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991.
CeO2–ZrO2–La2O3 (CZL) mixed oxides were prepared by citric acid sol–gel method. The as-received gel was calcined at 500, 700, 900 and 1050 °C to obtain the so-called C5, C7, C9 and CK, respectively. The C5, C7 and C9 powders were impregnated with H2PtCl6 and then calcined at 500 °C to prepare P5C5, P5C7 and P5C9, respectively. The impregnated CK powders were calcined at 500, 700 and 900 °C to prepare P5CK, P7CK and P9CK, respectively. The XRD and XPS analyses show that the surface distribution of Pt is evidently influenced by the structural and textural properties of the support. The CO adsorption followed by FTIR reveals that the dispersion and the chemisorption sites of Pt are reduced as the calcination temperature of CZL support increases. The chemisorption ability of the CK samples is even completely deactivated. The encapsulation mechanism, which has been applied to explain the so-called strong metal–support interaction (SMSI) after reductive treatment, is introduced here to demonstrate the abnormal observations though the samples were prepared in oxidative atmosphere. The HRTEM results also confirm this explanation. The effects of oxygen vacancies, the chemisorption sites on the Pt surface and Pt/Ce interfacial sites on the three-way catalytic activities are discussed. 相似文献
992.
Graft copolymerization of acrylic acid (AA) onto polyphenylene sulfide (PPS) nonwoven initiated by low temperature plasma was studied. The effects of various conditions on graft reaction and the grafting rate were investigated. SEM images showed that PPS nonwoven was grafted, and the graft copolymerization only occurred on the surface of PPS. It may be due to the chain transference going with the graft copolymerization. It was found that with the increasing of plasma power, treatment time, space between electrodes, monomer concentration, and temperature of graft polymerization, the grafting rate increased at first, went to the top, and then decreased. The PPS nonwoven surface graft reaction could be optimized by the following processing conditions: 120 s of plasma treatment time, 50 W of plasma power, 1.5 cm of space between electrodes, 30% (w/w) of monomer concentration, and 50°C of temperature of graft polymerization. Measurement of XPS showed that the peak of C1s of graft polyacrylic acid was existed, and the peak area increased with the increase of the grafting rate. © 2006 Wiley Periodicals, Inc. J Appl Polym Sci 102: 5884–5889, 2006 相似文献
993.
Song-Ya Ma Ming-Xing Luo Xiu-Bo Chen Yi-Xian Yang 《Quantum Information Processing》2014,13(9):1951-1965
Two schemes via different entangled resources as the quantum channel are proposed to realize remote preparation of an arbitrary four-particle \(\chi \) -state with high success probabilities. To design these protocols, some useful and general measurement bases are constructed, which have no restrictions on the coefficients of the prepared states. It is shown that through a four-particle projective measurement and two-step three-particle projective measurement under the novel sets of mutually orthogonal basis vectors, the original state can be prepared with the probability 50 and 100 %, respectively. And for the first scheme, the special cases of the prepared state that the success probability reaches up to 100 % are discussed by the permutation group. Furthermore, the present schemes are extended to the non-maximally entangled quantum channel, and the classical communication costs are calculated. 相似文献
994.
Jakobi et al. for the first time proposed a novel and practical quantum private query (QPQ) protocol based on SARG04 (Scarani et al. in Phys Rev Lett 92:057901, 2004) quantum key distribution protocol (Jakobi et al. in Phys Rev A 83:022301, 2011). Gao et al. generalized Jakobi et al’s protocol and proposed a flexible QPQ protocol (Gao et al. in Opt Exp 20(16):17411–17420, 2012). When $\theta <\pi /4$ , Gao et al’s protocol exhibits better database security than Jakobi et al’s protocol, but has a higher probability with which Bob can correctly guess the address of Alice’s query. In this paper, we propose a flexible B92-based QPQ protocol. Although SARG04 protocol is a modification of B92 protocol and can be seen as a generalization of B92 protocol, our protocol shows different advantages from Gao et al’s protocol. It can simultaneously obtain better database security and a lower probability with which Bob can correctly guess the address of Alice’s query when $\theta <\pi /4$ . By introducing entanglement, the proposed QPQ protocol is robust against channel-loss attack, which also implies lower classical communication complexity. Similar to Gao et al’s protocol, it is flexible, practical, and robust against quantum memory attack. 相似文献
995.
