全文获取类型
收费全文 | 433篇 |
免费 | 40篇 |
国内免费 | 2篇 |
专业分类
电工技术 | 4篇 |
综合类 | 1篇 |
化学工业 | 156篇 |
金属工艺 | 10篇 |
机械仪表 | 6篇 |
建筑科学 | 5篇 |
矿业工程 | 1篇 |
能源动力 | 17篇 |
轻工业 | 15篇 |
水利工程 | 1篇 |
石油天然气 | 7篇 |
无线电 | 42篇 |
一般工业技术 | 119篇 |
冶金工业 | 8篇 |
原子能技术 | 9篇 |
自动化技术 | 74篇 |
出版年
2023年 | 6篇 |
2022年 | 40篇 |
2021年 | 37篇 |
2020年 | 15篇 |
2019年 | 19篇 |
2018年 | 16篇 |
2017年 | 19篇 |
2016年 | 26篇 |
2015年 | 20篇 |
2014年 | 30篇 |
2013年 | 36篇 |
2012年 | 31篇 |
2011年 | 35篇 |
2010年 | 14篇 |
2009年 | 16篇 |
2008年 | 18篇 |
2007年 | 20篇 |
2006年 | 12篇 |
2005年 | 11篇 |
2004年 | 6篇 |
2003年 | 17篇 |
2002年 | 9篇 |
2001年 | 5篇 |
2000年 | 3篇 |
1998年 | 4篇 |
1997年 | 1篇 |
1995年 | 1篇 |
1993年 | 2篇 |
1986年 | 1篇 |
1984年 | 1篇 |
1982年 | 1篇 |
1979年 | 1篇 |
1978年 | 1篇 |
1970年 | 1篇 |
排序方式: 共有475条查询结果,搜索用时 15 毫秒
51.
52.
Marjo Kettunen Riitta J. Silvennoinen Nikolay Houbenov Antti Nykänen Janne Ruokolainen Jani Sainio Viljami Pore Marianna Kemell Mikael Ankerfors Tom Lindström Mikko Ritala Robin H. A. Ras Olli Ikkala 《Advanced functional materials》2011,21(3):510-517
Chemical vapor deposition of a thin titanium dioxide (TiO2) film on lightweight native nanocellulose aerogels offers a novel type of functional material that shows photoswitching between water‐superabsorbent and water‐repellent states. Cellulose nanofibrils (diameters in the range of 5–20 nm) with native crystalline internal structures are topical due to their attractive mechanical properties, and they have become relevant for applications due to the recent progress in the methods of their preparation. Highly porous, nanocellulose aerogels are here first formed by freeze‐drying from the corresponding aqueous gels. Well‐defined, nearly conformal TiO2 coatings with thicknesses of about 7 nm are prepared by chemical vapor deposition on the aerogel skeleton. Weighing shows that such TiO2‐coated aerogel specimens essentially do not absorb water upon immersion, which is also evidenced by a high contact angle for water of 140° on the surface. Upon UV illumination, they absorb water 16 times their own weight and show a vanishing contact angle on the surface, allowing them to be denoted as superabsorbents. Recovery of the original absorption and wetting properties occurs upon storage in the dark. That the cellulose nanofibrils spontaneously aggregate into porous sheets of different length scales during freeze‐drying is relevant: in the water‐repellent state they may stabilize air pockets, as evidenced by a high contact angle, in the superabsorbent state they facilitate rapid water‐spreading into the aerogel cavities by capillary effects. The TiO2‐coated nanocellulose aerogels also show photo‐oxidative decomposition, i.e., photocatalytic activity, which, in combination with the porous structure, is interesting for applications such as water purification. It is expected that the present dynamic, externally controlled, organic/inorganic aerogels will open technically relevant approaches for various applications. 相似文献
53.
