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971.
Hydrogen atom adsorption and diffusion properties on clean and vacancy defective Mg (0001) surface have been investigated
systematically by using a first-principles calculations method based on the density functional theory. The calculation results
of adsorption energy and diffusion energy barrier show that hydrogen atom is apt to be adsorbed at fcc and hcp sites on clean
Mg (0001) surface, and fcc adsorption site is found to be more preferred. The highest diffusion energy barrier is estimated
as 0.6784 eV for the diffusion of hydrogen from clean Mg (0001) surface into its bulk. Surface effects, which affect hydrogen
diffusion obviously, results in a slow diffusion velocity of hydrogen from surface to subsurface, while a fast one from subsurface
to bulk, indicating the range of surface effects is only restricted within two topmost layers of Mg (0001) surface. Comparatively,
Mg atom vacancy on Mg (0001) surface not only enhances the chemisorption interaction between H and Mg surface, but also benefits
H atom diffusion in Mg bulk with relatively more diffusion paths compared with that of clean surface. Besides, hydrogen atom
is found to occupy mostly the tetrahedral interstice when it diffuses into the Mg bulk. Further analysis of the density of
states (DOS) shows that the system for hydrogen atom to be adsorbed at fcc site has a lower DOS value (N (E
F)) at Fermi level and more bonding electrons at the energy range blow the Fermi level of H/Mg (0001) system as compared with
that at hcp site. On the other hand, the enhanced chemisorption interaction between hydrogen and defective surface should
be attributed to the fact that the electronic structures of Mg (0001) surface are modified by an Mg vacancy, and the bonding
electrons of the topmost layer Mg atoms are transferred from low energy range to Fermi level, which is in favor of improving
the surface activity of Mg (0001) surface.
Supported by the PhD Programs Foundation of Ministry of Education of China (Grant No. 200805321032), the Science and Technology
Program Project of Hunan Province (Grant No. 2008GK3083) and the Program for Changjiang Scholars and the Innovative Research
Team in university (Grant No. 531105050037) 相似文献
972.
GUAN Ping LIU ChangChun & Lü HeXiang College of Architectural Engineering Dalian University Dalian China State Key Laboratory of Structural Analysis for Industrial Equipment Dalian University of Technology Dalian 《中国科学E辑(英文版)》2009,52(5):1248-1253
The traditional unified viscoplasticity constitutive model can be only applied to metal materials. The study of the unified
constitutive theory for metal materials has discovered the correlation between the classical plasticity theory and the unified
viscoplasticity constitutive model, thus leading to the concepts of the classic plastic potential and yield surface in the
unified constitutive model. Moreover, this research has given the continuous expression of the classical plastic multiplier
and presented the corresponding constructive method, which extends its physical significance and lays down a good foundation
for the application of the unified constitutive theory to the material analysis in more fields. This paper also introduces
the unified constitutive model for metal materials and geo-materials. The numerical simulation indicates that the construction
should be both reasonable and practical.
Supported by the National Natural Science Foundation of China (Grant No. 90410012) 相似文献
973.
974.
表面三维形貌测量及其评定的研究 总被引:1,自引:0,他引:1
对表面三维形貌测量技术展开了较为全面的研究,测量过程由相移,采样,相位提取及数据处理等部分组成.整个测量系统采用激光为干涉光源,CCD为图像传感器,压电陶瓷提供微小位移,通过图像采集卡将干涉条纹采集到计算机内存.文中采用上述理论对标准样块进行了测量,计算机得到表面三维形貌图,根据建立的基准面分离出粗糙度信息,并由给出的参数评定数学模型,编制出合理的软件,计算出零件表面的三维参数.最后给出实验结果和分析,并提出下一步研究工作的设想. 相似文献
975.
采用微波辐射法改性胶粉,用苯乙烯对其进行溶胀,并通过平衡溶胀率、接触角、衰减全反射红外光谱及扫描电镜等研究微波改性对胶粉的交联度、表面润湿性、化学结构、表面形貌等的影响。结果表明,微波法打断了胶粉中部分S—S和C—S键,使得胶粉交联度降低,易于被苯乙烯溶胀;另外,微波辐射使得胶粉表面发生氧化,极性基团增多,因此使胶粉表面亲水性提高。 相似文献
976.
纳米聚丙烯酸酯微乳液改性纳米CaCO3研究 总被引:1,自引:0,他引:1
分别采用聚丙烯酸酯乳液和纳米级聚丙烯酸酯微乳液对纳米CaCO3进行改性,通过红外光谱分析、热重分析和扫描电镜分析研究改性纳米CaCO3的结构和性能。结果表明,改性后的纳米CaCO3由亲水疏油性变为亲油疏水性,纳米级聚丙烯酸酯微乳液与纳米CaCO3粒子表面发生了化学反应,并包覆到纳米CaCO3粒子表面。 相似文献
977.
978.
979.
980.