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排序方式: 共有371条查询结果,搜索用时 15 毫秒
31.
Tetrathiafulvalene tetrabenzoate (TTFTB) and several lanthanide ions self-assemble into metal-organic frameworks (MOFs) that exhibit a novel topology, a (3,3,3,6,6)-coordinated net, which features an unusual ligand coordination mode and stacking motif. The Yb and Lu MOFs are electrically conductive, with pellet conductivity values of 9(7) × 10−7 and 3(2) × 10−7 S/cm, respectively. The crystallographically-determined bond lengths indicate partial oxidation of the ligand, with close S ⋅ ⋅ ⋅ S contacts between ligands providing likely charge transport pathways in the material. Magnetometry reveals temperature-independent paramagnetism, consistent with the presence of ligand-based radicals, as well as weak antiferromagnetic coupling between Yb3+ centers. These results illustrate the diversity of MOF structures and properties that are accessible with the TTFTB ligand owing to its electroactive nature, propensity for intermolecular interactions, and conformational flexibility. 相似文献
32.
We present a fast incremental algorithm for constructing minimal Deterministic Finite Cover Automata (DFCA) for a given language. Since it was shown that the minimal DFCA for a language L has less states than the minimal Deterministic Finite Automata (DFA) for the same language L, this technique seems to be the best choice for incrementally building the automaton for a large language, especially when the number of states in the DFCA is significantly less than the number of states in the corresponding minimal DFA. We have implemented the proposed algorithm and have tested it against the best-known DFCA minimization technique. 相似文献
33.
Radu-Emil Precup Marius L. Tomescu Mircea-Bogdan Rădac Emil M. Petriu Stefan Preitl Claudia-Adina Dragoş 《Expert systems with applications》2012,39(9):8288-8299
This paper suggests the performance improvement of fuzzy control systems (FCSs) for three tank systems using iterative feedback tuning (IFT). The stable design of Takagi–Sugeno–Kang fuzzy controllers is guaranteed by means of a stability theorem based on LaSalle’s global invariant set theorem formulated for a class of multi input-multi output (MIMO) nonlinear processes. An IFT algorithm characterized by setting the step size to guarantee the FCS stability is proposed. The theoretical approaches are applied in a case study that deals with the IFT-based stable design of fuzzy controllers dedicated to the level control of a cylindrical three tank system as a representative MIMO system. A set of experimental results for a laboratory setup illustrates the performance improvement. 相似文献
34.
C. I. Simionescu A. A. Popa E. Comăniţlă B. Comăniţlă 《Polymer-Plastics Technology and Engineering》2013,52(5-6):451-461
The paper reports on the synthesis of a new bifunctional radicalic initiator and its behavior in the polymerization process. The synthesis of cumyl 4-t-butylazo-4-cyanoperoxypentanoate has been achieved by condensation of the corresponding acid chloride with cumen hydroperoxide. The structure of the azo perester is confirmed by IR, UV, and NMR spectra. The initiator has been used in styrene polymerization and the conversion of the polymer studied in connection to monomer and initiator concentration, time of reaction, and temperature. In compliance with multiple regression method, an equation correlating the PS conversion with the previously mentioned variables has been established. 相似文献
35.
Aura Angelica Popa Eugenia Comăniţă Luminiţ Cianga C. I. Simionescu 《Polymer-Plastics Technology and Engineering》2013,52(9-10):871-884
The paper discusses the synthesis of the N,N,′-azobis(formamidopropionic) acid (AFP), along with some characteristics determined from NMR spectrum, differential thermal analysis, and DSC. The behavior of AFP acid—as well as of its analogue, N,N′-azobis(formamidoacetic) acid (AFA)—has been studied in the reaction with aromatic diamine and with bis(glycol)terephthalate, leading to azopolymers of the azopolyamide, or azopolyester, type. On employing N,N′-bis(β-hydroxyethyl) azobis-formamide (HEAF) as the azo bifunctional compound in the reaction with diphenylmethane diisocyanate, a polyurethane possessing azo groups was obtained. The structure of the azopolymers has been spectroscopically confirmed. 相似文献
36.
Ana Maria Săcară Vasile-Mircea Cristea Liana Maria Mureşan 《Chemical Engineering Communications》2013,200(10):1249-1263
Removal of malachite green (MG) onto fir (Abies nordmanniana) cones biomass (FCB) as a lingo-cellulosic-based structure material was investigated in the present study. Characterization of FCB was performed using Fourier transform infra red and scanning electron microscobe analyses. Several parameters (biomass dose and particle size, dye concentration, temperature, and pH) were investigated to determine optimal working conditions. Subsequently, FCB yelded a qe of 2.2?mg/g for 50?g/L FCB, in an MG solution of 110?mg/L, pH 3.3, at a temperature of 21?°C, on a 0.2-0.4?mm fraction powder after 146?h of contact. Adaptive neuro-fuzzy interference system modeling was applied to experimental data and results showed that predicted model fitted experimental data with R2 = 0.994. In a nutshell, it can be concluded that FCB shows good potential for treating MG contaminated waters. 相似文献
37.