Yuan Hsing Fu Ai Qun Liu Wei Ming Zhu Xu Ming Zhang Din Ping Tsai Jing Bo Zhang Ting Mei Ji Fang Tao Hong Chen Guo Xin Hai Zhang Jing Hua Teng Nikolay I. Zheludev Guo Qiang Lo Dim Lee Kwong 《Advanced functional materials》2011,21(18):3589-3594
A micromachined reconfigurable metamaterial is presented, whose unit cell consists of a pair of asymmetric split‐ring resonators (ASRRs); one is fixed to the substrate while the other is patterned on a movable frame. The reconfigurable metamaterial and the supporting structures (e.g., microactuators, anchors, supporting frames, etc.) are fabricated on a silicon‐on‐insulator wafer using deep reactive‐ion etching (DRIE). By adjusting the distance between the two ASRRs, the strength of dipole–dipole coupling can be tuned continuously using the micromachined actuators and this enables tailoring of the electromagnetic response. The reconfiguration of unit cells endows the micromachined reconfigurable metamaterials with unique merits such as electromagnetic response under normal incidence and wide tuning of resonant frequency (measured as 31% and 22% for transverse electric polarization and transverse magnetic polarization, respectively). The reconfiguration could also allow switching between the polarization‐dependent and polarization‐independent states. With these features, the micromachined reconfigurable metamaterials may find potential applications in transformation optics devices, sensors, intelligent detectors, tunable frequency‐selective surfaces, and spectral filters. 相似文献
54.
Nikolay Tcholtchev Ina Schieferdecker 《International Journal of Communication Systems》2014,27(12):4103-4125
A main requirement for the Future Internet is to enable self‐management behaviors facilitating the network to adapt to changing conditions and self‐heal in the face of erroneous states. On the basis of Autonomic Fault‐Management principles, this paper proposes a framework consisting of a set of components operating inside the network elements and allowing the devices to collaboratively realize self‐healing. In that context, Autonomic Fault‐Management is intuitively constituted by the detection of the presence of faulty conditions, followed in turn by the self‐diagnosis and identification of the corresponding root causes, and completed consequently by the removal of the identified root causes and their effects. The proposed framework implements a distributed control loop that interacts with the network operations personnel in case the current erroneous state is not resolvable by means of Autonomic Fault‐Management. We argue that there are a number of mutual benefits between our proposed framework and the IPv6 protocol suite. This is demonstrated by a case study that illustrates these benefits and shows how the capabilities of IPv6 can be enhanced through the self‐healing mechanisms of the proposed framework. Finally, the prototype implementation used for the case study is analyzed in terms of scalability and overhead produced in the network nodes. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献
55.
Alexander M. Samoylov Sergey A. Buchnev Nikolay N. Dementev Yury V. Synorov Vladimir P. Zlomanov 《Materials Science in Semiconductor Processing》2003,6(5-6):327-333
The chemical quantitative composition, phase constitution, and crystal structure of doped with In lead telluride films on Si (1 0 0) or SiO2/Si (1 0 0) substrates have been studied in this work. By EPMA and atomic absorption measurements, it has been found that the concentration of In atoms yIn varied from 0.0011 to 0.045 in these deposited Pb1−yInyTe films. The results of EPMA, SEM, and X-ray diffraction (XRD) measurements show that formation of In solid solutions in lead telluride matrix revealed not only in PbTe–InTe cross-section, but in PbTe–In2Te3 pseudobinary system also. The results of XRD show that the lattice parameter aPbTe of PbTeIn/Si and PbTeIn/SiO2/Si heterostructures is described by nonmonotone function and does not obey the Vegard's law within concentration interval 0.0011yIn0.045. 相似文献
56.
57.
58.
Seven zooxanthellae-free species of octocorals (the genera Acanthogorgia, Acabaria, Chironephthya, Echinogorgia, Menella, Ellisella, and Bebryce) and two zooxanthellate octocorals (the genera Paralemnalia and Rumphella) were examined to elucidate their fatty acid (FA) composition. Arachidonic (about 40% of the total FA) and palmitic acids
were predominant in all the species studied. Seven furan FA (F-acids) (up to 9.7%) were identified in the azooxanthellate
octocorals. The main F-acids were 14,17-epoxy-15-methyldocosa-14,16-dienoic and 14,17-epoxy-15,16-dimethyldocosa-14,16-dienoic
acids. In all specimens of Bebryce studeri, C25–28 demospongic FA (about 20%) were identified. These FA reflect the presence of a symbiotic sponge in B. studeri and can be used as the specific markers for other corals. A significant difference (P < 0.01) between azooxanthellate and zooxanthellate corals was found for odd-chain and methyl-branched saturated FA, 18:1n-7,
and 7-Me-16:1n-10; that indicated the presence of an advanced bacterial community in azooxanthellate corals. The zooxanthellate
species were distinguished by significant amounts of 18:3n-6, 18:4n-3, and 16:2n-7 acids, which are proposed as the markers
of zooxanthellae in soft corals. Contrary to the normal level of 24:5n-6 (9.4%) and 22:4n-6 (0.6%), unexpected low concentrations
of 24:5n-6 (0.4%) accompanied by a high content of 22:4n-6 (up to 11.9%) were detected in some specimens. The presence of
an unknown factor in octocorals, specific for n-6 PUFA, which inhibited elongation of 22:4n-6 to 24:4n-6, is conjectured. 相似文献
59.
