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11.
Summary Poly(propylene oxide), PPO, obtained using diphenylzinc, Ph2Zn, and using the diphenylzinc-water system at various molar ratios H2O/Ph2Zn, were studied through 1H NMR and IR spectroscopy establishing that the polymerization initiates by coordition of propylene oxide (PO) to a terminal zinc atom of the active species followed by consecutive insertions of PO units at this zinc atom. The PPO obtained showed Ph-and HO-, HO-and HO-end-groups depending on the molar ratio H2O/Ph2Zn used, and also HO-and PhO-end-groups when oxygen was present in the polymerization system. 相似文献
12.
The Steady radial distribution of chemical species in a wire‐to‐cylinder ozone generator filled with pure oxygen has been computed by applying four different plasma chemistry models of increasing complexity. The most complete model considers ten species (e, O2 +, O2 ?, O3 ?, O?, O2, O2(1Δg), O2(1∑g +), O and O3) and 79 reactions, including ionization by electron impact, electron attachment and detachment, electron-ion recombination, charge transfer, etc. The chemical model is coupled with the electrical model through Poisson's equation. The spatially averaged ozone density has been computed as a function of the current intensity and compared with the experimental values obtained by UV spectroscopy. 相似文献
13.
Edna R Meza‐Escalante Anne‐Claire Texier Flor Cuervo‐López Jorge Gómez Francisco J Cervantes 《Journal of chemical technology and biotechnology (Oxford, Oxfordshire : 1986)》2008,83(3):372-377
BACKGROUND: Many industrial discharges, such as those generated from petrochemical refineries, contain large amounts of sulfurous, nitrogenous and organic contaminants. Denitrification has emerged as a suitable technology for the simultaneous removal of these pollutants in a single reactor unit; however, more evidence is demanded to clarify the limitations of denitrification on the simultaneous removal of sulfide and phenolic contaminants and to optimize the biological process. The aim of this study was to evaluate the capacity of a denitrifying sludge to simultaneously convert sulfide and p‐cresol via denitrification. RESULTS: Sulfide was the preferred electron donor over p‐cresol, imposing a 5 h lag phase (required for complete sulfide removal) on organotrophic denitrification. Addition of sulfide (20 mg S2? L?1) to p‐cresol‐amended denitrifying cultures also decreased the reduction rate of nitrate and nitrite, as well as the production rate of nitrogen gas. Nitrite reduction rate was the most affected step by sulfide, decreasing from 35 to 21 mg N (g VSS d)?1. A synergistic inhibitory effect of nitrate and sulfide was also observed on nitrite reduction. Despite the effects of sulfide on the respiratory rates monitored, complete removal of nitrate, sulfide and p‐cresol could be achieved after 48 h of incubation. CONCLUSION: Our results suggest that simultaneous removal of sulfide and p‐cresol could be achieved in denitrifying reactors, but a large hydraulic residence time may be required to sustain an efficient process due to inhibitory effects of sulfide. Copyright © 2008 Society of Chemical Industry 相似文献
14.
Simon P. Wilson Francisco J. Samaniego 《IEEE transactions on pattern analysis and machine intelligence》2007,33(3):198-208
In the literature on statistical inference in software reliability, the assumptions of parametric models and random sampling of bugs have been pervasive. We argue that both assumptions are problematic, the first because of robustness concerns and the second due to logical and practical difficulties. These considerations motivate the approach taken in this paper. We propose a nonparametric software reliability model based on the order-statistic paradigm. The objective of the work is to estimate, from data on discovery times observed within a type I censoring framework, both the underlying distribution F from which discovery times are generated and N, the unknown number of bugs in the software. The estimates are used to predict the next time to failure. The approach makes use of Bayesian nonparametric inference methods, in particular, the beta-Stacy process. The proposed methodology is illustrated on both real and simulated data 相似文献
15.
