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991.
UV‐Triggered Polydopamine Secondary Modification: Fast Deposition and Removal of Metal Nanoparticles
Yi Zeng Xin Du Wei Hou Xiaojiang Liu Cun Zhu Bingbing Gao Liangdong Sun Qiwei Li Junlong Liao Pavel A. Levkin Zhongze Gu 《Advanced functional materials》2019,29(34)
Since the first report in 2007, polydopamine (PDA) coating has shown great potential as a general and versatile method to create functional nanocoatings on arbitrary substrates. Slow kinetics and poor controllability of the coating and secondary modification processes, however, have limited the further development of this attractive method. In this work, it is demonstrated that UV irradiation at 365 nm significantly accelerates the process of secondary modification of a PDA‐coated surface. The kinetics of both thiol and amine modifications of PDA are increased 12‐fold via UV irradiation, while the kinetics of metal ion reduction at the PDA interface is increased more than 550 times. Moreover, it is demonstrated that irradiating a PDA/metal nanoparticle composite surface with UV light at 254 nm leads to dissolution of the deposited metal nanoparticles (MNPs). Finally, grayscale metallic patterns, dynamic deposition, and removal of MNPs on PDA surface are realized with the proposed method. 相似文献
992.
Zhanwei Zhou Yadong Liu Minghua Zhang Chenzi Li Ruoxi Yang Jing Li Chenggen Qian Minjie Sun 《Advanced functional materials》2019,29(39)
Protein‐based theranostic agents (PBTAs) exhibit superior performance in the diagnosis and therapy of cancers. However, the in vivo applications of PBTA are largely limited by undesired accumulation, penetration, or selectivity. Here, an ATP‐supersensitive protein cluster is fabricated for promoting PBTA delivery and enhancing magnetic resonance imaging (MRI)‐guided tumor photothermal therapy. Gd3+‐ and CuS‐coloaded small bovine serum albumin nanoparticles (GdCuB) are synthesized as the model protein with a size of 9 nm and are encapsulated into charge switchable polycations (DEP) to form DEP/GdCuB nanoclusters of 120 nm. In blood circulation, DEP/GdCuB significantly extends the half‐lifetime and thereby enhances the tumor accumulation of GdCuB. When the clusters reach the tumor site, the extracellular adenosine triphosphate (ATP) can effectively trigger the release of GdCuB, resulting in tumoral deep penetration as well as the activation of T1‐weighted MRI (r1 value switched from 2.8 × 10?3 to 11.8 × 10?3 m ?1 s?1). Furthermore, this delivery strategy also improves the tumoral photothermal therapy efficacy with the MRI‐guided therapy. The study of ATP‐activated nanoclusters develops a novel strategy for tumor deep penetration and on/off imaging of PBTA by size switchable technology, and reveals the potential for MRI‐guided therapy of cancers. 相似文献
993.
Fog radio access network (F‐RAN) architectures provide markedly improved performance compared to conventional approaches. In this paper, an efficient genetic algorithm‐based content distribution scheme is proposed that improves the throughput and reduces the transmission delay of a F‐RAN. First, an F‐RAN system model is presented that includes a certain number of randomly distributed fog access points (F‐APs) that cache popular content from cloud and other sources. Second, the problem of efficient content distribution in F‐RANs is described. Third, the details of the proposed optimal genetic algorithm‐based content distribution scheme are presented. Finally, simulation results are presented that show the performance of the proposed algorithm rapidly approaches the optimal throughput. When compared with the performance of existing random and exhaustive algorithms, that of the proposed method is demonstrably superior. 相似文献
994.
混合pin/肖特基(MPS)二极管是广泛应用于电子电路中的快恢复功率器件,具有高击穿电压、快速开关和正向电流大等特性。对MPS二极管漂移区的少数载流子的特性进行了仿真分析。仿真结果表明,MPS二极管的p^+区向漂移区注入的少数载流子浓度随外加正向电压和pn结面积占元胞总面积比例的增大而增大。虽然漂移区的少数载流子改变了MPS二极管的工作模式,增大了电流,但是存储在漂移区的少数载流子增大了反向峰值电流和恢复时间,进而增大了功耗并降低了关断速度。折中考虑正向电流和反向恢复特性,可获得具有正向电流大、反向峰值电流小和反向恢复时间短的MPS二极管。 相似文献
995.
