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51.
Alexandre Chmel Alexy Krivda Ekatherina Mazurina Victor Shashkin Valery Zhizhenkov 《Journal of the American Ceramic Society》1993,76(6):1563-1567
The gel-to-glass transition in SiO2 xerogels prepared by inorganic sol-gel synthesis was studied. The evolution of the molecular structure is traced using the infrared and lowfrequency Raman spectroscopy methods. The elastic moduli of the samples as well as the pore wall moduli at various stages of heat treatment are determined from the data on Brillouin scattering. The formation of monolithic glass on the macroscopic level manifests itself within a narrow temperature range by the dramatic increase of Young's modulus to the accepted value for fused silica. This phenomenon coincides with structural transformations on the molecular scale: (i) the definite correlation radius (the long-range order sphere) appears; (ii) local distortions of the silica network relax. The presence of structural defects influences the kinetics of vitreous SiO2 formation during xerogel heat treatment. 相似文献
52.
Carl Yuheng Ren Victor Prisacariu Ian Reid 《International Journal of Computer Vision》2014,106(3):269-281
We propose a novel regression based framework that uses online learned shape information to reconstruct occluded object contours. Our key insight is to regress the global, coarse, properties of shape from its local properties, i.e. its details. We do this by representing shapes using their 2D discrete cosine transforms and by regressing low frequency from high frequency harmonics. We learn this regression model using Locally Weighted Projection Regression which expedites online, incremental learning. After sufficient observation of a set of unoccluded shapes, the learned model can detect occlusion and recover the full shapes from the occluded ones. We demonstrate the ideas using a level-set based tracking system that provides shape and pose, however, the framework could be embedded in any segmentation-based tracking system. Our experiments demonstrate the efficacy of the method on a variety of objects using both real data and artificial data. 相似文献
53.
Dr. Christoph Goebel Prof.?Dr. Hans-Arno Jacobsen Victor del Razo Mag.? Christoph Doblander Dipl.-Ing. Jose Rivera Dipl-Inform.?Wirt Jens Ilg Dr. Christoph Flath Prof.?Dr. Hartmut Schmeck Prof.?Dr. Christof Weinhardt Dipl-Inform. Daniel Pathmaperuma Prof.?Dr. Dr.?h.?c. Hans-Jürgen Appelrath Prof.?Dr. Michael Sonnenschein Prof.?Dr. Sebastian Lehnhoff Prof.?Dr. Oliver Kramer Prof.?Dr. Thorsten Staake Prof.?Dr. Elgar Fleisch Prof.?Dr. Dirk Neumann Prof.?Dr. Jens Strüker Dr. Koray Erek Prof.?Dr. Rüdiger Zarnekow Dr. Holger Ziekow Prof.?Dr. J?rg L?ssig 《WIRTSCHAFTSINFORMATIK》2014,56(1):31-39
Due to the increasing importance of producing and consuming energy more sustainably, Energy Informatics (EI) has evolved into a thriving research area within the CS/IS community. The article attempts to characterize this young and highly dynamic field of research by describing current EI research topics and methods and provides an outlook of how the field might evolve in the future. It is shown that two general research questions have received the most attention so far and are likely to dominate the EI research agenda in the coming years: How to leverage information and communication technology (ICT) to (1) improve energy efficiency, and (2) to integrate decentralized renewable energy sources into the power grid. Selected EI streams are reviewed, highlighting how the respective research questions are broken down into specific research projects and how EI researchers have made contributions based on their individual academic background. 相似文献
54.
Filiberto González Garcia Bluma G. Soares Victor J. R. R. Pita Rubén Sánchez Jacques Rieumont 《应用聚合物科学杂志》2007,106(3):2047-2055
The mechanical properties of epoxy networks based on diglycidyl ether of bisphenol A epoxy resin cured with various linear aliphatic amines, such as ethylenediamine, diethylenetriamine, triethylenetetramine, tetraethylenepentamine, and cyclic amines such as 1‐(2‐aminoethyl)piperazine and isophorone diamine, were studied. General characteristics such as Tg, density, and packing density, were determined and related to the structure and funcionality of the curing agent. Dynamic mechanical spectra were used to study both the α and β relaxations. Tensile and the flexural tests were used to determine the Young's and flexural modulus, and fracture strength all in the glassy state. Furthermore, linear elastic fracture mechanics was used to determine KIC. As a rule, isophorone diamine network presented the higher tensile and flexure modulus while 1‐(2‐aminoethyl)piperazine gave the highest toughness properties. © 2007 Wiley Periodicals, Inc. J Appl Polym Sci 2007 相似文献
55.
