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Alexandra Manos‐Turvey Esther M. M. Bulloch Dr. Peter J. Rutledge Dr. Edward N. Baker Prof. J. Shaun Lott Dr. Richard J. Payne Dr. 《ChemMedChem》2010,5(7):1067-1079
Mycobacterium tuberculosis salicylate synthase (MbtI), a member of the chorismate‐utilizing enzyme family, catalyses the first committed step in the biosynthesis of the siderophore mycobactin T. This complex secondary metabolite is essential for both virulence and survival of M. tuberculosis, the etiological agent of tuberculosis (TB). It is therefore anticipated that inhibitors of this enzyme may serve as TB therapies with a novel mode of action. Herein we describe the first inhibition study of M. tuberculosis MbtI using a library of functionalized benzoate‐based inhibitors designed to mimic the substrate (chorismate) and intermediate (isochorismate) of the MbtI‐catalyzed reaction. The most potent inhibitors prepared were those designed to mimic the enzyme intermediate, isochorismate. These compounds, based on a 2,3‐dihydroxybenzoate scaffold, proved to be low‐micromolar inhibitors of MbtI. The most potent inhibitors in this series possessed hydrophobic enol ether side chains at C3 in place of the enol‐pyruvyl side chain found in chorismate and isochorismate. 相似文献
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Burns Shaun Michael; Boyd Briana L.; Hill Justin; Hough Sigmund 《Canadian Metallurgical Quarterly》2010,55(1):81
Objective: To explore the relationship between employment status and community access, perceived community discrimination, social support from significant others, depressive symptoms, and gender-related variables for 83 men living with spinal cord injury. Study Design: Correlational research. Setting: Internet-based investigation employing spinal cord injury listservs. Main Outcome Measure: Participant employment status. Results: A forced-entry hierarchical logistic regression indicated that means of injury, community access and perceived community discrimination, social support from significant others, depressive symptoms, and men’s adherence to masculine norms for primacy of work, self-reliance, and emotional control significantly predicted employment status. Conclusions: Psychosocial variables such as community access, perceived discrimination, social support from significant others, depressive symptoms, and gender identity represent important and understudied predictors of employment status among men living with spinal cord injury. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
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Shaun P. Gaus Martin P. Harmer Helen M. Chan Hugo S. Caram Nils Claussen 《Journal of the American Ceramic Society》2000,83(7):1599-1605
The general reaction behavior of the 3A process under the thermal explosion mode of synthesis has been investigated via a continuum model. The continuum model uses mass and energy balances to predict temperature difference ( T s,avg − T f ) curves, as well as profile curves of the reactant conversions and sample temperature. In particular, the effect of the dimensionless parameters associated with the rate of local heat generation (β, the thermicity factor), the activation energy (γ, the Arrhenius number), the rate of heat redistribution (α, the modified thermal diffusivity), the rate of heat transfer by convection (Bi, the Biot number or convective heat transfer parameter), and the rate of heat transfer by radiation (Ω, the radiative heat transfer parameter) were investigated. Conditions to control the reaction process, which should produce high-density final products, were determined. It was found that the overall maximum temperature may be reduced for high γ, low β, high α, and high Bi and Ω. In terms of processing conditions, this may be obtained by reducing the initial reactant concentrations, optimizing the particle size, using small sample sizes and high compaction pressure, and increasing the heat loss by using a high thermal conductivity inert gas. 相似文献
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Vecera Shaun P.; Vogel Edward K.; Woodman Geoffrey F. 《Canadian Metallurgical Quarterly》2002,131(2):194
Figure-ground assignment is an important visual process; humans recognize, attend to, and act on figures, not backgrounds. There are many visual cues for figure-ground assignment. A new cue to figure-ground assignment, called lower region, is presented: Regions in the lower portion of a stimulus array appear more figurelike than regions in the upper portion of the display. This phenomenon was explored, and it was demonstrated that the lower-region preference is not influenced by contrast, eye movements, or voluntary spatial attention. It was found that the lower region is defined relative to the stimulus display, linking the lower-region preference to pictorial depth perception cues. The results are discussed in terms of the environmental regularities that this new figure-ground cue may reflect. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
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An important issue in attention research concerns the representational format from which attention selects. S. P. Vecera and M. J. Farah (see record 1994-32352-001) presented results that they argued demonstrated attentional selection from a spatially invariant object representation. In their comment, A. F. Kramer, T. A. Weber, and S. E. Watson (see record 84-18014) questioned the interpretation of these results, and they presented evidence consistent with selection from a grouped location-based representation. In this reply, the author argues that although an absence of spatial, or distance, effects may be ambiguous as to whether attention is selecting from an object-based representation or from a location-based representation, there are computational considerations that favor object-based selection in certain tasks. The author concludes with a discussion of how object-based and location-based representations might interact with one another, thereby providing a possible explanation of Kramer et al.'s results. Such an account may lead to an understanding of how multiple forms of attentional selection may coexist in the visual system. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
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Does spatial attention follow a full preattentive analysis of the visual field, or can attention select from ungrouped regions of the visual field? We addressed this question by testing an apperceptive agnosic patient, J. W., in tasks involving both spatial selection and preattentive grouping. Results suggest that J. W. had intact spatial attention: He was faster to detect targets appearing at cued locations relative to targets appearing at uncued locations. However, his preattentive processes were severely disrupted. Gestalt grouping and symmetry perception, both thought to involve preattentive processes, were impaired in J. W. Also, he could not use gestalt grouping cues to guide spatial attention. These results suggest that spatial attention is not completely dependent on preattentive grouping processes. We argue that preattentive grouping processes and spatial attention may mutually constrain one another in guiding the attentional selection of visual stimuli but that these 2 processes are isolated from one another. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
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Grouzet Frederick M. E.; Kasser Tim; Ahuvia Aaron; Dols José Miguel Fernández; Kim Youngmee; Lau Sing; Ryan Richard M.; Saunders Shaun; Schmuck Peter; Sheldon Kennon M. 《Canadian Metallurgical Quarterly》2005,89(5):800
The authors investigated the structure of goal contents in a group of 1,854 undergraduates from 15 cultures around the world. Results suggested that the 11 types of goals the authors assessed were consistently organized in a circumplex fashion across the 15 cultures. The circumplex was well described by positing 2 primary dimensions underlying the goals: intrinsic (e.g., self-acceptance, affiliation) versus extrinsic (e.g., financial success, image) and self-transcendent (e.g., spirituality) versus physical (e.g., hedonism). The circumplex model of goal contents was also quite similar in both wealthier and poorer nations, although there were some slight cross-cultural variations. The relevance of these results for several theories of motivation and personality are discussed. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
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