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31.
Rational Design and Synthesis of Extremely Efficient Macroporous CoSe2–CNT Composite Microspheres for Hydrogen Evolution Reaction 下载免费PDF全文
Jin Koo Kim Gi Dae Park Jung Hyun Kim Seung‐Keun Park Yun Chan Kang 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(27)
Uniquely structured CoSe2–carbon nanotube (CNT) composite microspheres with optimized morphology for the hydrogen‐evolution reaction (HER) are prepared by spray pyrolysis and subsequent selenization. The ultrafine CoSe2 nanocrystals uniformly decorate the entire macroporous CNT backbone in CoSe2–CNT composite microspheres. The macroporous CNT backbone strongly improves the electrocatalytic activity of CoSe2 by improving the electrical conductivity and minimizing the growth of CoSe2 nanocrystals during the synthesis process. In addition, the macroporous structure resulting from the CNT backbone improves the electrocatalytic activity of the CoSe2–CNT microspheres by increasing the removal rate of generated H2 and minimizing the polarization of the electrode during HER. The CoSe2–CNT composite microspheres demonstrate excellent catalytic activity for HER in an acidic medium (10 mA cm?2 at an overpotential of ≈174 mV). The bare CoSe2 powders exhibit moderate HER activity, with an overpotential of 226 mV at 10 mA cm?2. The Tafel slopes for the CoSe2–CNT composite and bare CoSe2 powders are 37.8 and 58.9 mV dec?1, respectively. The CoSe2–CNT composite microspheres have a slightly larger Tafel slope than that of commercial carbon‐supported platinum nanoparticles, which is 30.2 mV dec–1. 相似文献
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Enhancing Interfacial Bonding between Anisotropically Oriented Grains Using a Glue‐Nanofiller for Advanced Li‐Ion Battery Cathode 下载免费PDF全文
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Nanotransfer Printing: Inkjet‐Assisted Nanotransfer Printing for Large‐Scale Integrated Nanopatterns of Various Single‐Crystal Organic Materials (Adv. Mater. 15/2016) 下载免费PDF全文
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Seungae Lee Jahyun Koo Seung-Kyun Kang Gayoung Park Yung Jong Lee Yu-Yu Chen Seon Ah Lim Kyung-Mi Lee John A. Rogers 《Materials Today》2018,21(3):207-215
Biologically and environmentally resorbable electronic devices support application possibilities that cannot be addressed with conventional technologies. This paper presents highly conductive, water-soluble composites that can be printed to form contacts, interconnects, antennas, and other important features that are essential to nearly all systems of this type. An optimized material formulation involves in situ polymerization to yield a polyanhydride containing a dispersion of molybdenum microparticles at appropriate concentrations. Comparisons of essential physical and electrical properties of these materials to those of composites formed with other polymers and other metal microparticles reveal the relevant considerations. Various functional demonstrations of screen-printed test structures and devices illustrate the suitability of these conductive inks for use in water-soluble electronic devices. A key advantage of the material introduced here compared to alternatives is its ability to maintain conductance over significant periods of time while immersed in relevant aqueous solutions. Studies involving live animal models establish the biocompatibility. 相似文献
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Amplification‐Free Multi‐RNA‐Type Profiling for Cancer Risk Stratification via Alternating Current Electrohydrodynamic Nanomixing 下载免费PDF全文
Simultaneous analysis of messenger RNA (mRNA), microRNA (miRNA), and long noncoding RNA (lncRNA)—multi‐RNA‐type profiling—is increasingly crucial in cancer diagnostics. Yet, rapid multi‐RNA‐type profiling is challenging due to enzymatic amplification reliance and RNA‐type‐dependent characteristics. Here, a nanodevice is reported to uniquely use alterable alternating current electrohydrodynamic (ac‐EHD) forces to enhance probe–target hybridization prior to direct native RNA target detection, without target amplification or surface functionalization. To exemplify clinical applicability, noninvasive screening of next‐generation prostate cancer (PCa) RNA biomarkers (of different types) in patient urine samples is performed. A strong correlation between multi‐RNA‐type expression and aggressive PCa is found, and the nanodevice performance is statistically evaluated. It is believed that this miniaturized system exhibits great potential for cancer risk stratification via multi‐RNA‐type profiling. 相似文献
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Porter sites have tried to increase their business potentials by helping users easily engage in diverse online activities such as search, entertainment, online communities, and others. Knowledge search engine is one of the most successful killer applications increasing user loyalty. However, most studies have independently focused on search engine technology such as search keyword algorithm, presentation of information and user characteristics such as cognitive style, search experiences, and skill levels. However, these previous studies lack an integrated understanding of causal links among critical factors predicting user motives and intention involving more situation-specific user characteristics. To fill these gaps in the literature, the present study focuses on whether knowledge characteristics such as specialization, preciseness, and diversity, and system characteristics such as interactivity, responsiveness, and communication richness are important in forming user motives and intention. The present study also identifies a moderating role of epistemic curiosity in the links between motives and intention. Two hundred and fifty-five data from Korean university students confirmed that knowledge and services characteristics such as specialty, preciseness, diversity, communication richness improve user motives, which have a positive impact on intention. Epistemic curiosity has a moderating effect on the links between motives and intention. Theoretical and practical implications are discussed in conclusion. 相似文献
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Vo-Gia Loc Ig Mo Koo Duc Trong Tran Sangdoek Park Hyungpil Moon Hyouk Ryeol ChoiAuthor vitae 《Robotics and Autonomous Systems》2011,59(12):1036-1048
This paper presents a study on improving the traversability of a quadruped walking robot in 3D rough terrains. The key idea is to exploit body movement of the robot. The position and orientation of the robot are systematically adjusted and the possibility of finding a valid foothold for the next swing is maximized, which makes the robot have more chances to overcome the rough terrains. In addition, a foothold search algorithm that provides the valid foothold while maintaining a high traversability of the robot, is investigated and a gait selection algorithm is developed to help the robot avoid deadlock situations. To explain the algorithms, new concepts such as reachable area, stable area, potential search direction, and complementary kinematic margin are introduced, and the effectiveness of the algorithms is validated via simulations and experiments. 相似文献