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131.
In this work we introduce and analyze a mixed virtual element method for the two-dimensional nonlinear Brinkman model of porous media flow with non-homogeneous Dirichlet boundary conditions. For the continuous formulation we consider a dual-mixed approach in which the main unknowns are given by the gradient of the velocity and the pseudostress, whereas the velocity itself and the pressure are computed via simple postprocessing formulae. In addition, because of analysis reasons we add a redundant term arising from the constitutive equation relating the pseudostress and the velocity, so that the well-posedness of the resulting augmented formulation is established by using known results from nonlinear functional analysis. Then, we introduce the main features of the mixed virtual element method, which employs an explicit piecewise polynomial subspace and a virtual element subspace for approximating the aforementioned main unknowns, respectively. In turn, the associated computable discrete nonlinear operator is defined in terms of the \(\mathbb {L}^2\)-orthogonal projector onto a suitable space of polynomials, which allows the explicit integration of the terms involving deviatoric tensors that appear in the original setting. Next, we show the well-posedness of the discrete scheme and derive the associated a priori error estimates for the virtual element solution as well as for the fully computable projection of it. Furthermore, we also introduce a second element-by-element postprocessing formula for the pseudostress, which yields an optimally convergent approximation of this unknown with respect to the broken \(\mathbb {H}(\mathbf {div})\)-norm. Finally, several numerical results illustrating the good performance of the method and confirming the theoretical rates of convergence are presented. 相似文献
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Alireza Kondori Zhen Jiang Mohammadreza Esmaeilirad Mahmoud Tamadoni Saray Arvin Kakekhani Kamil Kucuk Pablo Navarro Munoz Delgado Sadaf Maghsoudipour John Hayes Christopher S. Johnson Carlo U. Segre Reza Shahbazian-Yassar Andrew M. Rappe Mohammad Asadi 《Advanced materials (Deerfield Beach, Fla.)》2020,32(50):2004028
The main drawbacks of today's state-of-the-art lithium–air (Li–air) batteries are their low energy efficiency and limited cycle life due to the lack of earth-abundant cathode catalysts that can drive both oxygen reduction and evolution reactions (ORR and OER) at high rates at thermodynamic potentials. Here, inexpensive trimolybdenum phosphide (Mo3P) nanoparticles with an exceptional activity—ORR and OER current densities of 7.21 and 6.85 mA cm−2 at 2.0 and 4.2 V versus Li/Li+, respectively—in an oxygen-saturated non-aqueous electrolyte are reported. The Tafel plots indicate remarkably low charge transfer resistance—Tafel slopes of 35 and 38 mV dec−1 for ORR and OER, respectively—resulting in the lowest ORR overpotential of 4.0 mV and OER overpotential of 5.1 mV reported to date. Using this catalyst, a Li–air battery cell with low discharge and charge overpotentials of 80 and 270 mV, respectively, and high energy efficiency of 90.2% in the first cycle is demonstrated. A long cycle life of 1200 is also achieved for this cell. Density functional theory calculations of ORR and OER on Mo3P (110) reveal that an oxide overlayer formed on the surface gives rise to the observed high ORR and OER electrocatalytic activity and small discharge/charge overpotentials. 相似文献
135.
Veronica Gil-Costa Mauricio Marin Carolina Bonacic Roberto Solar 《The Journal of supercomputing》2018,74(5):2006-2034
Large-scale similarity search engines are complex systems devised to process unstructured data like images and videos. These systems are deployed on clusters of distributed processors communicated through high-speed networks. To process a new query, a distance function is evaluated between the query and the objects stored in the database. This process relays on a metric space index distributed among the processors. In this paper, we propose a cache-based strategy devised to reduce the number of computations required to retrieve the top-k object results for user queries by using pre-computed information. Our proposal executes an approximate similarity search algorithm, which takes advantage of the links between objects stored in the cache memory. Those links form a graph of similarity among pre-computed queries. Compared to the previous methods in the literature, the proposed approach reduces the number of distance evaluations up to 60%. 相似文献
136.
Cremona M Mauricio MH Scavarda Do Carmo LC Prioli R Nunes VB Zanette SI Caride AO Albuquerque MP 《Journal of microscopy》2000,197(3):260-267
The influence of the deposition temperature on the grain size of polycrystalline lithium fluoride (LiF) thin films is studied using a mathematical morphology method. On atomic force microscopy images of the LiF surface, the grain sizes and shapes are determined by applying the watershed technique, together with a shape factor algorithm. Also, the domain size of the film structure, determined by an X-ray diffraction data analysis, is compared and correlated with the mean grain size as a function of the deposition temperature. In both cases a linear increase with temperature and a very good agreement among the two structural parameters (grain and domain size) was found. 相似文献
137.
