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21.
22.
V YakhninM Menzinger 《Chemical engineering science》2002,57(21):4559-4567
In the course of catalytic combustion of hydrogen (1-5% H2 in air) in monolith reactors, strongly localized stationary and traveling hot spots arise in response to a sudden and persistent rise of gas flow velocity. Such hot spots may occur, e.g. in a catalytic converter following the acceleration of a car or in a catalytic combustor as a result of a load increase. This phenomenon is illustrated by simulations using a two-phase reactor model. The temperature overshoot of the adiabatic limit is typically of the order of the adiabatic temperature rise itself.The following mechanism underlies this behavior. Light fuel is supplied to the catalytic wall by fast diffusion (in the direction perpendicular to flow), while the heat released by reaction is removed from the wall by the slower, mixture-averaged heat conduction. This leads to accumulation of heat at the catalytic surface that eventually saturates at high temperatures. The hot spots may exhibit intricate dynamics, propagating downstream or upstream, or they may remain stationary. The direction of propagation depends on the relative strength of convective downstream and conductive upstream contributions to the overall displacement of reaction fronts. Generally, the hot spot tends to drift downstream at low flow velocities, remain stationary at intermediate flow velocities, and drift upstream at high flow velocities. 相似文献
23.
钨铜合金药型罩及其性能 总被引:3,自引:0,他引:3
钨铜合金药型罩的应用可以提高射流对均质钢靶的侵彻能力.这一提高得益于射流密度的提高以及断裂时间的延长. 本文对钨铜合金射流及其断裂形态通过X光照像进行了研究.它的旋转效应及其炸高特性也进行了实验研究. 钨铜合金药型罩的威力实验在φ30 mm的破甲弹上进行.在相同装药条件下与紫铜罩相比,威力提高20~30%. 相似文献
24.
定量电子晶体学硼对Ni3Al的电荷密度分布的影响 总被引:1,自引:0,他引:1
阐述了定量电子晶体学测定晶体电荷密度分布的基本原理和方法,不足之处和改善途径。以硼对Ni3Al的电荷密度分布的影响为实例,介绍了定量电子晶体学在研究晶体电子结构方面的应用前景。 相似文献
25.
F. D. McDaniel B. L. Doyle C. H. Seager D. S. Walsh G. Vizkelethy D. K. Brice C. Yang P. Rossi M. Nigam M. El Bouanani G. V. Ravi Prasad J. C. Schwartz L. T. Mitchell J. L. Duggan 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2002,190(1-4):1-10
A new ion beam analysis-based, single ion technique called the time to first photon has been developed to measure the decay of the luminescence signal of phosphors. Such measurements are currently needed to study luminescence decay mechanisms following high-density excitations and to identify strongly luminescent phosphor coatings with short lifetimes for ion photon emission microscopy (IPEM). The samples for this technique consist of thin phosphor layers placed or coated on the surface of PIN diodes. Single ions from an accelerator strike this sample and simultaneously create ion beam induced luminescence (IBIL) from the phosphor that is measured by a single-photon-detector, and an ion beam induced charge collection (IBICC) signal in the PIN diode. In this case, the IBICC signal provides the start pulse and the IBIL signal the stop pulse to a time to amplitude converter. It is straightforward to show that this approach also measures a signal proportional to activity versus time with an accuracy of 5% as long as the number of detected photons per ion is less than 0.1, which usually requires the use of absorbers for the IBIL detector or electronic discrimination for the IBIL signals. Details of the new analysis are given together with examples of luminescence decay measurements of several ceramic phosphors being considered to coat IPEM samples. IPEM is currently being developed at Sandia National Laboratory (SNL), the University of North Texas in Denton, and the Universities and INFN of Padova and Torino. 相似文献
26.
工程监理取费偏低,阻碍监理行业发展 总被引:1,自引:0,他引:1
工程监理制在我国建筑市场中,对提高工程质量、控制投资效益起着极其重要的作用,目前我国工程监理行业在低取费的条件下,困难重重,只能维持低水平运行。我们应找出存在的差距,采取相应的措施,适当提高监理取费,使监理行业迅速发展壮大。 相似文献
27.
热释电系数的测量方法 总被引:2,自引:0,他引:2
描述热释电系数的两种测量方法。其一为电荷积分法,测试系统简单,测量数据准确,且能满足零电场条件下的测量。其二为动态电流法,采用调制热源技术,研究在特定温度条件下热释电材料的动态热释电响应。 相似文献
28.
The interaction of alkali metal with surfaces has been of great interest to the community of catalysis since alkali metal can play an important role as a promoter. On alkali-doped MoS2, such a promotion effect of alkali metal has been exemplified in the direct synthesis of linear alcohols from CO and H2, where the alkali-doping switches the catalyst selectivity from methanation to alcohol synthesis. This paper reviews recent high-resolution X-ray photoelectron spectroscopy experiments that have provided direct
observation of electron transfer from alkali metals to a model single crystal MoS2 and the capture of the supra-valence electrons in the subsequent oxidation reactions. 相似文献
29.
P. K. Khare J. M. Keller M. S. Gaur Ranjeet Singh S. C. Datt 《Polymer International》1994,35(4):337-343
The electrical conductivity of solution-grown ethyl cellulose (EC) films, 5–30 μm thick, has been studied in the sandwich configuration (metal–EC–metal) as a function of iodine concentration from 0.5 to 5.0 wt% ratio. The studies were conducted in the temperature range 333–383 K, while the field was varied over the range (3.0–5.5) × 104V/cm. Aluminium was used as the lower electrode, while the upper electrode was of Al, Ag, Cu, Au or Sn. Certain transient effects such as a large burst of current immediately after the application of field were observed. An attempt was made to identify the nature of the current by comparing the observed dependence on electric field, electrode material and temperature with the respective characteristic features of the existing theories of electrical conduction. The results show that the electrical conduction follows Ohm's law at lower fields, while at higher fields, space-charge limited current (SCLC) was observed. It was also found that Richardson–Schottky emission was responsible, to some extent, for the transport of charge carriers in the polymer. The conductivity of the films increased on doping with iodine. The dopant molecules are considered to act as additional trapping centes and provide links between the polymer molecules in the amorphous region, thus resulting in the formation of charge transfer complexes. 相似文献
30.