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341.
342.
Hsiao IT Khurd P Rangarajan A Gindi G 《Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment》2006,569(2):429-433
Statistical reconstruction has become popular in emission computed tomography but suffers slow convergence (to the MAP or ML solution). Methods proposed to address this problem include the fast but non-convergent OSEM and the convergent RAMLA [1] for the ML case, and the convergent BSREM [2], relaxed OS-SPS and modified BSREM [3] for the MAP case. The convergent algorithms required a user-determined relaxation schedule. We proposed fast convergent OS reconstruction algorithms for both ML and MAP cases, called COSEM (Complete-data OSEM), which avoid the use of a relaxation schedule while maintaining convergence. COSEM is a form of incremental EM algorithm. Here, we provide a derivation of our COSEM algorithms and demonstrate COSEM using simulations. At early iterations, COSEM-ML is typically slower than RAMLA, and COSEM-MAP is typically slower than optimized BSREM while remaining much faster than conventional MAP-EM. We discuss how COSEM may be modified to overcome these limitations. 相似文献
343.
使用计算机免不了时常受到各种病毒的骚扰,而且随着网络应用的不断深入,这种骚扰也越来越多。在和计算机病毒的对抗中,专业人士发现了一些规律,我们在这儿将这些规律总结归纳,暂且叫做“三大注意”供大家参考,希望能为您对付病毒有所帮助。 相似文献
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345.
随着无线局域网设备的价格逐渐走低,无线局域网组网的简便和快速部署的优点越来越明显,应用也越来越普遍,特别在SOHU级(家庭间,小区楼宇间,对面街等)的无线组网中,这个市场特别活跃,作为无线传输,大家很容易将关心的话题集中到传输距离上, 相似文献
346.
Modeling global-scale fate and transport of perfluorooctanoate emitted from direct sources 总被引:1,自引:0,他引:1
Armitage J Cousins IT Buck RC Prevedouros K Russell MH MacLeod M Korzeniowski SH 《Environmental science & technology》2006,40(22):6969-6975
The long-term (1950-2050) global fate of perfluorooctanoate (PFO) is investigated using the global distribution model, GloboPOP. The model is used to test the hypotheses that direct PFO emissions can account for levels observed in the global oceans and that ocean water transport to the Arctic is an important global distribution pathway. The model emission scenarios are derived from historical and projected PFO emissions solely from direct sources. Modeled ocean water concentrations compare favorably to observed PFO concentrations in the world's oceans and thus ocean inventories can be accounted for by direct sources. The model results support the hypothesis that long-range ocean transport of PFO to the Arctic is important and estimate a net PFO influx of approximately 8-23 tons per year flowing into the model's Northern Polar zone in 2005, an amount at least 1 order of magnitude greater than estimated PFO flux to the Arctic from potential indirect sources such as atmospheric transport and degradation of fluorotelomer alcohols. Modeled doubling times of ocean water concentrations in the Arctic between 1975 and 2005 of approximately 7.5-10 years are in good agreement with doubling times of PFO in Arctic biota estimated from monitoring data. The model is further applied to predict future trends in PFO contamination levels using forecasted (2005-2050) direct emissions, including substantial reductions committed to by industry. Modeled ocean water concentrations in zones near to sources decline markedly after 2005, whereas modeled concentrations in the Arctic are predicted to continue to increase until approximately 2030 and show no significant decrease for the remaining 20 years of the model simulation. Since water is the primary exposure medium for Arctic biota, these model results suggest that concentrations in Arctic biota may continue to rise long after direct emissions have been substantially reduced or eliminated. 相似文献
347.
Calle GR Vargas IT Alsina MA Pasten PA Pizarro GE 《Environmental science & technology》2007,41(21):7430-7436
Traditional studies of copper release in plumbing systems assume that the water extracted from a pipe follows a plug-type flow and that the pipe surface does not interact with the bulk water under flow conditions. We characterized actual stagnation-flushing cycles in a household pipe undergoing corrosion in the presence of a microbial biofilm. The mass of copper released in 10 experiments was on average 8 times the value estimated by using the plug-flow assumption. The experimental copper release pattern was explained by an advection-diffusion model only if a high copper concentration occurs near the pipe surface after stagnation. Microscopic examination of the pipe surface showed a complex assemblage of biotic and abiotic features. X-ray diffraction analyses identified only malachite, while X-ray absorption spectroscopy also revealed cupric hydroxide and cuprite. These results indicate that the surface serves as a storage compartment of labile copper that may be released under flow conditions. Thus, the diffusive transport from the pipe surface to the bulk during stagnation is not the only control of the flux of copper to the tap water when porous reactive microstructures cover the pipe. Our results highlight the need for models that consider the interaction between the hydrodynamics, chemistry, and structure at the solid-water interface to predict the release of corrosion byproducts into drinking water. 相似文献
348.
