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31.
This contribution summarizes our recent efforts to unravel the radical chemistry of autoxidations. Abstraction of the weakly bonded αH-atom of the primary hydroperoxide product by chain carrying peroxyl radicals is identified as the source of major end products such as alcohol and ketone/aldehyde. In the case of cyclohexane autoxidation, this reaction is even responsible for the majority of ring-opened by-products. In a second part, different approaches to autoxidation catalysis are discussed, ranging from transition metal ion catalysis to organocatalysis with immobilized N-hydroxyphthalimide. 相似文献
32.
The IEEE 802.11e medium access control (MAC) layer protocol is an emerging standard to support quality of service (QoS) in
802.11 wireless networks. Some recent work shows that the 802.11e hybrid coordination function (HCF) can improve significantly
the QoS support in 802.11 networks. A simple HCF referenced scheduler has been proposed in the 802.11e which takes into account
the QoS requirements of flows and allocates time to stations on the basis of the mean sending rate. As we show in this paper,
this HCF referenced scheduling algorithm is only efficient and works well for flows with strict constant bit rate (CBR) characteristics.
However, a lot of real-time applications, such as videoconferencing, have some variations in their packet sizes, sending rates
or even have variable bit rate (VBR) characteristics. In this paper we propose FHCF, a simple and efficient scheduling algorithm
for 802.11e that aims to be fair for both CBR and VBR flows. FHCF uses queue length estimations to tune its time allocation
to mobile stations. We present analytical model evaluations and a set of simulations results, and provide performance comparisons
with the 802.11e HCF referenced scheduler. Our performance study indicates that FHCF provides good fairness while supporting
bandwidth and delay requirements for a large range of network loads.
Pierre Ansel received a multidisciplinary in-depth scientific training in different fields such as Pure and Applied Mathematics, Physics,
Mechanics, Computer Science and Economics from the Ecole Polytechnique, Palaiseau, France. Then, he joined the Ecole Nationale
Superieure des Telecommunications, Paris, France in 2005 where he went further into electronics, databases, computer network
security and high speed networks. He received a multidisciplinary master of sciences degree and an additional master of sciences
degree in telecommunications in 2005. He did a summer internship in 2003 in INRIA, Sophia Antipolis, France where he worked
on the Quality of Service in 802.11 networks at Planete Group, France. Then in 2004, he joined France Telecom R&D, Issy-les-Moulineaux,
France to work on Intranet Security issues. He designed a WiFi security supervision architecture based on WiFi Intrusion Detection
Sensors. He is currently a French civil servant and belongs to the French Telecommunications Corps.
Qiang Ni received the B.Eng., M.Sc. and Ph.D. degrees from Hua Zhong University of Science and Technology (HUST), Wuhan City, China
in 1993, 1996 and 1999 respectively. He is currently a faculty member in the Electronic and Computer Engineering Division,School
of Engineering and Design, Brunel University, West London, U.K. Between 2004 and 2005 he was a Senior Researcher at the Hamilton
Institute, National University of Ireland, Maynooth. From 1999 to 2001, he was a post-doctoral research fellow in the multimedia
and wireless communication laboratory, HUST, China. He visited and conducted research at the wireless and networking group
of Microsoft Research Asia Lab during the year of 2000. From Sept. 2001 until may 2004, he was a research staff member at
the Planète group of INRIA Sophia Antipolis France. Since 2002, he has been active as a voting member at the IEEE 802.11 wireless
LAN standard working group. His current research interests include communication protocol design and performance analysis
for wireless networks, cross-layer optimizations, vertical handover and mobility management in mobile wireless networks, and
adaptive multimedia transmission over hybrid wired/wireless networks. He has authored /co-authored over 40 international journal/conference
papers, book chapters, and standard drafts in this field. He is a member of IEEE. E-mail: Qiang.Ni@ieee.org
Thierry Turletti received the M.S. (1990) and the Ph.D. (1995) degrees in computer science both from the University of Nice – Sophia Antipolis,
France. He has done his PhD studies in the RODEO group at INRIA Sophia Antipolis. During the year 1995–96, he was a postdoctoral
fellow in the Telemedia, Networks and Systems group at LCS, MIT. He is currently a research scientist at the Planete group
at INRIA Sophia Antipolis. His research interests include multimedia applications, congestion control and wireless networking.
