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991.
《International Journal of Hydrogen Energy》2021,46(78):38854-38870
The pyrolysis and combustion mechanism of the hydrocarbon fuel has important scientific and practical significance. However, it is difficult to detect the whole intermediates and products using traditional methods, which brings trouble to the analysis of the reaction process. In this paper, the microscopic reaction mechanism and the main products of n-eicosane (C20H42) were simulated based on the reactive force field molecular dynamics (ReaxFF-MD). The effects of temperature (2000–3500 K) and oxygen on the initial decomposition, the distribution of main products, and the reactive pathways of C20H42 fuel were studied to determine its reaction mechanism. The initial decomposition of C20H42 was mainly initiated by small alkyl radicals in pyrolysis, and by the oxygen-containing radicals in combustion. The participation of oxygen had a greater effect on accelerating the decomposition reaction. The reactions involving oxygen of C20H42 initial decomposition accounted for 87.5% of the total reactions at 2000 K. Moreover, the detailed distribution and formation pathways of the main products of H2, C2H4, CH4, H2O, CO, and CO2 were depicted to construct the overall reaction mechanism of C20H42. •H radical formed from the composition of C2H4 was exactly consistent with the •H radical consumed by the generation of CH4 and H2 in the pyrolysis stage. The feasibility of the simulation method was verified by the result of thermal analysis. The results are helpful for further research on the reaction mechanism of hydrocarbon fuels. 相似文献
992.
The current study examined the self-excited thermoacoustic instability of hydrogen/methane premixed flames using a variable-length combustor (300–1100 mm). The global dynamic pressure, heat release rate oscillation, together with the flame dynamics were studied. Results showed that both the hydrogen concentration and the chamber length were critical in determining the acoustic oscillation mode and instability trend. Low-frequency primary acoustic modes (<200 Hz) were mainly excited when the hydrogen concentration was low, whereas primary acoustic modes with relatively higher frequencies (~400 Hz) tended to occur in cases with a high hydrogen proportion (>40%). For primary acoustic modes lower than 200 Hz, the primary oscillation frequency tended to increase linearly with a rising hydrogen proportion. Heat release oscillation and flame dynamics analyses demonstrated that for the flame with large-scale shape deformation, the initial addition of hydrogen would intensify the heat release oscillation. Nevertheless, a further increase in the hydrogen level tended to inhibit the heat release oscillation by weakening the flame shape deformation. Eventually, a sufficient high-level of hydrogen addition would weaken the primary acoustic modes that have similar frequencies. 相似文献
993.
Runze Mao Jinhua Wang Weijie Zhang Zhenhua An Wenjun Lin Meng Zhang Zuohua Huang 《International Journal of Hydrogen Energy》2021,46(34):17969-17981
In this study, we investigated the H2-induced transition of confined swirl flames from the “V” to “M” shape. H2-enriched lean premixed CH4/H2/air flames with H2 fractions up to 80% were conducted. The flame structure was obtained with Planar Laser-Induced Fluorescence (PLIF) of the OH radical. Flow fields were measured with Particle Image Velocimetry (PIV). It was observed that the flame tip in the outer shear layer gradually propagated upstream and finally anchored to the injector with the hydrogen fractions increase, yielding the transition from the “V” to “M” flame. We examined the flame structures and the flame flow dynamics during the transition. The shape transition was directly related to the evolution of the corner flame along the outer shear layer. With H2 addition, the outer recirculation zone first appeared downstream where the corner flame started to propagate upstream; then, the recirculation zone expanded upward to form a stable “M” flame gradually. The flow straining was observed to influence the stabilization of the outer shear layer flame significantly. This study can be useful for the understanding of recirculation-stabilized swirling flames with strong confinement. The flame structure and the flow characteristics of flames with a high H2 content are also valuable for model validation. 相似文献
994.
Yosuke Abe Tomohito Tsuru Shi Shi Naoko Oono Shigeharu Ukai 《Journal of Nuclear Science and Technology》2016,53(10):1528-1534
Various types of nanometric defects such as voids and helium (He) bubbles produced by high-energy neutron irradiations are known to degrade the mechanical properties of irradiated materials. In this study, we have evaluated the obstacle strength of He bubbles to the mobility of an edge dislocation in α-iron for 2 and 4 nm bubbles with He-to-vacancy (He/V) ratios ranging from 0 to 1 at 300 and 500 K, by molecular dynamics simulation. Results showed that as the He/V ratio increases, the obstacle strength needed for the release of a dislocation from the bubble becomes stronger up to a moderate He/V ratio (0.6 and 0.4 for 2 and 4 nm bubbles, respectively, at both temperatures), and a further increase in the He/V ratio leads to weakening of the obstacle strength. For He/V = 1, the obstacle strengths are 10–30% weaker than those at moderate He/V ratios depending on the bubble size and temperature. The extent of obstacle strength was found to be correlated with the dilation caused by He bubbles depending on the bubble size, He/V ratio, and temperature. 相似文献
995.
《国际计算机数学杂志》2012,89(5):1013-1023
This article deals with the peristaltic flow of a Sisko fluid in an endoscope. The inner tube of the endoscope is fixed, while outer tube is flexible. Continuity and momentum equations are utilized in the mathematical analysis and obtained both the analytical and numerical solutions. The analytical solution has been found by the homotopy analysis method and the numerical solutions are carried out by the shooting technique. The comparison of both the solutions are presented. And the quantitative behaviours of the solutions are discussed. 相似文献
996.
《Current Opinion in Solid State & Materials Science》2013,17(6):271-276
For this article, we call scientific software a community code if it is freely available, written by a team of developers who welcome user input, and has attracted users beyond the developers. There are obviously many such materials modeling codes. The authors have been part of such efforts for many years in the field of atomistic simulation, specifically for two community codes, the LAMMPS and GULP packages for molecular dynamics and lattice dynamics respectively. Here we highlight lessons we have learned about how to create such codes and the pros and cons of being part of a community effort. Many of our experiences are similar, but we also have some differences of opinion (like modeling vs modelling). Our hope is that readers will find these lessons useful as they design, implement, and distribute their own materials modelling software for others to use. 相似文献
997.
998.
We report a course-grained, large scale simulation of the outer membrane from Pseudomonas aeruginosa. Using the MARTINI force field approach of 4-to-1 atom mapping, we simulate an asymmetrically constructed bilayer with over 1100 rough lipopolysaccharide (LPS) and 3100 16:0-18:1-phosphatidylethanolamine. We achieve 90-fold improvement in computational efficiency on a system much larger than reasonable for all-atom simulation. We also compare a coarse-grained LPS/LPS bilayer simulation with known parameters determined from neutron diffraction. 相似文献
999.
Two-dimensional (2D) pressure field estimation in molecular dynamics (MD) simulations has been done using three-dimensional (3D) pressure field calculations followed by averaging, which is computationally expensive due to 3D convolutions. In this work, we develop a direct 2D pressure field estimation method which is much faster than 3D methods without losing accuracy. The method is validated with MD simulations on two systems: a liquid film and a cylindrical drop of argon suspended in surrounding vapor. 相似文献
1000.
Alessio Alexiadis 《International journal for numerical methods in engineering》2014,100(10):713-719
In this work, a hybrid numerical approach, which combines elements of SPH and coarse‐grained molecular dynamics, is used to investigate the effect of various flow conditions to deformable and breakable shell‐structures such as capsules, vesicles or biological cells. Copyright © 2014 John Wiley & Sons, Ltd. 相似文献