Lithium metal batteries (LMBs), due to their ultra-high energy density, are attracting tremendous attentions. However, their commercial application is severely impeded by poor safety and unsatisfactory cycling stability, which are induced by lithium dendrites, side reactions, and inferior anodic stability. Electrolytes, as the indispensable and necessary components in lithium metal batteries, play a crucial role in regulating the electrochemical performance of LMBs. Recently, the fluorinated electrolytes are widely investigated in high-performance LMBs. Thus, the design strategies of fluorinated electrolytes are thoroughly summarized, including fluorinated salts, fluorinated solvents, and fluorinated additives in LMBs, and insights of the fluorinated components in suppressing lithium dendrites, improving anodic stability and cycling stability. Finally, an outlook with several design strategies and challenges will be proposed for novel fluorinated electrolytes. 相似文献
Neural Computing and Applications - Considering some problems of local linear embedding methods in semi-supervised scenarios, a robust scheme for generating soft labels is designed and a... 相似文献
The Industrial Internet of Things is crucial for enterprise and country to drive the strategic upgrade and raise the level of national intelligent manufacturing. When pondering the IIoT industry evaluation, the corresponding dominating issues involve numerous indeterminacies. Spherical fuzzy set, portrayed by memberships of positive, neutral and negative, is a more efficient methods of seizing indeterminacy. In this article, firstly, the fire-new spherical fuzzy score function is explored for solving some suspensive comparison issues. Moreover, the objective weight and combined weight are determined by Renyi entropy method and non-linear weighted comprehensive method, respectively. Later, the multi-criteria decision making method based on combined compromise solutionis developed under spherical fuzzy environment. Finally, the corresponding method is effectively validated by the issue of IIoT industry evaluation. The main characteristics of the presented algorithm are: (1) without counterintuitive phenomena; (2) no division or antilogarithm by zero problem; (3) no square root by negative number issue; (4) no violation of the original definition issue.
Due to air turbulence, large areas of coal will fall when the special coal-transportation trains pass the tunnel exits and entrances. Aiming at the problems of low efficiency and high cost of manual cleaning for long distance coal cleaning in the tunnel, a new railway tunnel fallen coal dust collection device which was composed of a main conveying coal feeding pipe and multiple branch pipes of coal suction was designed. It was used to clean the small particles and lightweight railway tunnel fallen coal. Firstly, the gas-solid two-phase flow model based on the Euler-Lagrange approach for the design of the main conveying coal feeding pipe was established in the coal conveying pipelines. Secondly, the effect of the coal particles' incident angle and multiple branch pipe spacing on the main coal conveying pipe flow field, which was based on Fluent finite element simulation software, was studied. What was more, the optimal angle of incidence and the optimal value of the number of branch coal suction pipe, which was installed on the main conveying pipe, were analyzed. Finally, the finite element simulation was verified by field test. Simulation and experimental results showed that it was more conducive to the railway tunnel fallen coal transportation when coal particles' incident angle was less than 45° and the branch pipe spacing was in the vicinity of 750 mm. For that when incident angle was less than 45°, the main conveying coal pipe pressure-drop became weaker and particle flow could obtain large horizontal transport velocity. And when the branch pipe spacing was in the vicinity of 750 mm, the horizontal transport velocity had a smaller fluctuation range and the transportation of coal was larger than that of the other groups. The research results are of great significance to improve the structure of the main conveying coal pipe, increase the efficiency of tunnel coal conveying and optimize the railway tunnel coal dust collection device. 相似文献