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991.
Alternating Stacked Graphene‐Conducting Polymer Compact Films with Ultrahigh Areal and Volumetric Capacitances for High‐Energy Micro‐Supercapacitors 下载免费PDF全文
992.
Sarmad Ali Khan Muhammad Aftab Ahmad Zakria Ghulam Muhammad Asif Mahmood Qureshi 《Materials and Manufacturing Processes》2017,32(6):670-677
Multi-radii tool inserts offer novel configuration that comprises of multiple radii at tool nose. A review of the available literature indicates that there exists a need for experimental investigation on certain key machining characteristics of such tools. This paper reports on tool wear/life, material removed, and workpiece surface roughness when multi-radii mixed alumina TiN coated tool inserts are employed for turning D2 steel. Inserts of three different nose radii (0.40, 0.80, 1.20?mm) at six levels of feed rates (ranging from 0.157 to 0.562?mm/rev) are used. Results show that flank wear is the dominant wear mode with catastrophic tool failure occurring at highest nose radius (1.20?mm) and feed rate (0.562?mm/rev) combination. Also, there is ~59% reduction in tool life accompanied by ~62% increase in quantity of material removed as the feed rate increases from 0.157 to 0.562?mm/rev at maximum nose radius (1.20?mm). Feed rate is found to be statistically significant factor for all three responses considered herein at 95% confidence level. Surface integrity assessment at maximum feed rate reveals presence of a strain hardened layer extending to the depth of 150?µm below the machined surface without any observance of white layer for all the tool conditions and nose radius. 相似文献
993.
Abstract By taking advantage of four‐tone structure in the pitch contour of Mandarin speech, we described text‐independent speaker identification using orthogonal pitch parameters. Slopes, mean and duration of the pitch contours of words in an utterance are taken as recognition features. An identification rate of 85% is achieved by using the parameters of pitch contour only. When incorporating parameters of pitch contour with the parameter of vocal tract, this system outperforms that using parameters of vocal tract or pitch contour only. A recognition rate of 99.7% is reached in such a system. 相似文献
994.
Influence of Temperature on the Colloidal Stability of Polymer‐Coated Gold Nanoparticles in Cell Culture Media 下载免费PDF全文
Mikhail V. Zyuzin Tobias Honold Susana Carregal‐Romero Karsten Kantner Matthias Karg Wolfgang J. Parak 《Small (Weinheim an der Bergstrasse, Germany)》2016,12(13):1723-1731
The temperature‐dependence of the hydrodynamic diameter and colloidal stability of gold‐polymer core‐shell particles with temperature‐sensitive (poly(N‐isopropylacrylamide)) and temperature‐insensitive shells (polyallylaminine hydrochloride/polystyrensulfonate, poly(isobutylene‐alt‐maleic anhydride)‐graft‐dodecyl) are investigated in various aqueous media. The data demonstrate that for all nanoparticle agglomeration, i.e., increase in effective nanoparticle size, the presence of salts or proteins in the dispersion media has to be taken into account. Poly(N‐isopropylacrylamide) coated nanoparticles show a reversible temperature‐dependent increase in size above the volume phase transition of the polymer shell when they are dispersed in phosphate buffered saline or in media containing protein. In contrast, the nanoparticles coated with temperature‐insensitive polymers show a time‐dependent increase in size in phosphate buffered saline or in medium containing protein. This is due to time‐dependent agglomeration, which is particularly strong in phosphate buffered saline, and induces a time‐dependent, irreversible increase in the hydrodynamic diameter of the nanoparticles. This demonstrates that one has to distinguish between temperature‐ and time‐induced agglomerations. Since the size of nanoparticles regulates their uptake by cells, temperature‐dependent uptake of thermosensitive and non‐thermosensitive nanoparticles by cells lines is compared. No temperature‐specific difference between both types of nanoparticles could be observed. 相似文献
995.
996.
Simple image intensity compensation (SIMIC) method prior to application of distortion correction algorithms in brain diffusion Tensor Magnetic Resonance Imaging: Validation test for two cost functions of distortion correction algorithms 下载免费PDF全文
Dong‐Hoon Lee Do‐Wan Lee Bong‐Soo Han 《International journal of imaging systems and technology》2015,25(4):328-333
The purpose of this study is to design a simple image intensity compensation (SIMIC) method prior to the application of a variety of cost functions for distortion correction in diffusion tensor imaging (DTI). The synthetic dataset consists of each direction of diffusion weighted imaging (DWI) made by multiplication of nondiffusion weighted image (b = 0 image) and tensor matrices. We added the effects of patient motion and eddy current distortion using translation, rotation, scaling and shearing matrices. We calculated the b = 0 image of each direction from original DTI, inversely. A co‐registration method was applied to the extracted b = 0 images of each direction based on the original b = 0 image and then, the transformation matrices were generated and the original DTI were transformed using this transformation matrix. For the DTI distortion correction, two kinds of cost functions, normalized mutual information (NMI) and normalized cross‐correlation (NCC), were used. Visual assessments and quantitative measurements were used to evaluate the results. When using the NMI as a cost function, the quantitative results showed no significant differences between NMI and NMI with SIMIC method. However, there are significant differences compared with using the NCC as a cost function. Our study showed cost function for image distortion correction with SIMIC method improved the results both quantitatively and in terms of qualitative accuracy. This method may be helpful for DTI analysis and helpful for increasing accuracy. © 2015 Wiley Periodicals, Inc. Int J Imaging Syst Technol, 25, 328–33, 2015 相似文献
997.
