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941.
A mathematical model has been developed for the simulation of the ammonia oxidation in a reverse flow reactor. Computer simulations were carried out with a kinetic scheme, based upon elementary reaction steps. Aim was to explore the potential of a reverse flow reactor for selective oxidation of NH3 to produce either N2, NO, or N2O via a dedicated operation procedure. Therefore, the conversion of NH3 and the selectivity toward N2, NO, or N2O, were compared for a reverse flow operation and a steady state, once-through operation.A new operation concept of reverse flow operation in combination with a periodically lower feed concentration is proposed. The novel reactor concept shows a better performance compared to normal reverse flow operation and to steady state, once-through operation. The results indicate that reverse flow operation can be applied for manipulation of conversion and selectivity. A periodically lower feed concentration may increase the conversion, even up to levels that exceed the steady state value. 相似文献
942.
Large aggregation interval asymptotics are used to investigate the relation between Granger causality in disaggregated vector autoregressions (VARs) and associated contemporaneous correlation among innovations of the aggregated system. One of our main contributions is that we outline various conditions under which the informational content of error covariance matrices yields insight into the causal structure of the VAR. Monte Carlo results suggest that our asymptotic findings are applicable even when the aggregation interval is small, as long as the time series are not characterized by high levels of persistence. 相似文献
943.
The contact time of particles at the walls of gas fluidized beds has been studied using a radioactive particle tracking technique to monitor the position of a radioactive tracer. The solids used were sand or FCC particles fluidized by air at room temperature and atmospheric pressure at various superficial velocities, covering both bubbling and turbulent regimes of fluidization. Based on the analysis of tracer positions, the motion of individual particles near the walls of the fluidized bed was studied. The contact time, contact distance and contact frequency of the particles at the wall were evaluated from these experimental data. It was found that in a bed of sand particles, the mean wall contact time of the fluidized bed of sand particles decreases by increasing the gas velocity in the bubbling and increases in the turbulent fluidization. In other words, the particle-wall contact time is minimum at the onset of turbulent fluidization in the bed of sand particles. However, the mean wall contact time is almost constant in both regimes of fluidization in the bed of FCC particles. All the existing models in the literature predict a decreasing contact time when the gas velocity in the bed is increased. It was also shown that the contact distance increases monotonously by increasing the gas velocity in the bed of sand particles, while it is almost constant for the bed of FCC particles. Contact frequency has a trend similar to that of the contact time for both sand and FCC particles. 相似文献
944.
A thin circular film clamped at the periphery is adhered to the planar surface of a rigid cylindrical punch. An external tensile load is applied to the punch, causing the film to delaminate from the substrate and the circular contact edge to contract. The film spontaneously separates from the punch, or pulls off, when the contact radius reduces to a range between 0.1758 and 0.3651 of the film radius, depending on the magnitude of the residual membrane stress. The mechanical delamination process is derived by a thermodynamic energy balance based on a coupled interfacial adhesion and residual membrane stress. The theoretical model has significant implications in nanoforce measurement, microelectromechanical systems (MEMS) comprising active moveable films, and biological cell adhesion. 相似文献
945.
Mohit Singh 《Chemical engineering science》2003,58(1):1-18
The interplay of viscous, gravity and capillary forces determines the flow behavior of two or more phases through porous materials. In this study, a rule-based dynamic network model is developed to simulate two-phase flow in three-dimensional porous media. A cubic network analog of porous medium is used with cubic bodies and square cross-section throats. The rules for phase movement and redistribution are devised to honor the imbibition and drainage physics at pore scale. These rules are based on the pressure field within the porous medium that is solved for by applying mass conservation at each node. The pressure field governs the movement and flow rates of the fluids within the porous medium. Film flow has been incorporated in a novel way. A pseudo-percolation model is proposed for low but non-zero capillary number (ratio of viscous to capillary forces). The model is used to study primary drainage with constant inlet flow rate and constant inlet pressure boundary conditions. Non-wetting phase front dynamics, apparent wetting residuals (Swr), and relative permeability are computed as a function of capillary number (Nca), viscosity ratio (M), and pore-throat size distribution. The simulation results are compared with experimental results from the literature. Depending upon the flow rate and viscosity ratio, the displacement front shows three distinct flow patterns—stable, viscous fingering and capillary fingering. Capillary desaturation curves (Swr vs. Nca) depend on the viscosity ratio. It is shown that at high flow rates (or high Nca), relative permeability assumes a linear dependence upon saturation. Pseudo-static capillary pressure curve is also estimated (by using an invasion percolation model) and is compared with the dynamic capillary pressure obtained from the model. 相似文献
946.
Three-dimensional solid-liquid flow is mathematically formulated by means of the "two-fluid" approach and the two-phase k-ε-Ap turbulence model. The turbulent fluctuation correlations appearing in the Reynolds time averaged governing equations are fully incorporated. The solid-liquid flow field and solid concentration distribution in baffled stirred tanks with a standard Rushton impeller are numerically simulated using an improved "inner-outer" iterative procedure. The flow pattern is identified via the velocity vector plots and a recirculation loop with higher solid concentration is observed in the central vicinity beneath the impeller. Comparison of 相似文献
947.
948.
V. Singh 《Chemical engineering science》2006,61(20):6855-6866
A study of non-wetting flow in a packed bed under the influence of gas flow has been carried out. Departing from the usual continuum models, a discrete and deterministic model for liquid flow has been presented to model the liquid flow from single and multiple point sources. Liquid flow is modelled based on force balance approach considering gas drag, bed resistance and gravity forces. Gas flow is modelled using k-ε model for turbulent flow. An X-ray flow visualization technique, developed by our group, is used to study the liquid flow paths in the packed bed. Liquid flow path and velocity has been obtained for various liquid and gas flow rate. Flow paths obtained from the simulation results are in good agreement to those obtained from flow visualization procedure under various conditions. Also, liquid distribution at the bed bottom is reported and compared with the experimental results. 相似文献
949.
950.
基于流动平衡的塑料挤出模优化设计 总被引:1,自引:0,他引:1
在构建流道三维参数化模型的基础上,将有限元数值分析和优化技术相结合,以口模出口处型材截面上各子区域平均流速相等为优化目标,以压缩段入口壁厚和平直段长度为设计变量,对挤出模优化设计进行了研究。并以实例说明了优化设计的具体过程,验证了所用方法的正确性和有效性。 相似文献