Montserrat Bóo Francisco Argüello Javier D. Bruguera Emilio L. Zapata 《The Journal of VLSI Signal Processing》1997,17(1):57-73
A rate 1/n binary generic convolutional encoder is a shift-register circuit where the inputs are information bits and the outputs are blocks of n bits generated as linear combinations on the appropriate shift register contents. The decoding of the outputs of a convolutional encoder can be carried out by the well-known Viterbi algorithm. The communication pattern of the Viterbi Algorithm is given as a graph, called trellis, associated to the state diagram of the corresponding encoder. In this paper we present a methodology that permits the efficient mapping of the Viterbi algorithm onto a column of an arbitrary number of processors. This is done through the representation of the data flow by using mathematical operators which present an inmediate hardware projection. A single operator string has been obtained to represent a generic encoder through the study of the data flow of free-forward encoders and feed-back encoders. The formal model developed is employed for the partitioning of the computations among an arbitrary number of processors in such a way that the data are recirculated opimizing the use of the processors and the communications. As a result, we obtain a highly regular and modular architecture suitable for VLSI implementation. 相似文献
16.
Participating media with an inhomogeneous index of refraction make light follow curved paths. Simulating this in a global
illumination environment has usually been neglected due to the complexity of the calculations involved, sacrificing accurate
physical simulations for efficient visual results.
This paper aims to simulate non-linear media in a more reasonable time than previous works without losing physical correctness.
Accuracy is achieved by solving the Eikonal equation of geometrical optics, which describes the path followed by a light beam
that traverses a non-linear medium. This equation is used in the context of a photon mapping extension. 相似文献
17.
Nowadays, cities are the most relevant type of human settlement and their population has been endlessly growing for decades. At the same time, we are witnessing an explosion of digital data that capture many different aspects and details of city life. This allows detecting human mobility patterns in urban areas with more detail than ever before. In this context, based on the fusion of mobility data from different and heterogeneous sources, such as public transport, transport‐network connectivity and Online Social Networks, this study puts forward a novel approach to uncover the actual land use of a city. Unlike previous solutions, our work avoids a time‐invariant approach and it considers the temporal factor based on the assumption that urban areas are not used by citizens all the time in the same manner. We have tested our solution in two different cities showing high accuracy rates. 相似文献
18.
Quesada-Barriuso Pablo Blanco Heras Dora Argüello Francisco 《The Journal of supercomputing》2021,77(9):10040-10052
The Journal of Supercomputing - The high computational cost of the superpixel segmentation algorithms for hyperspectral remote sensing images makes them ideal candidates for parallel computation.... 相似文献
19.
Moutafis Panagiotis García-García Francisco Mavrommatis George Vassilakopoulos Michael Corral Antonio Iribarne Luis 《Distributed and Parallel Databases》2021,39(3):733-784
Distributed and Parallel Databases - Given two datasets of points (called Query and Training), the Group (K) Nearest-Neighbor (GKNN) query retrieves (K) points of the Training with the smallest sum... 相似文献
20.
Julián Luengo José A. Sáez Francisco Herrera 《Soft Computing - A Fusion of Foundations, Methodologies and Applications》2012,16(5):863-881
Fuzzy rule-based classification systems (FRBCSs) are known due to their ability to treat with low quality data and obtain
good results in these scenarios. However, their application in problems with missing data are uncommon while in real-life
data, information is frequently incomplete in data mining, caused by the presence of missing values in attributes. Several
schemes have been studied to overcome the drawbacks produced by missing values in data mining tasks; one of the most well
known is based on preprocessing, formerly known as imputation. In this work, we focus on FRBCSs considering 14 different approaches
to missing attribute values treatment that are presented and analyzed. The analysis involves three different methods, in which
we distinguish between Mamdani and TSK models. From the obtained results, the convenience of using imputation methods for
FRBCSs with missing values is stated. The analysis suggests that each type behaves differently while the use of determined
missing values imputation methods could improve the accuracy obtained for these methods. Thus, the use of particular imputation
methods conditioned to the type of FRBCSs is required. 相似文献