Non‐oscillatory and non‐singular asymptotic solutions to stress fields at interface cracks 下载免费PDF全文
W.‐S. Lei 《Fatigue & Fracture of Engineering Materials & Structures》2017,40(12):2032-2049
This work concerns the complex oscillatory singularities revealed in Williams's asymptotic solutions to stress fields around arbitrary interface cracks, which are the foundation of phenomenological interface fracture mechanics. First, we highlight the fatal discrepancy between the asymptotic stress fields for cracks in a homogeneous material obtained by assigning an identical material on both regions embracing an interface crack, and the solutions directly derived from cracks in a single material. Next, following a brief introduction to Williams's formulation process, we adopt the method of repeatedly eliminating variables instead of solving the determinant equation for the coefficient matrix to reformulate the asymptotic analysis of stress fields at arbitrary interface cracks. The resultant stresses get rid of oscillatory character. Further, under two specific loading conditions, namely, remotely uniaxial tension or shear, non‐oscillatory and non‐singular asymptotic solutions to stress fields around interface cracks are obtained. 相似文献
998.
Bioinspired Synthesis of All‐in‐One Organic–Inorganic Hybrid Nanoflowers Combined with a Handheld pH Meter for On‐Site Detection of Food Pathogen 下载免费PDF全文
999.
Kuan‐I Ho Jia‐Hong Liao Chi‐Hsien Huang Chang‐Lung Hsu Wenjing Zhang Ang‐Yu Lu Lain‐Jong Li Chao‐Sung Lai Ching‐Yuan Su 《Small (Weinheim an der Bergstrasse, Germany)》2014,10(5):989-997
In this study, the scalable and one‐step fabrication of single atomic‐layer transistors is demonstrated by the selective fluorination of graphene using a low‐damage CF4 plasma treatment, where the generated F‐radicals preferentially fluorinated the graphene at low temperature (<200 °C) while defect formation was suppressed by screening out the effect of ion damage. The chemical structure of the C–F bonds is well correlated with their optical and electrical properties in fluorinated graphene, as determined by X‐ray photoelectron spectroscopy, Raman spectroscopy, and optical and electrical characterizations. The electrical conductivity of the resultant fluorinated graphene (F‐graphene) was demonstrated to be in the range between 1.6 kΩ/sq and 1 MΩ/sq by adjusting the stoichiometric ratio of C/F in the range between 27.4 and 5.6, respectively. Moreover, a unique heterojunction structure of semi‐metal/semiconductor/insulator can be directly formed in a single layer of graphene using a one‐step fluorination process by introducing a Au thin‐film as a buffer layer. With this heterojunction structure, it would be possible to fabricate transistors in a single graphene film via a one‐step fluorination process, in which pristine graphene, partial F‐graphene, and highly F‐graphene serve as the source/drain contacts, the channel, and the channel isolation in a transistor, respectively. The demonstrated graphene transistor exhibits an on‐off ratio above 10, which is 3‐fold higher than that of devices made from pristine graphene. This efficient transistor fabrication method produces electrical heterojunctions of graphene over a large area and with selective patterning, providing the potential for the integration of electronics down to the single atomic‐layer scale. 相似文献
1000.
Jiangzhao Chen Xing Zhao Seul‐Gi Kim Nam‐Gyu Park 《Advanced materials (Deerfield Beach, Fla.)》2019,31(39)
Chemical interaction at a heterojunction interface induced by an appropriate chemical linker is of crucial importance for high efficiency, hysteresis‐less, and stable perovskite solar cells (PSCs). Effective interface engineering in PSCs is reported via a multifunctional chemical linker of 4‐imidazoleacetic acid hydrochloride (ImAcHCl) that can provide a chemical bridge between SnO2 and perovskite through an ester bond with SnO2 via esterification reaction and an electrostatic interaction with perovskite via imidazolium cation in ImAcHCl and iodide anion in perovskite. In addition, the chloride anion in ImAcHCl plays a role in the improvement of crystallinity of perovskite film crystallinity. The introduction of ImAcHCl onto SnO2 realigns the positions of the conduction and valence bands upwards, reduces nonradiative recombination, and improves carrier life time. As a consequence, average power conversion efficiency (PCE) is increased from 18.60% ± 0.50% to 20.22% ± 0.34% before and after surface modification, respectively, which mainly results from an enhanced voltage from 1.084 ± 0.012 V to 1.143 ± 0.009 V. The best PCE of 21% is achieved by 0.1 mg mL?1 ImAcHCl treatment, along with negligible hysteresis. Moreover, an unencapsulated device with ImAcHCl‐modified SnO2 shows much better thermal and moisture stability than unmodified SnO2. 相似文献