全文获取类型
收费全文 | 2278篇 |
免费 | 75篇 |
国内免费 | 8篇 |
专业分类
电工技术 | 119篇 |
综合类 | 4篇 |
化学工业 | 599篇 |
金属工艺 | 56篇 |
机械仪表 | 52篇 |
建筑科学 | 49篇 |
矿业工程 | 4篇 |
能源动力 | 121篇 |
轻工业 | 193篇 |
水利工程 | 6篇 |
武器工业 | 1篇 |
无线电 | 192篇 |
一般工业技术 | 380篇 |
冶金工业 | 345篇 |
原子能技术 | 72篇 |
自动化技术 | 168篇 |
出版年
2023年 | 8篇 |
2022年 | 21篇 |
2021年 | 42篇 |
2020年 | 16篇 |
2019年 | 30篇 |
2018年 | 39篇 |
2017年 | 32篇 |
2016年 | 44篇 |
2015年 | 33篇 |
2014年 | 41篇 |
2013年 | 121篇 |
2012年 | 80篇 |
2011年 | 130篇 |
2010年 | 86篇 |
2009年 | 110篇 |
2008年 | 106篇 |
2007年 | 114篇 |
2006年 | 102篇 |
2005年 | 92篇 |
2004年 | 88篇 |
2003年 | 86篇 |
2002年 | 66篇 |
2001年 | 52篇 |
2000年 | 54篇 |
1999年 | 46篇 |
1998年 | 138篇 |
1997年 | 79篇 |
1996年 | 61篇 |
1995年 | 51篇 |
1994年 | 58篇 |
1993年 | 49篇 |
1992年 | 40篇 |
1991年 | 26篇 |
1990年 | 16篇 |
1989年 | 27篇 |
1988年 | 21篇 |
1987年 | 12篇 |
1986年 | 11篇 |
1985年 | 15篇 |
1984年 | 8篇 |
1983年 | 15篇 |
1982年 | 14篇 |
1981年 | 10篇 |
1980年 | 11篇 |
1979年 | 12篇 |
1977年 | 9篇 |
1976年 | 11篇 |
1974年 | 4篇 |
1971年 | 5篇 |
1970年 | 4篇 |
排序方式: 共有2361条查询结果,搜索用时 187 毫秒
101.
Sang-Kyu Shin Jeong-Eun Sim Hideki Kishimura Byung-Soo Chun 《Journal of Industrial and Engineering Chemistry》2012,18(1):546-550
Ethanolysis of menhaden oil was performed with 1,3-regiospecific lipase to produce diglycerides and monoglycerides containing polyunsaturated fatty acids, and fatty acid ethyl esters. Immobilized lipases like lipozyme TL-IM (Thermomuces lanuginosa immobilized on silica gel) were used for enzymatic ethanolysis. Ethanolysis was carried out in different processes (solvent free, organic solvent and supercritical fluid system) to compare the reaction rate and yield obtained by menhaden oil ethanolysis. Organic solvent (hexane) and supercritical carbon dioxide (SC-CO2) were used as reaction medium. The reaction products were analyzed by gas chromatography (GC), thin layer chromatography (TLC) and high performance liquid chromatography (HPLC). Higher amounts of ethanol as a substrate caused substrate inhibition which dramatically decreased the reaction rate of ethanolysis. To elucidate the effect of pressure, enzymatic ethanolysis was performed in SC-CO2 at pressures ranging from 75 to 121 bar. Enzymatic ethanolysis of menhaden oil in SC-CO2 decreased by substrate inhibition. Reaction rate and optimum amount of ethanol used were depended on SC-CO2 density individually. Kinetic model with substrate inhibition (dead-end inhibition) by excess ethanol was set up to measure the reaction and inhibition rates. 相似文献
102.
Miwa N Kashiwagi M Kawamori F Masuda T Sano Y Hiroi M Kurashige H 《Shokuhin eiseigaku zasshi. Journal of the Food Hygienic Society of Japan》2006,47(2):41-45
The incidence and levels of Vibrio parahaemolyticus and thermostable direct hemolysin gene (tdh)-positive organisms in retail seafood were determined. The most probable number-polymerase chain reaction (MPN-PCR) method using a PCR procedure targeting the species-specific thermolabile hemolysin gene (tlh) and tdh was used to determine the levels of V. parahaemolyticus and tdh-positive organisms, respectively. In seafood for raw consumption, V. parahaemolyticus was found in four (13.3%) of 30 fish samples, 11 (55.0%) of 20 crustacean samples, and 29 (96.7%) of 30 mollusc samples. Levels of V. parahaemolyticus were below 10(4) MPN/100 g in all fish and crustacean samples tested. However, they were above 10(4) MPN/100 g in 11 (36.7%) of the 30 mollusc samples. In all seafood for raw consumption, the level of tdh-positive organisms was below the limit of detection (< 30 MPN/100 g). In seafood for cooking, V. parahaemolyticus was found in 15 (75.0%) of 20 fish samples, nine (45.0%) of 20 crustacean sample, and 20 (100%) of 20 mollusc samples. Levels of V. parahaemolyticus were above 10(4) MPN/100 g in only three (15.0%) and one (5.0%) of the 20 fish and 20 crustacean samples, respectively. However, they were above 10(4) MPN/100 g in 18 (90.0%) of the 20 mollusc samples. In seven (35.0%) of the 20 mollusc samples, tdh-positive organisms were found and their levels ranged from 3.6x10 to 1.1 x 103 MPN/100 g. From four of seven tdhpositive samples, tdh-positive V. parahaemolyticus was isolated. 相似文献
103.
