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91.
二甲苯是一种重要的人为源 VOC, 也是城市地区 SOA 的重要前体物。二甲苯光氧化形成的 SOA 受多种环
境因素影响, 而 NH3 对该反应形成的 SOA 生成产率及反应机制的影响尚不清楚。基于室内烟雾箱模拟系统, 探讨了
NH3 对二甲苯光氧化形成 SOA 质量浓度、物理特性及化学组成的影响。研究表明, 在低浓度条件下, NH3 对二甲苯
光氧化生成 SOA 具有明显的促进作用, 结合气溶胶质谱结果发现 NH3 促进醛酮类物质进入颗粒相以及含氮有机物的
生成是导致 SOA 质量浓度增加的主要原因。此外, NH3 能够提高邻二甲苯生成 SOA 的吸光度, 但是对对二甲苯无明
显影响。分析表明, 相较于对二甲苯, 邻二甲苯光氧化会生成大量醛类物质, NH3 与醛类发生美拉德反应是导致 SOA
吸光性增加的主要原因。 相似文献
92.
目的本实验探索驾驶负荷累积与轻音乐对驾驶疲劳的影响。方法采用2(驾驶负荷累积)×2(音乐条件)×3(模拟驾驶阶段)混合设计,对32名驾驶员被试进行模拟驾驶实验,采集驾驶员驾驶速度和他们的垂直搜索广度与瞳孔直径。结果第45-60 min时,对于无驾驶负荷累积的被试,轻音乐组车速显著快于无音乐组,轻音乐组垂直搜索广度显著大于无音乐组;对于有驾驶负荷累积的被试,轻音乐组的瞳孔直径小于无音乐组(边缘显著),轻音乐组的车速慢于无音乐组。结论轻音乐对无累积疲劳的驾驶员具有唤醒作用,加快他们的车速,扩大垂直搜索广度,对驾驶绩效具有积极的影响;轻音乐对有累积疲劳的驾驶员会产生催眠作用,缩小瞳孔直径,车速减慢,对驾驶绩效具有消极的影响。 相似文献
93.
Poly(N‐phenylglycine)‐Based Nanoparticles as Highly Effective and Targeted Near‐Infrared Photothermal Therapy/Photodynamic Therapeutic Agents for Malignant Melanoma 下载免费PDF全文
Bang‐Ping Jiang Li Zhang Xiao‐Lu Guo Xing‐Can Shen Yan Wang Yang Zhu Hong Liang 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(8)
Malignant melanoma is a highly aggressive tumor resistant to chemotherapy. Therefore, the development of new highly effective therapeutic agents for the treatment of malignant melanoma is highly desirable. In this study, a new class of polymeric photothermal agents based on poly(N‐phenylglycine) (PNPG) suitable for use in near‐infrared (NIR) phototherapy of malignant melanoma is designed and developed. PNPG is obtained via polymerization of N‐phenylglycine (NPG). Carboxylate functionality of NPG allows building multifunctional systems using covalent bonding. This approach avoids complicated issues typically associated with preparation of polymeric photothermal agents. Moreover, PNPG skeleton exhibits pH‐responsive NIR absorption and an ability to generate reactive oxygen species, which makes its derivatives attractive photothermal therapy (PTT)/photodynamic therapy (PDT) dual‐modal agents with pH‐responsive features. PNPG is modified using hyaluronic acid (HA) and polyethylene glycol diamine (PEG‐diamine) acting as the coupling agent. The resultant HA‐modified PNPG (PNPG‐PEG‐HA) shows negligible cytotoxicity and effectively targets CD44‐overexpressing cancer cells. Furthermore, the results of in vitro and in vivo experiments reveal that PNPG‐PEG‐HA selectively kills B16 cells and suppresses malignant melanoma tumor growth upon exposure to NIR light (808 nm), indicating that PNPG‐PEG‐HA can serve as a very promising nanoplatform for targeted dual‐modality PTT/PDT of melanoma. 相似文献
94.
Tissue Engineering: Effective Light Directed Assembly of Building Blocks with Microscale Control (Small 24/2017) 下载免费PDF全文
95.
Tuomas Haggren Ali Shah Anton Autere Joona-Pekko Kakko Veer Dhaka Maria Kim Teppo Huhtio Zhipei Sun Harri Lipsanen 《Nano Research》2017,10(8):2657-2666
Light management and electrical isolation are essential for the majority of optoelectronic nanowire (NW) devices.Here,we present a cost-effective technique,based on vapor-phase deposition of parylene-C and subsequent annealing,that provides conformal encapsulation,anti-reflective coating,improved optical properties,and electrical insulation for GaAs nanowires.The process presented allows facile encapsulation and insulation that is suitable for any nanowire structure.In particular,the parylene-C encapsulation functions as an efficient antireflection coating for the nanowires,with reflectivity down to <1% in the visible spectrum.Furthermore,the parylene-C coating increases photoluminescence intensity,suggesting improved light guiding to the NWs.Finally,based on this process,a NW LED was fabricated,which showed good diode performance and a clear electroluminescence signal.We believe the process can expand the fabrication possibilities and improve the performance of optoelectronic nanowire devices. 相似文献
96.
Under water-rich conditions, small amphiphilic and hydrophobic drug molecules self-assemble into supramolecular nanostructures. Thus, substantial modifications in their interaction with cellular structures and the ability to reach intracellular targets could happen. Additionally, drug aggregates could be more toxic than the non-aggregated counterparts, or vice versa. Moreover, since self-aggregation reduces the number of effective “monomeric” molecules that interact with the target, the drug potency could be underestimated. In other cases, the activity could be ascribed to the non-aggregated molecule while it stems from its aggregates. Thus, drug self-assembly could mislead from drug throughput screening assays to advanced preclinical and clinical trials. Finally, aggregates could serve as crystallization nuclei. The impact that this phenomenon has on the biological performance of active compounds, the inconsistent and often controversial nature of the published data and the need for recommendations/guidelines as preamble of more harmonized research protocols to characterize drug self-aggregation were main motivations for this review. First, the key molecular and environmental parameters governing drug self-aggregation, the main drug families for which this phenomenon and the methods used for its characterization are described. Then, promising nanotechnology platforms investigated to prevent/control it towards a more efficient drug development process are briefly discussed. 相似文献
97.
Evaporation‐ and Solution‐Process‐Feasible Highly Efficient Thianthrene‐9,9′,10,10′‐Tetraoxide‐Based Thermally Activated Delayed Fluorescence Emitters with Reduced Efficiency Roll‐Off 下载免费PDF全文
98.
99.
Jun Pan Li Na Quan Yongbiao Zhao Wei Peng Banavoth Murali Smritakshi P. Sarmah Mingjian Yuan Lutfan Sinatra Noktan M. Alyami Jiakai Liu Emre Yassitepe Zhenyu Yang Oleksandr Voznyy Riccardo Comin Mohamed N. Hedhili Omar F. Mohammed Zheng Hong Lu Dong Ha Kim Edward H. Sargent Osman M. Bakr 《Advanced materials (Deerfield Beach, Fla.)》2016,28(39):8718-8725
100.