Dr. Turletti currently serves on the Editorial Board of Wireless Communications and Mobile Computing. 相似文献
33.
34.
Sagaspe Patricia; Charles André; Taillard Jacques; Bioulac Bernard; Philip Pierre 《Canadian Metallurgical Quarterly》2003,57(4):265
The literature contains inconsistent data on the effects of acute sleep deprivation on the superior cognitive functions. The primary purpose of this study is to determine the effectiveness of inhibition, one of the functions of the working memory executive centre (EC), over an extended, 36-hour waking period. Inhibition is a cognitive mechanism whereby individuals ignore non-relevant information recorded in their working memory. We also tested the effects of a 36- hour period of acute sleep deprivation on simple reaction time. Twelve young, healthy volunteers (M=21.5 years, ?=2.3) performed a random generation task involving letters and a simple reaction time psychomotor test over four sessions held at 10-hour intervals. Each participant was assigned a "constant routine." Participants were kept awake in a prone position within a room whose environment was held strictly constant (light, noise, temperature, meals, etc.). This control procedure provided assurance that any variation in participant performance was solely caused by sleep deprivation. The random generation task, nearly two minutes in length, consisted in verbally producing a sequence of 100 letters in a random fashion (i.e. by inhibiting, for example, alphabetical order) and by keeping to a set rhythm... (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
35.
Bile acids as constituents for dental composites: in vitro cytotoxicity of (meth)acrylate and other ester derivatives of bile acids. 下载免费PDF全文
Marc A Gauthier Pierre Simard Zhao Zhang X X Zhu 《Journal of the Royal Society Interface》2007,4(17):1145-1150
Methacrylic derivatives of bile acids have been synthesized for use as monomers in dental composites. Polymeric dental materials are known to leach cytotoxic unreacted monomers and degradation products. In this study, the in vitro cytotoxicity of bile acids and their derivatives towards 3T3 fibroblasts has been evaluated by colorimetric MTT assay and compared with that of the common dental monomers BisGMA, UDMA and TEGDMA. In general, the bile acids and their derivatives induced mitochondrial dysfunction at similar or higher concentrations than the commercial dental monomers. Certain monomers did not influence MTT response over their entire range of solubility. 相似文献
36.
37.
Careful combination of a metal compound,a ligand and an inorganic support material leads to supramolecular catalysts that mimic the structural, organizational and functional aspects of enzyme activity.After discussing essential features of metalloenzyme-catalyzed reactions and coordination chemistry in inorganic hosts, we present examples of supramolecular materials selected from our own work that eventually resulted in useful catalysts for organic transformations in the liquid phase. 相似文献
38.
Swaminathan Sivasubramanian Guillaume Pierre Maarten van Steen Gustavo Alonso 《Internet Computing, IEEE》2007,11(1):60-66
Developers often use replication and caching mechanisms to enhance Web application performance. The authors present a qualitative and quantitative analysis of state-of-the art replication and caching techniques used to host Web applications. Their analysis shows that selecting the best mechanism depends heavily on data workload and requires a careful review of the application's characteristics. They also propose a technique for Web practitioners to compare different mechanisms' performance on their own 相似文献
39.
40.
Résumé Cet article présente un modèle permettant de calculer le fluage de poutres fléchies de différentes sections soumises à des
environnements variables en ce qui concerne l'humidité relative. Ce modèle est utilisé ici pour interpréter de nouveaux essais
à long terme sur des poutres en bois massif et lamellé-collé qui ont été chargées pendant plus de 800 jours en conditions
extérieures sous abri à Paris
Summary Long term bending experiments on full size timber and glulam beams have been carried out under external and sheltered climatic conditions in Paris, and more than two years of test results on the creep behaviour of 75 beams are available. A model for predicting the long term mechanical behaviour of timber under variable humidity and load conditions, previously developed by the author, is described. The model is based on transient moisture transfer analysis linked with deformation analysis using a step-by-step computation scheme, and has been compared previously with experiments carried out under laboratory conditions of controlled variable climates by the author as well as with test results obtained from several other institutions. In general, the model has agreed satisfactorily with the experimental results. In the present paper the model is compared with experiments on full size beams carried out under the changeable conditions of a natural climate. The results show that, for low stress levels and corresponding loads, the model provides a reasonable prediction of the end creep levels after two years of loading.相似文献