Law GT Geissler A Lloyd JR Livens FR Boothman C Begg JD Denecke MA Rothe J Dardenne K Burke IT Charnock JM Morris K 《Environmental science & technology》2010,44(23):8924-8929
Microbial processes can affect the environmental behavior of redox sensitive radionuclides, and understanding these reactions is essential for the safe management of radioactive wastes. Neptunium, an alpha-emitting transuranic element, is of particular importance because of its long half-life, high radiotoxicity, and relatively high solubility as Np(V)O(2)(+) under oxic conditions. Here, we describe experiments to explore the biogeochemistry of Np where Np(V) was added to oxic sediment microcosms with indigenous microorganisms and anaerobically incubated. Enhanced Np removal to sediments occurred during microbially mediated metal reduction, and X-ray absorption spectroscopy showed this was due to reduction to poorly soluble Np(IV) on solids. In subsequent reoxidation experiments, sediment-associated Np(IV) was somewhat resistant to oxidative remobilization. These results demonstrate the influence of microbial processes on Np solubility and highlight the critical importance of radionuclide biogeochemistry in nuclear legacy management. 相似文献
349.
Burke IT Boothman C Lloyd JR Livens FR Charnock JM McBeth JM Mortimer RJ Morris K 《Environmental science & technology》2006,40(11):3529-3535
Technetium is a redox active radionuclide, which is present as a contaminant at a number of sites where nuclear fuel cycle operations have been carried out. Recent studies suggest that Tc(VII), which is soluble under oxic conditions, will be retained in sediments as Fe(III)-reducing conditions develop, due to reductive scavenging as hydrous TcO2. However, the behavior of technetium during subsequent reoxidation of sediments remains poorly characterized. Here, we describe a microcosm-based approach to investigate the reoxidation behavior of reduced, technetium-contaminated sediments. In reoxidation experiments, the behavior of Tc was strongly dependent on the nature of the oxidant. With air, reoxidation of Fe(II) and, in sulfate-reducing sediments, sulfide occurred accompanied by approximately 50% remobilization of Tc to solution as TcO4-. With nitrate, reoxidation of Fe(II) and, in sulfate-reducing sediments, sulfide only occurred in microbially active experiments where Fe(II) and sulfide oxidation coupled to nitrate reduction was occurring. Here, Tc was recalcitrant to remobilization with <10% Tc remobilized to solution even when extensive Fe(II) and sulfide reoxidation had occurred. X-ray absorption spectroscopy on reoxidized sediments suggested that 15-50% of Tc bound to sediments was present as Tc(VII). Overall, these results suggest that Tc reoxidation behavior is not directly coupled to Fe or S oxidation and that the extent of Tc remobilization is dependent on the nature of the oxidant. 相似文献
350.
In the radioactive waste management, metal chloride wastes from a pyrochemical process is one of problematic wastes not directly applicable to a conventional solidification process. Different from a use of minerals or a specific phosphate glass for immobilizing radioactive waste salts, our research group applied an inorganic composite, SAP (SiO(2)-Al(2)O(3)-P(2)O(5)), to stabilize them by dechlorination. From this method, a unique wasteform composing of phosphate and silicate could be fabricated. This study described the characteristic of the wasteform on the morphology, chemical durability, and some physical properties. The wasteform has a unique "domain-matrix" structure which would be attributed to the incompatibility between silicate and phosphate glass. At higher amounts of chemical binder, "P-rich phase encapsulated by Si-rich phase" was a dominant morphology, but it was changed to be Si-rich phase encapsulated by P-rich phase at a lower amount of binder. The domain and subdomain size in the wasteform was about 0.5-2 μm and hundreds of nm, respectively. The chemical durability of wasteform was confirmed by various leaching test methods (PCT-A, ISO dynamic leaching test, and MCC-1). From the leaching tests, it was found that the P-rich phase had ten times lower leach-resistance than the Si-rich phase. The leach rates of Cs and Sr in the wasteform were about 10(-3)g/m(2)· day, and the leached fractions of them were about 0.04% and 0.06% at 357 days, respectively. Using this method, we could stabilize and solidify the waste salt to form a monolithic wasteform with good leach-resistance. Also, the decrease of waste volume by the dechlorination approach would be beneficial in the final disposal cost, compared with the present immobilization methods for waste salt. 相似文献