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991.
Younggeun Lee Jinhyeong Kwon Jaemook Lim Wooseop Shin Sewoong Park Eunseung Hwang Jaeho Shin Hyunmin Cho Jinwook Jung Hyun-Jong Kim Seungyong Han Habeom Lee Yong Son Cheol Woo Ha Prem Prabhakaran Junyeob Yeo Seung Hwan Ko Sukjoon Hong 《Advanced functional materials》2021,31(1):2006854
Structural coloration is closely related to the progress of innovative optoelectronic applications, but the absence of direct, on-demand, and rewritable coloration schemes has impeded advances in the relevant area, particularly including the development of customized, reprogrammable optoelectronic devices. To overcome these limitations, a digital laser micropainting technique, based on controlled thin-film interference, is proposed through direct growth of the absorbing metal oxide layer on a metallic reflector in the solution environment via a laser. A continuous-wave laser simultaneously performs two functions—a photothermal reaction for site-selective metal oxide layer growth and in situ real-time monitoring of its thickness—while the reflection spectrum is tuned in a broad visible spectrum according to the laser fluence. The scalability and controllability of the proposed scheme is verified by laser-printed painting, while altering the thickness via supplementary irradiation of the identical laser in the homogeneous and heterogeneous solutions facilitates the modification of the original coloration. Finally, the proof-of-concept bolometer device verifies that specific wavelength-dependent photoresponsivity can be assigned, erased, and reassigned by the successive application of the proposed digital laser micropainting technique, which substantiates its potential to offer a new route for reprogrammable optoelectronic applications. 相似文献
992.
Min Ju Kim Changhyeon Lee Eui Joong Shin Tae In Lee Seongho Kim Jaejoong Jeong Junhwan Choi Wan Sik Hwang Sung Gap Im Byung Jin Cho 《Advanced functional materials》2021,31(41):2103291
With the recent interest in data storage in flexible electronics, highly reliable charge trap-type organic-based non-volatile memory (CT-ONVM) has attracted much attention. CT-ONVM should have a wide memory window, good endurance, and long-term retention characteristics, as well as mechanical flexibility. This paper proposed CT-ONVM devices consisting of band-engineered organic–inorganic hybrid films synthesized via an initiated chemical vapor deposition process. The synthesized poly(1,3,5-trimethyl-1,3,5,-trivinyl cyclotrisiloxane) and Al hybrid films are used as a tunneling dielectric layer and a blocking dielectric layer, respectively. For the charge trapping layer, different Hf, Zr, and Ti hybrids are examined, and their memory performances are systematically compared. The best combination of hybrid dielectric stacks showed a wide memory window of 6.77 V, good endurance of up to 104 cycles, and charge retention of up to 71% after 108 s even under the 2% strained condition. The CT-ONVM device using the hybrid dielectric stacks outperforms other organic-based charge trap memory devices and is even comparable in performance to conventional inorganic-based poly-silicon/oxide/nitride/oxide/silicon structures devices. The CT-ONVM using hybrid dielectrics can overcome the inherent low reliability and process complexity limitations of organic electronics and expedite the realization of wearable organic electronics. 相似文献
993.
Ramanaskanda Braveenth Hyuna Lee Jae Doh Park Ki Joon Yang Soon Jae Hwang Kenkera Rayappa Naveen Raju Lampande Jang Hyuk Kwon 《Advanced functional materials》2021,31(47):2105805
Simultaneously obtaining high efficiency and deep blue emission in organic light emitting diodes (OLEDs) remains a challenge. To overcome the demands associated with deep blue thermally activated delayed fluorescence (TADF) emitters, two deep blue TADF materials namely, DBA–BFICz and DBA–BTICz, are designed and synthesized by incorporating oxygen-bridged boron (DBA) acceptor with heteroatoms, oxygen and sulphur-based donors, BFICz and BTICz, respectively. Both TADF materials show deep blue photoluminescence emissions below 450 nm by enhancing the optical band gap over 2.8 eV through deeper highest occupied molecular orbital (HOMO) level of heteroatom based donor moieties. At the same time, the photoluminescence quantum yields (PLQYs) of both TADF materials remain over 94%. The TADF device with DBA–BFICz as an emitter exhibits a good external quantum efficiency (EQE) of 33.2%. Since both new TADF materials show deep blue emissions and high efficiencies, hyperfluorescence (HF) OLED devices are fabricated using ν-DABNA as a fluorescence dopant. DBA–BFICz as a TADF sensitized host in HF–OLED reveals an outstanding EQE of 38.8% along with narrow full width at half maximum of 19 nm in the bottom emission pure blue OLEDs. This study provides an approach to develop deep blue TADF emitters for highly efficient OLEDs. 相似文献
994.
Minho Seong Insol Hwang Seongjin Park Hyejin Jang Geonjun Choi Jaeil Kim Shin-Kwan Kim Gun-Ho Kim Junyeob Yeo Hoon Eui Jeong 《Advanced functional materials》2021,31(48):2107023
Minimizing the thermal contact resistance (TCR) at the boundary between two bodies in contact is critical in diverse thermal transport devices. Conventional thermal contact methods have several limitations, such as high TCR, low interfacial adhesion, a requirement for high external pressure, and low optical transparency. Here, a self-interfacing flexible thermal device (STD) that can form robust van der Waals mechanical contact and low-resistant thermal contact to planar and non-planar substrates without the need for external pressure or surface modification is presented. The device is based on a distinctive integration of a bioinspired adhesive architecture and a thermal transport layer formed from percolating silver nanowire (AgNW) networks. The proposed device exhibits a strong attachment (maximum 538.9 kPa) to target substrates while facilitating thermal transport across the contact interface with low TCR (0.012 m2 K kW−1) without the use of external pressure, thermal interfacial materials, or surface chemistries. 相似文献
995.