We present a new theory for photogenerated carrier escape rates from single quantum wells, as a function of an applied electric field, that includes thermionic emission, direct tunneling, and tunneling via thermal occupation of upper subbands, and compare the results for GaAs/AlxGa1-xAs quantum wells with recent experiments. We account for the two dimensional (2D) density of states below the barrier, assume thermal equilibrium of carriers within the well, allow for the possibility of strain in the well and/or barrier, and include the contribution to electron thermionic emission from indirect conduction band minima. Our expressions for thermionic emission reduce, in the limit of large well width, to those derived by assuming a three-dimensional (3D) density of states. The results for electron emission from GaAs/AlxGa1-xAs quantum wells with x=0.2 and x=0.4 barriers at room temperature agree well with experiment. For wells with x=0.2 barriers, thermally assisted tunneling overtakes thermionic emission around 40 kV/cm, while for wells with x=0.4 barriers thermionic emission from the L valley conduction band minima dominates for fields less than 70 kV/cm. For holes we show that the escape rates are very sensitive to the in-plane effective masses, and results using simple expressions for the in-plane masses that do not include light/heavy-hole mixing agree poorly with experiment. The agreement with experiment is improved using in-plane masses that include light/heavy-hole mixing, particularly for wells with high barriers. We suggest that agreement with experiment would be improved by using more accurate in-plane hole masses for all of the subbands 相似文献
104.
Tetsuya OGAWA Hideki ISHIDA Nami MATSUDA Ayuko FUJIU Akiko MATSUDA Kyoko ITO Yoshitaka ANDO Kosaku NITTA 《Hemodialysis international. International Symposium on Home Hemodialysis》2009,13(3):301-306
Vascular calcification is associated with a poor prognosis in dialysis patients. It can be assessed with computed tomography but simple inoffice techniques may provide useful information. We compared the results obtained with a simple noninvasive technique with those obtained using multidetector computed tomography for aortic arch calcification volume (AoACV) in chronic hemodialysis (HD) patients. The enrolled study subjects were 63 (32 men and 31 women) maintenance HD patients. Calcification of the aortic arch was semiquantitatively estimated with a AoAC score (AoACS) on plain chest radiology. The AoACV was increased, with a mean value of 6.6 ranging from 0% to 36.5%. The coefficient of intraobserver variation was less than 2.5%. Aortic arch calcification score was highly correlated with AoACV (r=0.635, P<0.001). Multiple regression analysis showed age (F value=12.62, P<0.001) and pulse pressure (F value=4.54, P=0.037) to be significant independent determinants of AoACS. In conclusion, a simple measurement of AoACS may be useful for inoffice imaging to choose a therapeutic regimen in HD patients. 相似文献
105.
Rubber‐toughened polyamide‐6 with a low thermal expansion coefficient: effect of preferential distribution of rubber and inorganic filler
下载免费PDF全文
![点击此处可从《Polymer International》网站下载免费的PDF全文](/ch/ext_images/free.gif)
Guozhang Wu Kun Zhang Kiyoji Takagi Hironari Sano Hiroshi Yui 《Polymer International》2016,65(1):102-108
The effects of morphological changes on the thermal expansion, toughness and heat resistance of polyamide‐6 (PA)/styrene–ethylene–butylene–styrene (SEBS)/polyphenylene ether (PPE) blends were investigated. Compared with the typical ‘sea (PA matrix)–island (PPE domain)–lake (SEBS in PPE domain)’ morphology, an injection‐molded ternary blend with a preferential distribution of SEBS component at the interface between PA and PPE exhibited a low coefficient of linear thermal expansion (CLTE) in the flow direction. This low CLTE was ascribed to the deformation of SEBS and PA into a co‐continuous microlayer network structure during injection molding. Consequently, the expansion preferentially occurred towards the thickness direction. Further CLTE reduction either by a change in PA viscosity or by the selective location of an inorganic filler was examined, and its influences on impact strength and heat resistance are discussed based on transmission electron microscopy observations. © 2015 Society of Chemical Industry 相似文献
106.