Marina Y. Khodanovich Andrey E. Akulov Tatyana V. Ananina Marina S. Kudabaeva Anna O. Pishchelko Elena P. Krutenkova Nikolay M. Nemirovich-Danchenko Mikhail V. Svetlik Yana A. Tumentceva Chris Van den Haute Rik Gijsbers Veronique Daniëls Irina Thiry Alexandra G. Pershina Maria M. Shadrina Anna V. Naumova 《International journal of molecular sciences》2020,21(23)
(1) Background: Neurogenesis is considered to be a potential brain repair mechanism and is enhanced in stroke. It is difficult to reconstruct the neurogenesis process only from the histological sections taken from different animals at different stages of brain damage and restoration. Study of neurogenesis would greatly benefit from development of tissue-specific visualization probes. (2) Purpose: The study aimed to explore if overexpression of ferritin, a nontoxic iron-binding protein, under a doublecortin promoter can be used for non-invasive visualization of neurogenesis using magnetic resonance imaging (MRI). (3) Methods: Ferritin heavy chain (FerrH) was expressed in the adeno-associated viral backbone (AAV) under the doublecortin promoter (pDCX), specific for young neurons, in the viral construct AAV-pDCX-FerrH. Expression of the enhanced green fluorescent protein (eGFP) was used as an expression control (AAV-pDCX-eGFP). The viral vectors or phosphate-buffered saline (PBS) were injected intracerebrally into 18 adult male Sprague–Dawley rats. Three days before injection, rats underwent transient middle-cerebral-artery occlusion or sham operation. Animals were subjected to In vivo MRI study before surgery and on days 7, 14, 21, and 28 days after injection using a Bruker BioSpec 11.7 T scanner. Brain sections obtained on day 28 after injection were immunostained for ferritin, young (DCX) and mature (NeuN) neurons, and activated microglia/macrophages (CD68). Additionally, RT-PCR was performed to confirm ferritin expression. (4) Results: T2* images in post-ischemic brains of animals injected with AAV-pDCX-FerrH showed two distinct zones of MRI signal hypointensity in the ipsilesioned hemisphere starting from 14 days after viral injection—in the ischemic lesion and near the lateral ventricle and subventricular zone (SVZ). In sham-operated animals, only one zone of hypointensity near the lateral ventricle and SVZ was revealed. Immunochemistry showed that ferritin-expressing cells in ischemic lesions were macrophages (88.1%), while ferritin-expressing cells near the lateral ventricle in animals both after ischemia and sham operation were mostly mature (55.7% and 61.8%, respectively) and young (30.6% and 7.1%, respectively) neurons. RT-PCR confirmed upregulated expression of ferritin in the caudoputamen and corpus callosum. Surprisingly, in animals injected with AAV-pDCX-eGFP we similarly observed two zones of hypointensity on T2* images. Cellular studies also showed the presence of mature (81.5%) and young neurons (6.1%) near the lateral ventricle in both postischemic and sham-operated animals, while macrophages in ischemic lesions were ferritin-positive (98.2%). (5) Conclusion: Ferritin overexpression induced by injection of AAV-pDCX-FerrH was detected by MRI using T2*-weighted images, which was confirmed by immunochemistry showing ferritin in young and mature neurons. Expression of eGFP also caused a comparable reduced MR signal intensity in T2*-weighted images. Additional studies are needed to investigate the potential and tissue-specific features of the use of eGFP and ferritin expression in MRI studies. 相似文献
60.