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61.
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利用燃烧合成工艺原位合成了TiB2-Cu基复合材料,为了改善TiB2陶瓷和Cu基体的润湿性,将金属Ni作为合金化元素加入到TiB2-Cu复合材料。通过XRD,SEM,EPMA和TEM等检测手段对金属Ni的添加对TiB2-Cu基复合材料微观组织的影响进行了研究。结果表明,含Ni复合材料的金属粘结相的面间距比不含Ni时Cu的面间距均有不同程度的减小;Ni加入后,TiB2-Cu-Ni复合材料的组织较TiB2-Cu复合材料更加致密,但陶瓷颗粒尺寸却大于TiB2-Cu复合材料的颗粒尺寸;Ni的加入降低了复合材料的导热率和冷却速度,使得部分TiB2陶瓷颗粒有足够的时间长成棒状,同时造成TiB2陶瓷颗粒间形成更多的烧结颈;Ni的加入也改善了陶瓷与金属粘结相之间的润湿性,使陶瓷相与金属粘结相的界面结合牢固,看不到TiB2-Cu复合材料中界面脱开的现象。金属Ni的添加有利于改善TiB2-Cu基复合材料的微观组织,进而利于复合材料的致密化。 相似文献
63.
As an alternative to previously developed catalytic FeCrAlloy fibre mat burners based on perovskite catalysts, new catalytic burners have been developed based on Pd catalyst on lantana-stabilised Al2O3 and different fibre structures (NIT100A, NIT100S and NIT200S by ACOTECH NV). All development steps are considered, shifting from catalyst preparation (based on combustion synthesis of γ-Al2O3) to the optimisation of lantana and Pd loadings, from the definitions of the best catalyst-deposition conditions (washcoating) to the catalytic burners performances, determined in an ad hoc developed combustion chamber. The results show almost half pollutants emissions and better performance compared to various non-catalytic counterparts, especially as far as CO and NOx emissions are concerned. Some flame instability problems were though registered, especially for one of the catalytic burner mattresses employed, at low specific power inputs and excesses of air (<375 kW/m2 and <12%, respectively). Further, PdO/Pd transition is shown to influence the dynamic behaviour of the catalytic burners. 相似文献
64.
The catalytic activity of fresh Pd and Pt catalysts supported on γ-alumina in the complete oxidation of CH4 traces under lean-burn conditions was studied in the presence or the absence of water or H2S. Steam-aged catalysts were also studied in order to simulate long-term ageing in real lean-burn natural gas fuelled vehicles (NGVs) exhaust conditions. Without water or H2S added to the feed, Pd catalysts exhibit a superior catalytic activity in methane oxidation compared to Pt ones, whatever the catalysts were fresh or aged. The addition of 10 vol.% water vapour to the feed strongly affects the activity of the fresh Pd catalyst, thus being only slightly more efficient than the fresh Pt one. H2S has a strong poisoning effect on the catalytic activity of Pd catalysts, while Pt catalysts are more resistant. The fresh H2S-poisoned Pd/Al2O3 catalyst was studied by TPD in O2/He. Poisoning species decompose above 873 K as SO2 and O2 in relative concentrations consistent with the decomposition of surface sulphate species. However, a treatment in O2/He at temperatures as high as 923 K does not allow the complete regeneration of the catalytic activity of H2S-poisoned Pd/Al2O3. A mechanism involving the poisoning of PdO by sulphate species is proposed. Different diffusion processes by which these sulphate species can migrate back and forth between PdO and the support, depending on the experimental conditions, are suggested. 相似文献
65.
P. S. Lawson 《Biomass & bioenergy》1992,2(1-6):319-330
In recent years it has been recognised by an increasing number of nations that there is considerable energy potential within MSW. As a result many countries have established R,D& D programmes to examine methods of exploiting this potential. The IEA's MSW Conversion Activity was set up in 1986 to provide an infrastructure for sharing information and co-ordinating work in this area internationally. This Activity was extended in 1989 and currently a total of 9 nations participate in it.
To cope with the wide scope of the area (encompassing both biological and thermal processing of MSW) the Activity was divided into three subgroups or Expert Working Groups (EWGs). Each of these dealt with a distinct area of expertise:
- 1. •Downstream effects of source separation and screening of MSW
- 2. •Sampling and analytical protocols
- 3. •Landfill gas
In addition to these groups a central secretariat based at Harwell (UK) has provided guidance, established and administered databases of contacts and produced a series of national reports.
This paper describes the achievements of the Activity and discusses work proposed for the future. 相似文献
66.
67.
Atilla Bilgin 《国际能源研究杂志》2002,26(11):987-1000
Flame front surface area and enflamed volume (the volume enclosed with flame front) is theoretically analysed for a spark‐ignition engine, having cylindrical disc‐shaped combustion chamber with two spark plugs located axisymmetrically on cylinder head, between cylinder axis and cylinder wall. Spherical flame front assumption is used. A computer code is developed based on purely geometric consideration of the flame development process in combustion chamber, and is used to investigate the effects of variations of spark plugs' locations on geometric features of the flame front. A comparison has also been made with a spark‐ignition engine having one spark plug at the same location. Copyright © 2002 John Wiley & Sons, Ltd. 相似文献
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