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991.
该文对盒中脑(BSB)神经网络在超立方体内的平衡点的渐近稳定性进行了新的分析,利用Ostrowski定理及相似变换得到了判定平衡点为渐近稳定的几个充分条件。为了说明所提出新方法的有效性,给出了模拟例子。 相似文献
992.
993.
在传感器节点受到能量和带宽严重制约的情况下,如何合理、有效地利用有限的资源来采集有效、可信的数据,成为当前无线传感器网络(Wireless Sensor Network,WSN)研究的热点问题之一。在分析了大量WSN感知数据的基础上,利用时间序列对数据进行建模处理,得出了适合WSN的数据处理模型ARMA(1,1),同时利用基于移动Agent的中间件技术,提出了基于ARMA的无线传感器网络可信数据采集方法。理论和实验结果表明,该方法可保证采集数据的高度可信,同时显著提高了网络的整体性能,有效的减少网络的能耗,延长了网络的生命周期。 相似文献
994.
Ruidong Xia Wen‐Yong Lai Peter A. Levermore Wei Huang Donal D. C. Bradley 《Advanced functional materials》2009,19(17):2844-2850
Here, a detailed characterization of the optical gain properties of sky‐blue‐light‐emitting pyrene‐cored 9,9‐dialkylfluorene starbursts is reported; it is shown that these materials possess encouragingly low laser thresholds and relatively high thermal and environmental stability. The materials exhibit high solid‐state photoluminescence (PL) quantum efficiencies (>90%) and near‐single‐exponential PL decay transients with excited state lifetimes of ~1.4 ns. The thin‐film slab waveguide amplified spontaneous emission (ASE)‐measured net gain reaches 75–78 cm?1. The ASE threshold energy is found to remain unaffected by heating at temperatures up to 130 °C, 40 to 50 °C above Tg. The ASE remained observable for annealing temperatures up to 170 or 200 °C. 1D distributed feedback lasers with 75% fill factor and 320 nm period show optical pumping thresholds down to 38–65 Wcm?2, laser slope efficiencies up to 3.9%, and wavelength tuning ranges of ~40 nm around 471–512 nm. In addition, these lasers have relatively long operational lifetimes, with N1/2 ≥ 1.1 × 105 pulses for unencapsulated devices operated at ten times threshold in air. 相似文献
995.
996.
We investigate the thermal stability of HfTaON films prepared by physical vapor deposition using high resolution transmission electronic microscope (HRTEM) and X-ray photoelectron spectroscopy (XPS). The results indicate that the magnetron-sputtered HtTaON films on Si substrate are not stable during the post-deposition an-healing (PDA). HfTaON will react with Si and form the interfacial layer at the interface between HfTaON and Si substrate. Hf-N bonds are not stale at high temperature and easily replaced by oxygen, resulting in significant loss of nitrogen from the bulk film. SiO2 buffer layer introduction at the interface of HfTaON and Si substrate may effec-tively suppress their reaction and control the formation of thicker interfacial layer. But SiO2 is a low k gate dielectric and too thicker SiO2 buffer layer will increase the gate dielectric's equivalent oxide thickness. SiON prepared by oxidation of N-implanted Si substrate has thinner physical thickness than SiO2 and is helpful to reduce the gate dielectric's equivalent oxide thickness. 相似文献
997.
A New Design Paradigm for Smart Windows: Photocurable Polymers for Quasi‐Solid Photoelectrochromic Devices with Excellent Long‐Term Stability under Real Outdoor Operating Conditions 下载免费PDF全文
Federico Bella George Leftheriotis Gianmarco Griffini George Syrrokostas Stefano Turri Michael Grätzel Claudio Gerbaldi 《Advanced functional materials》2016,26(7):1127-1137
A new photoelectrochromic device (PECD) is presented in this work proposing the combination of a WO3‐based electrochromic device (ECD) and a polymer‐based dye‐sensitized solar cell (DSSC). In the newly designed architecture, a photocurable polymeric membrane is employed as quasi‐solid electrolyte for both the ECD and the DSSC. In addition, a photocurable fluoropolymeric system is incorporated as solution‐processable external protective thin coating film with easy‐cleaning and UV‐shielding functionalities. Such new polymer‐based device assembly is characterized by excellent device operation with improved photocoloration efficiency and switching ability compared with analogous PECDs based on standard liquid electrolyte systems. In addition, long‐term (>2100 h) stability tests under continuous exposure to real outdoor conditions reveal the remarkable performance stability of this new quasi‐solid PECD system, attributed to the protective action of the photocurable fluorinated coating that effectively prevents photochemical and physical degradation of the PECD components during operation. This first example of quasi‐solid PECD systems paves the way for a new generation of thermally, electrochemically, and photochemically stable polymer‐based PECDs, and provides for the first time a clear demonstration of their true potential as readily upscalable smart window components for energy‐saving buildings. 相似文献
998.