This paper presents a finite element solution to the problem of low Peclet number fluid flow in the thermal entrance region of a round pipe. The velocity is assumed to be laminar and fully developed throughout the pipe and the fluid temperature is kept uniform atX = —∞. The pipe wall is adiabatic at X ≤ 0 and cooled convectively at X ≥ 0. The solutions include temperature distributions and Nusselt numbers for the parameters, Bi = 0.04, 0.4, 4, 20 and Pe = 1, 3, 5, 10, 20, 30, which are in excellent agreement with the existing analytic solution except in the region near the singular point Δ A temperature discrepancy in the analytic solution at this point is physically impossible. The finite element method overcomes this mathematical difficulty and shows a greater value in the Nusselt number due to a higher wall temperature at X ≥ 0. 相似文献
996.
Hyun Gyu Kim Dong Won Hwang Sang Won Bae Jong Hyeon Jung Jae Sung Lee 《Catalysis Letters》2003,91(3-4):193-198
Highly donor-doped (110) layered perovskite materials, La2Ti2O7, with high surface areas were synthesized by the polymerizable complex (PC) method. Relative to La2Ti2O7 prepared by the solid state reaction (SSR) method, PC catalysts showed higher surface areas, crystallization at lower temperatures, higher phase purity, more uniform morphology and better-distributed nickel on the outer surface of La2Ti2O7. All these factors led to higher photocatalytic activity for overall water splitting under UV irradiation. The quantum yield of the reaction over La2Ti2O7 prepared by the PC method was as high as 27%, which was about twofold greater than that over La2Ti2O7 prepared by the SSR method. 相似文献
997.
Hyung Joon Cha Kyoung Ro Kim Byeong Hee Hwang Dae Hee Ahn Young Je Yoo 《Korean Journal of Chemical Engineering》2007,24(5):812-815
Glucoamylase that hydrolyses starch to glucose is one of the important industrial enzymes for ethanol production industry.
Therefore, genetic production of recombinant glucoamylase has been widely studied. Previously, we reported secreted production
of Saccharomyces diastaticus-originated glucoamylase in Saccharomyces cerevisiase expression system using its own signal sequence and the SUC2 promoter that is regulated by glucose level in culture medium. In the present work, we performed a comparative study between
batch and fed-batch bioreactor cultures for secreted production of recombinant glucoamylase. Through maintaining low glucose
levels in the culture broth, we obtained about 7-fold higher secreted production levels of glucoamlyase in fed-batch culture.
Fed-batch culture strategy also enhanced (∼3.1-fold) secretion efficiency of recombinant glucoamylase in S. cerevisiae. 相似文献
998.
Reducing steel slag (RSS) was mainly acquired from five electric-arc furnace (EAF) steelmaking plants (among them, the products
of two plants were carbon steel and those of other plants were stainless steel) for research tests. The chemical properties,
compound compositions, activities and contents of main expansive compounds were tested. The results showed that the field
sampled RSS had a very high crystallinity and hydraulicity with main chemical compositions close to those of Portland cement.
It can be known from the study that in case of C/S ratio higher than 2.0, the main compound compositions are C2S, C3S, C2F and f-CaO. However, after the RSS was stored for six months, an obvious variation occurred with potential pre-hydration in RSS,
where the SO3 content was slightly reduced and the compressive activity index was obviously higher than that at the 28th day. 相似文献
999.
Humic acid, a natural organic matter, was separated with a polyamide (PA) composite membrane with a molecular weight cutoff (MWCO) of 500 g/mol. The PA composite membrane was prepared by the interfacial polymerization of piperazine and trimesoyl chloride on a polysulfone support with an MWCO of about 30,000 g/mol. The separation conditions through the membrane were varied, and factors affecting the permeation performance of the membranes, such as the concentration, pH, and storage time of the humic acid solutions, were studied. The surface chemistry of the membrane changed dynamically as a function of the operating time during the permeation tests, and the size and ζ potential of the colloid of humic acid solutions under different conditions were characterized with a ζ potentiometer. © 2002 Wiley Periodicals, Inc. J Appl Polym Sci 86: 2847–2853, 2002 相似文献
1000.
The preparation of poly(vinyl alcohol) (PVA) fibers by multi-step drawing was examined. The high draw ratio was attained when the drawing just before melting point was repeated. The influences of the draw ratio on mechanical and thermal properties of the fibers were studied. We utilized the wide angle x-ray diffraction (WAXD) as a medium to observe the erystallinity and the orientation of PVA fibers to study their effects on the physical properties of the fibers. With various coagulation bath concentration, both the tenacity and Young's modulus of fibers would increase as the draw ratios increased, the elongation would decrease at the same time. The tenacity was able to reach 41.0 cN/tex with the Young's modulus being 856.2 cN/tex; also, as the draw ratios increased, both crystallinity and orientation would increase. The crystallinity was about 67.2 % and the orientation was about 86.4%. 相似文献