Victor T. Wyatt Alberto Nuñez Thomas A. Foglia William N. Marmer 《Journal of the American Oil Chemists' Society》2006,83(12):1033-1039
Novel oligomeric prepolymers were synthesized by acid-catalyzed condensation of glycerol with iminodiacetic, azelaic, or succinic
acid. The prepolymers were obtained, on average, in 62% yield and were characterized by 13C NMR, 1H NMR, matrix-assisted laser desorption ionization-time of flight-mass spectrometry, and gel permeation chromatography. The
synthesized oligomers had an average M.W. of 1543 Daltons (average polydispersity (PD)=1.34, average degree of polymerization
(DOP)=5.5). Hyperbranching was evident in the oligomers produced when using azelaic acid and succinic acid as co-monomers
with glycerol, whereas the reaction between iminodiacetic acid and glycerol resulted in linear products bearing cyclic urethane
structures. 相似文献
56.
Strong polyelectrolytes, known as superplasticizers, improve the initial fluidity of concentrated cement suspensions through electrostatic stabilization. These polyelectrolytes do not maintain the initial fluidity, however, primarily due to an increase in the ionic strength of the cementitious suspension. Consequently, non-ionic polymers are often used in conjunction with polyelectrolytes to provide steric stabilization and hence to sustain the desired fluidity over a longer time, and this has lead to the development of copolymers with both electrostatic and steric (electrosteric) functionalities. To design such polymers, it is necessary to optimize the balance between electrostatic and steric stabilization to maximize suspension fluidity. We have quantified the effects of a strong anionic polyelectrolyte, melamine formaldehyde sulfonate (MFS), and a non-ionic polymer, hydroxypropylmethylcellulose (HPMC), on the zeta potential of cement particles and the steady shear and low-amplitude rheological properties of concentrated cement suspensions. While the adsorption of MFS onto the cement particle surfaces leads to a sign inversion in the zeta potential, the adsorption of the non-ionic HPMC has no significant effect on the potential. The addition of HPMC to the suspensions substantially reduces the steady shear viscosity and the storage modulus at constant MFS concentration; in addition, there exists an intermediate HPMC concentration that minimizes fluidity. The resulting suspension fluidity is also maintained over a longer time than in the absence of HPMC. This improvement in the stability and fluidity of cement suspensions is attributed to “complementary electrosteric dispersion/stabilization”, and provides insight to the design of polymers with electrosteric functionality. 相似文献
57.
58.
We present an algorithm that stylizes an input video into a painterly animation without user intervention. In particular, we focus on pointillist animation with stable temporal coherence. Temporal coherence is an important problem in non-photorealistic rendering for videos. To realize pointillist animation, the various characters of pointillism should be considered in painting process to maintain temporal coherence. For this, weused the particle video algorithm which is a new approach to long-range motion estimation in video. Based on this method, we introduce a method to control the density of particles considering the features of frames and importance maps. Finally, the propagation methods of stroke to minimize flickering effects of brush strokes are introduced. 相似文献
59.
Gregory B. Furman Shaul D. Goren Victor M. Meerovich Vladimir L. Sokolovsky 《Quantum Information Processing》2014,13(12):2759-2768
We study behavior of quantum discord, a kind of quantum correlation, in systems of dipole–dipole interacting spins in an external magnetic field in the whole temperature range ( \(-\infty ). It was shown that negative temperatures, which are introduced to describe inversions in the population in a finite level system, provide more favorable conditions for emergence of quantum correlations including entanglement. We show that at negative temperature, the correlations become more intense and discord exists between remote spins being in separated states. 相似文献
60.
Maria Helena de Oliveira Nunes Victor Teixeira da Silva Martin Schmal 《Catalysis Letters》2004,97(1-2):1-8
There is a high industrial demand for MMA and DMA, however, the production of TMA is favored with the commercial catalysts. This work tested the methanol amination reaction with HZSM-5 and Cu/HZSM-5 zeolites (%Cu = 1.2, 3.7 and 6.0). Regarding the MMA selectivity, light differences were observed among Cu/HZSM-5 catalysts and pure zeolite, although the catalysts containing 3.7% copper was slightly more selective to MMA than the other metallic catalysts studied. From these results it is suggested that the metal loading present in the catalysts leads to a modification in the nature of the acidic sites, in particular, the selectivity depends on ratio Brönsted/Lewis acid sites. This modifications would facilitate the amines desorption during the reaction. 相似文献