Gabriel Salierno Mauricio Maestri Stella Piovano Miryan Cassanello María Angélica Cardona Daniel Hojman Héctor Somacal 《中国化学工程学报》2018,26(6):1370-1382
Features of the motion of gel particles in a three-phase bubble column with non-foaming and foaming gas–liquid systems,determined by using experiments of radioactive particle tracking(RPT),have been compared.The tracer used is a gel particle which resembles typical immobilized biocatalyst.The tracer trajectory is analyzed to extract relevant information for design purposes.The solid velocity field,turbulence parameters,dispersion coefficients,mixing times and flow transitions are determined and compared.The presence of foam significantly affects many quantified parameters,especially within the heterogeneous flow regime.The hydrodynamic stresses are reduced in the presence of foam,especially close to the disengagement.The dispersion coefficients also decrease,and the solid mixing time is only slightly affected by the presence of foam.Gas holdup,inferred both from RPT experiments and from gamma ray scanning,is higher for foaming systems and leads to a shift in the transition gas velocity towards higher values. 相似文献
138.
CFD as an approach to understand flammable dust 20 L standard test: Effect of the ignition time on the fluid flow
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Daniel Vizcaya Andrés Pinilla Mariangel Amín Nicolás Ratkovich Felipe Munoz Carlos Murillo Nathalie Bardin‐Monnier Olivier Dufaud 《American Institute of Chemical Engineers》2018,64(1):42-54
A computational study based on the Euler–Lagrange approach was developed for the characterization of flammable dusts in the 20 L sphere standard test. The aim of the study was to analyze some parameters that might affect the experimental data (e.g., cold turbulence and particle size). The turbulence of a wheat starch cloud was described with the Detached Eddy Simulation model. Both the pressure of the system and the RMS velocity were compared with the flow patterns established with a particle image velocimetry analysis. It was concluded that the rebound nozzle forms a cloud that is composed by clumps. This fact implies dissimilarities between the local concentrations and the nominal value. Finally, a granulometric analysis established that the mean diameter of the particle size distribution (PSD) decreased by 69% during the dispersion. Thus, it is suggested to consider the PSD at the ignition zone rather than the PSD of the sample. © 2017 American Institute of Chemical Engineers AIChE J, 63: 42–54, 2018 相似文献
139.
Queirolo F Stegen S Mondaca J Cortés R Rojas R Contreras C Munoz L Schwuger MJ Ostapczuk P 《The Science of the total environment》2000,255(1-3):85-95
Lake Velenje is located in one of the most polluted regions in Slovenia, the Salek Valley. The major source of pollution in the valley is the coal-fired thermal power plant in Sostanj (STPP, capacity 775 MW). It has five separate units. All units have electrostatic precipitators for fly ash removal. Unit 4 also has installed a wet flue gas desulfurisation system (FGD system). Total mercury (THg) concentrations were measured in lignite, slag and ash samples from the STPP. In flue gas, different mercury species (THg, MeHg, Hg2+, Hg0) were determined separately for unit 4 and unit 5 which use different flue gas cleaning technology. Mercury and methyl mercury (MeHg) concentrations were also measured in lake water at different depths, in inflow water, outflow water, rain, snow and lake sediments in order to establish the influence of the power plant on the lake. Most mercury emitted from the power plant is in the elemental form. The ratio between oxidised and elemental Hg depends on the flue gas cleaning technology. Mass balance calculations have been performed for the STPP. The results show that the major sources of mercury in Lake Velenje are wet deposition and lake inflows. Total and MeHg concentrations in the water column are very low and can be compared to other non-contaminated freshwater lakes in the world. 相似文献
140.
Karina Donadel Marcos D.V. Felisberto Valfredo T. Fávere Mauricio Rigoni Nelson Jhoe Batistela Mauro C.M. Laranjeira 《Materials science & engineering. C, Materials for biological applications》2008,28(4):509-514
Magnetic particles are extremely interesting for several biomedical applications; amongst these are therapeutic applications, such as: hyperthermia and release of drugs. The use of magnetic particles to induce hyperthermia in biological tissues is an important factor in cancer therapy. The aim of this study was to prepare and characterize iron oxide magnetic particles coated with biopolymer chitosan, and also to produce ferrofluids from the magnetic particles. The iron oxide magnetic particles (IOMP) were coated with chitosan (CS) by spray-drying method using two IOMP/coating ratios (IOMP/CS = 1.6 and IOMP/CS = 4.5). The magnetic particles were characterized by way of scanning electronic microscopy and energy-dispersive X-ray. The analysis by energy-dispersive X-ray was carried out to determine the chemical composition of particles in samples. The size distribution the iron oxide magnetic particles uncoated and coated were evaluated by the laser diffraction analysis and image analysis, respectively. Amongst the prepared ferrofluids, the sample IOMP/CS = 1.6 proved to be the one that has brought about the best results in therapeutics applications, such as in hyperthermia treatment. This sample was placed within an alternating magnetic field during 40 min, it was observed that 1 °C heated in 3 min and underwent a temperature variation of 7 °C, since it varied from 25 °C to 32 °C. Considering that the experiment would be carried out at body temperature 37 °C, probably, the temperature variation would be very close to the one reported at 25 °C. In such a way, the cancerous cells would reach 44–45 °C and at such temperatures the cancer cells generally perish. 相似文献