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Isotopic transient techniques were applied to study oxidative coupling of methane over lanthanum oxide and strontium promoted La2O3 catalysts. Results of the18O2/16O2 isotopic exchange experiments indicate that Sr promotion increases oxygen uptake from the lattice of the catalyst. Oxygen self diffusion coefficients, which were determined for the series of lanthana catalysts, reach a maximum for the 1% Sr/La2O3. Steps of18O2 in the presence of a steady flow of methane over Sr/La2O3 catalysts, indicate that surface and bulk oxygen appear in the reaction products before gas-phase18O2. Steps of CO2 over catalysts in which lattice oxygen has been exchanged with18O2, show that gas/solid exchange involves over 50% of the lattice oxygen. Under reaction conditions, methane pulses with no gas-phase oxygen yield negligible amounts of products which indicates that methane interacts with lattice oxygen only in the presence of the gas-phase oxygen. 相似文献
23.
ZHANG YuJun ZHANG WeiQing & YANG ChaoShuai State Key Laboratory of Geomechanics Geotechnical Engineering 《中国科学:信息科学(英文版)》2011,(7)
With the models of stress corrosion and pressure solution, by Yasuhara et al., two computation conditions were designed for a hypothetical nuclear waste repository in an unsaturated dual-porosity rock mass: (i) the fracture apertures are changed with the stress corrosion and pressure solution (the porosity of rock matrix is also a function of stress); (ii) the fracture apertures and the porosity of rock matrix are constants. Then the corresponding two-dimensional FEM analyses for the coupled thermohydro-mec... 相似文献
24.
军工院校大学文化与大学发展耦合度评价实证分析 总被引:1,自引:0,他引:1
大学文化在现代大学发展中的作用越来越突出,已成为提升大学核心竞争力的重要因素,越来越多的大学把大学文化建设作为学校建设的重要组成部分.因此,大学文化建设的效果评价十分重要.通过建立"大学文化与大学发展耦合度"评价模型,对军工院校大学文化建设的效果进行实证分析.结果表明,哈尔滨工程大学的大学文化与大学发展之间的耦合度较高,耦合作用较强,大学文化在促进学校自觉肩负服务国防使命、实现自身发展目标中的作用明显,大学文化系统与大学发展系统之间呈正相关关系. 相似文献
25.
针对现有冻结站盐水流量和温度控制方法存在控制精度低的问题,提出了一种盐水流量和温度的模糊解耦控制方法。首先根据盐水流量和温度控制精度的不同,采用模糊控制法对流量和温度进行模糊控制;然后分析和研究盐水流量和温度间的耦合关系,采用解耦控制法对模糊控制输出的流量和温度进行解耦控制。仿真结果表明,该控制方法无需对盐水流量和温度建立精确数学模型,可实现盐水流量和温度的解耦控制,控制精度高。 相似文献
26.
Toshiaki Fukuhara 《Polymer》2004,45(3):843-847
New thermosetting poly(2-allyl-6-methylphenol-co-2,6-dimethylphenol)s (3) have been developed by oxidative coupling copolymerization of 2-allyl-6-methylphenol (1) with 2,6-dimethylphenol (2), followed by thermal curing. Copolymerization was conducted in nitrobenzene in the presence of copper(I) chloride and pyridine as the catalyst under a stream of oxygen, producing high molecular weight copolymers (Mn∼50,000) with broad molecular weight distributions (Mw/Mn∼35). The structure of resulting copolymers 3 was characterized by IR, 1H, and 13C NMR spectroscopy. Cross-linking reactions of copolymers were carried out by thermal treatment in the absence or presence of a peroxide (3 wt%, 2,5-dimethyl-2,5-di(tert-butylperoxy)-3-butane). The 10% weight loss and glass transition temperatures of the cured copolymers were 436 °C in nitrogen and 235 °C, respectively after curing at 70 °C for 1 h and 300 °C for 1 h. The average refractive index of the cured copolymer (3b) film was 1.5407, from which the dielectric constant (ε) at 1 MHz was estimated as 2.6. The ε and dissipation factor of copolymer-films at 1 MHz were directly measured from their capacitances as 2.5-2.6 and 0.0015-0.0019, respectively. 相似文献
27.
This paper is concerned with the synchronization problem about linear singularly perturbed complex network system with coupling delay. The sufficient delay-dependent conditions for the synchronization of the network are established by introducing an equivalent network system with the Lyapunov stability theory. These conditions, which are formulated in terms of linear matrix inequalities, can be solved efficiently by the LMI toolbox of MATLAB. A simulation example is provided to show the validity of the proposed the synchronization conditions of the whole network. 相似文献
28.
29.
为了减少感应加热对电磁清蜡器腔管的热蚀,提高电磁清蜡器的使用寿命,在分析油井电磁清蜡器感应加热过程的基础上,利用ANSYS的APLD语言建立了电磁清蜡器的电磁热耦合场有限元模型.重点对油井电磁清蜡器处理腔管中的电磁—热耦合场进行了仿真分析,得出了腔管内外壁的温度分布规律.仿真结果表明:电磁感应加热5s,钢管表面温度升高至175.128℃;加热10s钢管表面温度达到了343.286℃,避免了常规电阻式加热钢管明显的温升滞后现象,体现了电磁感应加热的升温速度快的特点,20s后钢管内的温度分布比较均匀,钢管总体温度在490~ 569℃的范围内,钢管内壁与钢管表面温差在77.323℃以下. 相似文献
30.
The design and test of dual/triple‐mode bandpass filter based on temporal coupled‐mode theory 下载免费PDF全文
Hui Xu Jiong‐Jiong Mo Xiu‐Qin Xu Xu Ding Zhi‐Yu Wang Yong‐Heng Shang Li‐Ping Wang Fa‐Xin Yu 《国际射频与微波计算机辅助工程杂志》2016,26(7):609-622
In this article, the design and test of both a K‐band dual‐mode bandpass filter (BPF) pair and a K‐band triple‐mode BPF are presented based on N‐mode temporal coupled‐mode theory (CMT). The expressions of transmission and reflection responses are analytically derived. All the parameters in the expressions have clear physical meanings and are easily optimized to reach the required filter performance. Aided by eigenmode simulations, concrete structures of the three integrated BPFs are designed and optimized to approach the calculated physical parameters. After the fabrications and measurements of the three BPFs, extended upper/lower stopband with high stopband rejections are achieved, and by increasing the number of resonant modes, improved frequency selectivity and better passband flatness are obtained. The analytical analysis well predicts the simulation and measurement results, which provides an efficient way for BPF designs. © 2016 Wiley Periodicals, Inc. Int J RF and Microwave CAE 26:609–622, 2016. 相似文献