38.
Costin S Bîldea Cătălin Pătruţ Sten Bay Jørgensen Jens Abildskov Anton A Kiss 《Journal of chemical technology and biotechnology (Oxford, Oxfordshire : 1986)》2016,91(5):1215-1223
Process intensification in distillation systems has received much attention during past decades, with the aim of increasing both energy and separation efficiency. Various techniques, such as internal heat‐integrated distillation, membrane distillation, rotating packed bed, dividing‐wall columns and reactive distillation were studied and reported in the literature. All these techniques employ the conventional continuous counter‐current contact of vapor and liquid phases. Cyclic distillation technology is based on an alternative operating mode using separate phase movement which leads to key practical advantages in both chemical and biochemical processes. This article provides a mini‐review of cyclic distillation technology. The topics covered include the working principle, design and control methods, main benefits and limitations as well as current industrial applications. Cyclic distillation can be rather easily implemented in existing columns by simply changing the internals and the operating mode, thus bringing new life to old distillation towers by significantly increasing the column throughput, reducing the energy requirements and offering better separation performance. © 2016 Society of Chemical Industry 相似文献
39.
Marcela Stoia Cornelia Păcurariu Ciprian Mihali Iosif Mălăescu Cătălin Nicolae Marin Aylin Căpraru 《Ceramics International》2019,45(2):2725-2735
Magnetic MnFe2O4 nanopowders were synthesized by an original solvothermal method in the absence and in the presence of tetra-n-butylammonium bromide (TBAB) and Tween 80 (TW) as surfactants. Manganese ferrite/polyaniline (PANI) hybrid materials were synthesized by in situ polymerization of aniline on the surface of MnFe2O4 using ammonium persulfate as oxidant. The purpose of the study was to investigate the influence of the two surfactants on the properties of the MnFe2O4 powders and of their composites with PANI. The specific surface area, the cumulative surface area of pores and the cumulative volume of pores are influenced by the nature of surfactant in case of MnFe2O4 powders and are higher by comparison to those of the MnFe2O4/PANI hybrid materials. The values of saturation magnetization in case of MnFe2O4 powders are higher than those of the hybrid materials and are not influenced by the surfactant nature. These features revealed that MnFe2O4 powders can be efficiently used as adsorbents for the purification of wastewaters. The values of the electrical conductivity of the composites exhibit a significant increase in comparison to the MnFe2O4 powders and depend on the surfactant nature. The highest value of electrical conductivity was achieved by the composite obtained using Tween 80 as surfactant (σDC = 54.5·10?5S?m?1) which was close to that of PANI (σDC = 61.2·10?5 S?m?1). The fact that the magnetic and electric properties of the synthesized MnFe2O4/PANI composites can be changed by design, demonstrate the high potential of these materials to be used in magneto-electric applications. 相似文献
40.
Sorin-Cristian Vlădescu Alessandra Ciniero Khizer Tufail Arup Gangopadhyay Tom Reddyhoff 《摩擦学汇刊》2018,61(3):522-531
It has recently been shown that rectangular surface pockets are effective in reducing friction in a piston–liner type contact, providing that they are oriented with their long axis transverse to the sliding direction so that entrained features fit completely within the contact area (Vl?descu, et al., Tribology International, 82, 28–42, 2015; Vl?descu, et al., Tribology International, 115, 140–153, 2017). The aim of the current study was to identify the optimal geometric parameters of theses rectangular features. To do this, a friction rig that simulated a piston–liner contact under highly controlled conditions was used to test a series of textured specimens with pockets of different depth, breadth and density. Each of these geometric parameters was varied and tested independently, while keeping the other two constant. Experimental conditions were set in order to place the contact in different lubrication regimes.Results were analyzed to determine a set of criteria for the optimum pocket geometry; however, this was shown to change depending on the test conditions and should therefore be adjusted depending on the position along the stroke. Specifically, at low speed when the contact is operating under boundary lubrication, pockets should be deep, wide, and densely spaced. This confirms recent findings, which suggested that, in this regime, pocket volume is often a more critical parameter than depth, width, or spacing individually. Conversely, under mixed lubrication toward the transition to the full film regime, pockets should be narrow and sparsely spaced. These results also explain the difficulties encountered in several previous studies that attempted to define a single optimum pocket geometry.Finally, the impact of pocket position relative to reversal was assessed for various lubrication conditions. This revealed how pockets should be placed close to, but not directly at, top and bottom dead center to provide a beneficial squeeze film, which is present at reversal. 相似文献