Diffused Phase Transition Boosts Thermal Stability of High‐Performance Lead‐Free Piezoelectrics 下载免费PDF全文
Fang‐Zhou Yao Ke Wang Wook Jo Kyle G. Webber Timothy P. Comyn Jing‐Xuan Ding Ben Xu Li‐Qian Cheng Mu‐Peng Zheng Yu‐Dong Hou Jing‐Feng Li 《Advanced functional materials》2016,26(8):1217-1224
High piezoelectricity of (K,Na)NbO3 (KNN) lead‐free materials benefits from a polymorphic phase transition (PPT) around room temperature, but its temperature sensitivity has been a bottleneck impeding their applications. It is found that good thermal stability can be achieved in CaZrO3‐modified KNN lead‐free piezoceramics, in which the normalized strain d 33* almost keeps constant from room temperature up to 140 °C. In situ synchrotron X‐ray diffraction experiments combined with permitivity measurements disclose the occurrence of a new phase transformation under an electrical field, which extends the transition range between tetragonal and orthorhombic phases. It is revealed that such an electrically enhanced diffused PPT contributed to the boosted thermal stability of KNN‐based lead‐free piezoceramics with high piezoelectricity. The present approach based on phase engineering should also be effective in endowing other lead‐free piezoelectrics with high piezoelectricity and good temperature stability. 相似文献
999.
Cisplatin‐Prodrug‐Constructed Liposomes as a Versatile Theranostic Nanoplatform for Bimodal Imaging Guided Combination Cancer Therapy 下载免费PDF全文
Liangzhu Feng Min Gao Danlei Tao Qian Chen Hairong Wang Ziliang Dong Meiwan Chen Zhuang Liu 《Advanced functional materials》2016,26(13):2207-2217
Up to date, a large variety of liposomal nanodrugs have been explored for cancer nanomedicine, showing encouraging results in both preclinical animal experiments and clinical treatment of cancer patients. Herein, a phospholipid conjugated with a cisplatin prodrug is used as the major structure component of liposomes together with other commercial lipids via self‐assembling. By doping with 1,1′‐dioctadecyl‐3,3,3′,3′‐tetramethylindotricarbocyanine iodide (DiR), a lipophilic dye with strong near infrared (NIR) absorbance and fluorescence, the obtained DiR‐Pt(IV)‐liposome is found to be an effective probe for in vivo NIR fluorescence and photoacoustic bimodal imaging. Attributing to its intrinsically doped cis‐Pt(IV) prodrug, efficient photothermal conversion ability, and excellent tumor homing ability, DiR‐Pt(IV)‐liposome confers greatly enhanced therapeutic outcomes in the combined photothermal‐chemotherapy. Moreover, Pt(IV)‐liposome is also demonstrated to be an efficient carrier for both small hydrophilic molecules and proteins, which are encapsulated inside the water‐cavity of liposomes, further demonstrating the versatile functions of this nanoplatform. This study develops a unique type of liposomal nanomedicine with a prodrug conjugated phospholipid as the major structure component. Such Pt(IV)‐liposome is featured with advantages including precisely defined/easily tunable drug compositions, stealth‐like pharmacokinetics, efficient tumor passive uptake, and the capabilities to simultaneously load with various types of imaging or therapeutic agents. 相似文献
1000.
New Drug‐Structure‐Directing Agent Concept: Inherent Pharmacological Activity Combined with Templating Solid and Hollow‐Shell Mesostructured Silica Nanoparticles 下载免费PDF全文
Victoria Morales María Gutiérrez‐Salmerón Moisés Balabasquer Josefa Ortiz‐Bustos Ana Chocarro‐Calvo Custodia García‐Jiménez Rafael A. García‐Muñoz 《Advanced functional materials》2016,26(40):7291-7303
One of the major challenges in medicine is the delivery and control of drug release over time. Current approaches take advantage of mesostructured silica nanoparticles (MSNs) as carriers but suffer several problems including complex synthesis that requires sequential steps for (1) removal of surfactants and (2) functionalization of MSNs to allow upload of the drugs. Here, a novel solution is presented to these restrictions: the design of drug‐structure‐directing agents (DSDAs) with dual inherent pharmacological activity and ability to direct the formation of solid and hollow‐shell MSNs. Pharmacologically active DSDAs obtained by amidation of drugs with fatty acids are allowed to form micelles, around which the inorganic species self‐assembled to form MSNs. Since the DSDAs direct the formation of MSNs, the steps to remove surfactants, functionalization, and drug upload are not required. The MSNs thus prepared provide sustained release of the drug over more than six months, as well as rapid cellular internalization by both physiological and tumoral human colon cells without affecting cell viability. Moreover, the gradual intracellular release of both, the active drug and lipid moiety with potential nutraceutical properties is proved. MSN particles designed with this approach are promising vehicles for controlled and sustained intra‐or extracellular drug‐delivery. 相似文献