The compound architecture of CMAC (Cerebellar Model Articulation Controller) and PD (Proportional-Derivative) can effectively reduce the loading error and restrain the surplus torque of electric load simulators. But due to its generalization ability, the CMAC controller has an unsmooth output, which leads to the motor vibration even the divergence of control system. The unsmooth problem of CMAC is analyzed in this paper and a novel scalar cost function of CMAC is proposed, which consists of an error item and a weight smoothing item to guarantee fast learning capacity and improved output smoothness of CMAC. With the novel scalar cost function, a compound torque controller of PD and smooth CMAC is derived by using the gradient descent algorithm. Both the simulation and experimental results demonstrate that the novel CMAC-PD compound controller can effectively improve the output smoothness of the electric load simulator, eliminate the surplus torque and assure the stability of system as well. 相似文献
996.
Hao Yang Bin Jiang Youmin Zhang 《International Journal of Control, Automation and Systems》2014,12(1):29-36
This paper studies the fault tolerant formation keeping problem of multi-agent systems with consideration of shortest connection topology. This is motivated by the requirement of low communication cost which largely depends on the communication length. Given a formation shape, a connection topology design method and its reconfiguration strategy are proposed in the sense that the whole connection path is shortest despite of communication faults. A control framework that combines the individual formation controller of each agent and connection topology is further presented. The stability of the whole system process is analyzed by switched system theories. Simulation results of unmanned aerial vehicles (UAVs) show the effectiveness of the proposed strategy. 相似文献
997.
In reliability-based structural analysis and design optimization, there exist some limit state functions exhibiting disjoint failure domains, multiple design points and discontinuous responses. This study addresses this type of challenging problem of reliability assessment of structures with complex limit state functions based on the probability density evolution method (PDEM). Probability density function (PDF) of stochastic structures under static and dynamic loads can be acquired, which is independent of the specific form of limit state functions. Numerical results of several typical examples illustrate that, the time-invariant and instantaneous PDF curves and failure probabilities of stochastic structures with disjoint failure domains, multiple design points and discontinuous responses are calculated effectively and accurately. Moreover, the PDEM is validated to be more efficient than the Monte Carlo simulation and the subset simulation, and is a feasible and general approach to tackle the reliability analysis of complicated problems. In addition, the influence of random design parameters of structures on uncertainty propagation is also scrutinized. 相似文献
998.
Guang-yu Zhu Gao-na Lu Chen-Guang Yang Peng Zhang 《Personal and Ubiquitous Computing》2014,18(8):1955-1961
Unified judgment standards and methods are often adopted to identify traffic state in certain road network based on traffic flow parameters. However, drivers often have different perceptions about the traffic state on different road sections, since their expectations on traffic state vary more or less from each other on different road sections. In particular, under the vehicle networking, out of considerations for safety and other relevant factors, requirements for the correlation and coordination of running vehicles have also raised significantly. Therefore, it is necessary to take driver’s perception about the driving conditions of certain road sections into consideration to adjust the release of traffic state. This paper has provided a comprehensive traffic state evaluation model linked with driver’s perception under the vehicle networking. The authors first establish an ANFIS model based on the T–S model and then conduct statistical analysis on drivers’ perceptions about certain traffic state. At last, the authors use the results of statistical analysis as regulatory factors to amend the parameters input through ANFIS. Through simulation, this paper has demonstrated that the model established has a high rate of convergence, a high identification precision and the generalization ability to conduct researches on the identification of traffic state. 相似文献
999.
1000.