To progressively provide the competitive rate-distortion performance for aerial imagery,a quantized block compressive sensing(QBCS) framework is presented,which incorporates two measurement-side control parameters:measurement subrate(S) and quantization depth(D).By learning how different parameter combinations may affect the quality-bitrate characteristics of aerial images,two parameter allocation models are derived between a bitrate budget and its appropriate parameters.Based on the corresponding allocation models,a model-guided image coding method is proposed to pre-determine the appropriate(S,D) combination for acquiring an aerial image via QBCS.The data-driven experimental results show that the proposed method can achieve near-optimal quality-bitrate performance under the QBCS framework. 相似文献
996.
Xiaowu He Yifeng Song Ying Yu Ben Ma Zesheng Chen Xiangjun Shang Haiqiao Ni Baoquan Sun Xiuming Dou Hao Chen Hongyue Hao Tongtong Qi Shushan Huang Hanqing Liu Xiangbin Su Xinliang Su Yujun Shi Zhichuan Niu 《半导体学报》2019,40(7):27-37
A brief introduction of semiconductor self-assembled quantum dots (QDs) applied in single-photon sources is given. Single QDs in confined quantum optical microcavity systems are reviewed along with their optical properties and coupling characteristics. Subsequently, the recent progresses in In(Ga)As QDs systems are summarized including the preparation of quantum light sources, multiple methods for embedding single QDs into different microcavities and the scalability of single-photon emitting wavelength. Particularly, several In(Ga)As QD single-photon devices are surveyed including In(Ga)As QDs coupling with nanowires, InAs QDs coupling with distributed Bragg reflection microcavity and the In(Ga)As QDs coupling with micropillar microcavities. Furthermore, applications in the field of single QDs technology are illustrated, such as the entangled photon emission by spontaneous parametric down conversion, the single-photon quantum storage, the chip preparation of single-photon sources as well as the single-photon resonance-fluorescence measurements. 相似文献
997.
998.
光纤表面等离子体共振(SPR)传感器是目前应用在环境介质检测和生物大分子检测等方面的新型、高精度传感器。首先,以表面等离子体共振传感理论为基础,对系统检测结果进行数据处理,得出采用均值估计的线性模型。在不同时刻与相同环境介质下,检测某一溶液的十组光谱数据并进行均值估计,从而得到有效的共振波长。其次,利用小波分析方法进行信号处理,校正了噪声产生的漂移,对光谱信号压缩处理,以提高检测精度。再通过Matlab进行模拟仿真优化传感系统性能。并对不同折射率溶液如蒸馏水、酒精等进行检测,得到了良好的光谱响应曲线,证明了在检测范围内折射率和共振波长之间具有良好的线性关系。 相似文献
999.
近场支付由于其产业链过长、相关硬件厂商众多的特点,给其兼容性带来了巨大挑战.在NFC一致性测试的基础上,提出了严格的一致性测试、仪表兼容性测试、R/W兼容性测试、POS兼容性测试等4种提高NFC终端与POS之间兼容性的测试方法,并分析了其优缺点.行业相关方可结合自身资源及需求,采用其中一种或几种方法相结合的测试手段,提高NFC端到端兼容性,优化NFC支付生态环境. 相似文献
1000.
The sixth generation(6G)of wireless cellular networks is expected to incorporate the latest developments in network infrastructure and emerging advances in technology.In the age of 6G,edge caching technology will evolve towards intelligence,dynamics,and security.However,the security problems of edge caching,including data tampering and eavesdropping,are seldomly considered in most literatures.In this paper,we consider the two-hop edge caching where the blockchain and physical layer security technologies are adopted to prevent data from being tampered with and eavesdropped.We design blockchain-based framework to guarantee the reliability of important data such as the frequency of contents and jointly optimize content caching probability and redundancy rate to maximize the secure transmission probability.Extensive simulation shows that our optimization scheme can significantly improve the secure transmission probability of edge cache network,whether facing the threat of independent eavesdropping or joint eavesdropping. 相似文献