accumulation on such communities, and the most efficient scales and tools needed for the biomonitoring of contaminated sediments in such environments. Two run-of-river dams located in the French alpine area were selected and three spatial scales were examined: transversal (banks and channel), transversal × longitudinal (banks/channel × tail/middle/dam) and patch scale (erosion, sedimentation and vegetation habitats). At the patch scale, we noted that the heterogeneity of littoral habitats provided many available niches that allow for the development of diversified macroinvertebrate communities. This implies highly variable responses to contamination. Once combined on a global ‘banks’ spatial scale, littoral habitats can highlight the effects of toxic disturbances. 相似文献
23.
24.
Isabelle Déléris Anne Saint-Eve Fanny Dakowski Etienne Sémon Jean-Luc Le Quéré Hervé Guillemin Isabelle Souchon 《Food chemistry》2011
We investigated the role of both candy texture and eating technique (melting or chewing) on the dynamics of aroma release. One novelty of this type of analysis was the simultaneous application of instrumental and sensory analysis. Four candy textures were established based on their storage modulus at 1 Hz by varying the gelatine content between 0 and 15% w/w. The invivo release of three aroma compounds was monitored using Proton Transfer Reaction Mass Spectrometry and with a trained panel of testers. The gelatine content had no significant effect on the headspace/product partition and diffusion properties of the aroma compounds. The highest invivo release for all aroma compounds was obtained with the 2% gelatine sample. Our findings indicated that aroma release was determined by interaction between the product properties and oral behaviour. Relations between the dynamics of release and perception (method of Temporal Dominance of Sensations) have been established on temporal parameters. 相似文献
25.
Saint Martin Marie-Judith Orlhac Fanny Akl Pia Khalid Fahad Nioche Christophe Buvat Irène Malhaire Caroline Frouin Frédérique 《Magma (New York, N.Y.)》2021,34(3):355-366
Magnetic Resonance Materials in Physics, Biology and Medicine - Quantitative analysis in MRI is challenging due to variabilities in intensity distributions across patients, acquisitions and... 相似文献
26.
27.
Ballihaut G Claverie F Pécheyran C Mounicou S Grimaud R Lobinski R 《Analytical chemistry》2007,79(17):6874-6880
A laser ablation-ICPMS method using an infrared (1030 nm), low-energy (39 microJ/pulse), high repetition rate (10 kHz), femtosecond laser was developed to improve the sensitivity of detection of heteroatom-containing proteins in 1D polyacrylamide gels. A 2-mm-wide lane was ablated by ultrafast (10 cm s(-1)) back-and-forth movement of a 20-microm laser beam parallel to the protein bands while the gel advanced perpendicularly. This procedure resulted in a considerable increase in detection sensitivity (>40-fold) compared to the nanosecond 266-nm laser ablation-ICPMS, mainly because of the much larger amount of ablated material introduced into the plasma on the time scale of the dwell time of the mass spectrometer. The method was applied to the specific detection in the gel of formate dehydrogenase expressed in Escherichia coli and of selenoproteins in Desulfococcus multivorans with detection limits at the low-femtomolar levels. 相似文献
28.
Naveau A Monteil-Rivera F Guillon E Dumonceau J 《Environmental science & technology》2007,41(15):5376-5382
The present study was initiated to determine the capacity of sulfide minerals (pyrite FeS2 and chalcopyrite CuFeS2) to delay the migration of inorganic selenium species in geological formations. Interactions between Se(IV) and Se(-II) and synthetic and natural sulfide minerals were investigated under anoxic conditions using the batch method. Significant sorption of selenium occurred under acidic conditions. Analysis of the solids after Se sorption using X-ray photoelectron spectroscopy (XPS) and X-ray absorption near edge structure (XANES) demonstrated the presence of reduced selenium species on the metallic sulfide surfaces, thus suggesting an oxido-reduction process coupled with sorption. Selenium reduction occurred concomitantly with the oxidation of pyritic sulfur, whereas metallic species (Fe, Cu) were not involved in the redox process. Formation of ferroselite (FeSe2) was postulated to take place on the synthetic solid while surface complexation or ionic exchange processes were more likely on the natural solids. 相似文献
29.
Boccard M Battaglia C Hänni S Söderström K Escarré J Nicolay S Meillaud F Despeisse M Ballif C 《Nano letters》2012,12(3):1344-1348
The challenge for all photovoltaic technologies is to maximize light absorption, to convert photons with minimal losses into electric charges, and to efficiently extract them to the electrical circuit. For thin-film solar cells, all these tasks rely heavily on the transparent front electrode. Here we present a multiscale electrode architecture that allows us to achieve efficiencies as high as 14.1% with a thin-film silicon tandem solar cell employing only 3 μm of silicon. Our approach combines the versatility of nanoimprint lithography, the unusually high carrier mobility of hydrogenated indium oxide (over 100 cm(2)/V/s), and the unequaled light-scattering properties of self-textured zinc oxide. A multiscale texture provides light trapping over a broad wavelength range while ensuring an optimum morphology for the growth of high-quality silicon layers. A conductive bilayer stack guarantees carrier extraction while minimizing parasitic absorption losses. The tunability accessible through such multiscale electrode architecture offers unprecedented possibilities to address the trade-off between cell optical and electrical performance. 相似文献
30.
Stability of Betacyanin Pigments and Antioxidants in Ayrampo (Opuntia soehrensii Britton and Rose) Seed Extracts and as a Yogurt Natural Colorant 下载免费PDF全文