Wubian Tian Hideki Kita Hideki Hyuga Naoki Kondo Takaaki Nagaoka 《Journal of the European Ceramic Society》2010,30(15):3203-3208
SiC ceramics were reaction joined in the temperature range of 1450–1800 °C using TiB2-based composites starting from four types of joining materials, namely Ti–BN, Ti–B4C, Ti–BN–Al and Ti–B4C–Si. XRD analysis and microstructure examination were carried out on SiC joints. It is found that the former two joining materials do not yield good bond for SiC ceramics at temperatures up to 1600 °C. However, Ti–BN–Al system results in the connection of SiC substrates at 1450 °C by the formation of TiB2–AlN composite. Furthermore, nearly dense SiC joints with crack-free interface have been produced from Ti–BN–Al and Ti–B4C–Si systems at 1800 °C, i.e. joints TBNA80 and TBCS80, whose average bending strengths are measured to be 65 MPa and 142 MPa, respectively. The joining mechanisms involved are also discussed. 相似文献
107.
Estimation of Small Reservoir Storage Capacities with Remote Sensing in the Brazilian Savannah Region 总被引:2,自引:0,他引:2
Lineu N. Rodrigues Edson E. Sano Tammo S. Steenhuis Denílson P. Passo 《Water Resources Management》2012,26(4):873-882
Small reservoirs play an important role in supporting the local economy in the savannah areas of Brazil and are primarily
used for the provision of water for irrigation and watering livestock. Hundreds of small reservoirs have been built in the
last few decades in the Preto River Basin, but efficient water management and sound planning are hindered by inadequate knowledge
of the number, storage capacity and spatial distribution of reservoirs in the basin. The main reason for the lack of this
information is that current methodologies for quantifying the physical parameters of reservoirs are laborious, time consuming
and costly. To address this lack of data, a simple method to estimate reservoir storage volumes based on remotely sensed reservoir
surface area measured with LANDSAT was developed. The method was validated with a subset of reservoirs in the Preto River
Basin for which surface areas, shapes and depths were determined with ground-based survey measurements. The agreement between
measured and the remotely sensed reservoir volumes was satisfactory, indicating that remotely-sensed images can be used for
improved management of water in the Brazilian Savannah region. With the newly developed methods we found that the Preto River
Basin’s 147 small reservoirs can store 19 × 106 m3 of water at full capacity. 相似文献
108.
By applying square wave AC voltage to the Au source electrode of tetracene based field-effect transistor (FET), electroluminescence (EL) was obtained. The results suggest that electrons and holes were injected alternately from the source electrode and recombined each other, and lead to the EL. This type of EL was localized at the interface between the source electrode and tetracene, and enhanced periodically with two relaxation times in accordance with the applied AC voltage cycle. We modeled the carrier behavior in the FET and explained the decay of EL, taking into account the space charge field contribution. Finally, using an AC voltage superposed on DC bias voltage, it was shown that electron injection was prompted only by space charge field. 相似文献
109.
Kikuo Matsui Hideki Shimada Takashi Sasaoka Hirofumi Furukawa Takeshi Ueda Atsuko Yabuki 《国际露天开采、回填与环境杂志》2013,27(3):185-204
Conventional highwall mining extracts coal with an auger machine or a continuous miner from exposed seams at the base of opencut or strip operations. However, under poor strata and high stress conditions, highwall mining cannot be conducted due to pillar and roof failures. In such cases, punch highwall mining is more effective than the conventional highwall mining. This paper describes conventional highwall mining and punch highwall mining systems and discusses the stability of the highwall due to punch highwall mining at opencut coal mines. 相似文献
110.
Hideki Tanaka Daisuke Noguchi Akiko Yuzawa Tetsuya Kodaira Hirofumi Kanoh Katsumi Kaneko 《Journal of Low Temperature Physics》2009,157(3-4):352-373
We have investigated the applicability of simulations and theoretical techniques for exploring the selectivities of hydrogen isotopes. We have simulated the adsorption isotherms of H2 in an idealized carbon slit pore at 77 K by using the grand canonical Monte Carlo simulations with the Feynman-Hibbs effective potential (FH-GCMC) and the rigorous path integral method (PI-GCMC), and we obtained good agreement between the isotherms from both simulations. This suggests that FH-GCMC, which uses the approximative Feynman-Hibbs treatment, is as useful as PI-GCMC for exploring H2 adsorption at 77 K. Moreover, we show that the ideal adsorption solution theory (IAST) can predict the selectivity of D2 over H2 in the interstices of single-wall carbon nanotube (SWNT) bundles at 77 K (below 0.1 MPa) very well by comparing the obtained results with the mixture adsorption FH-GCMC simulations. This indicates that IAST is also applicable to the estimation of the selectivity of D2 over H2 at moderate pressures and at 77 K from experimental single-component adsorption isotherms. We also demonstrate that the FH-GCMC simulation can reproduce the experimental adsorption isotherms of H2 and D2 in aluminophosphate AlPO4-5 at 77 K. Finally, we analyze the selectivity of D2 over H2 by IAST with the experimental single-component adsorption isotherms of H2 and D2 at 77 K for a variety of adsorbents: AlPO4-5, activated carbon fibers (ACFs), HiPco SWNT, and SWNHs. The selectivities predicted by the experimental adsorption data based on the results from the FH-GCMC simulations are presented and discussed. 相似文献